US2943058A - Liquid detergent compositions - Google Patents

Liquid detergent compositions Download PDF

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Publication number
US2943058A
US2943058A US615761A US61576156A US2943058A US 2943058 A US2943058 A US 2943058A US 615761 A US615761 A US 615761A US 61576156 A US61576156 A US 61576156A US 2943058 A US2943058 A US 2943058A
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liquid detergent
water
diethanolamide
ethanol
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US615761A
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Daniel A Cook
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Diamond Shamrock Corp
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Diamond Alkali Co
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    • CCHEMISTRY; METALLURGY
    • C11ANIMAL OR VEGETABLE OILS, FATS, FATTY SUBSTANCES OR WAXES; FATTY ACIDS THEREFROM; DETERGENTS; CANDLES
    • C11DDETERGENT COMPOSITIONS; USE OF SINGLE SUBSTANCES AS DETERGENTS; SOAP OR SOAP-MAKING; RESIN SOAPS; RECOVERY OF GLYCEROL
    • C11D1/00Detergent compositions based essentially on surface-active compounds; Use of these compounds as a detergent
    • C11D1/66Non-ionic compounds
    • C11D1/83Mixtures of non-ionic with anionic compounds
    • C11D1/831Mixtures of non-ionic with anionic compounds of sulfonates with ethers of polyoxyalkylenes without phosphates

Definitions

  • This invention relates to a novel liquid detergent composition, and more particularly relates to a new and improved liquid detergent characterized by excellent cleansing power" and larity throughout a wide range of temperatures' and with water of varying "degrees of hardness.
  • Liquid detergents have found application in a variety of washing andcleansing operations, e.g., in dishwashirig, windowwashing, hand cleaning, machinery cleansing and a variety of applications in the dairy. industry in cleaning milking machines, inflations, utensils, milk tanks, pipelines, milk cans, and the like.
  • a further object of this invention is to'provide a new and improved liquid detergent which is characterized by a desirable viscosity, color, film characteristics, hard water resistance, cold weather properties and excellent detergency.
  • the present invention contemplates a liquid detergent composition
  • a liquid detergent composition comprising 'in admixture the following ingiedients: J
  • a liquid detergent composition of the above type is found to have a desirable viscosity and yet is not thick enough to cause difliculty in pouring nor is it subject to freezing at any typically-encountered low temperature. Further, a liquid detergent of the above composition has a desirable color, excellent sudsing characteristics, and is characterized by clarity and an absence of cloud point up to C. and an excellent hard water resistance whereby clear solutions are provided in water having hardness values ranging from 10-100 grains or more.
  • alkyl aryl sulfonate as used throughout the specification and claims is intended, of course, to refer to various alkyl aryl sulfonates and their alkali metal salts such as sodium salts, potassium salts, andthe like.
  • Preferred alkyl aryl sulfonates are alkyl benzene, toluene, and/or naphthalene sulfonates where the alkyl group contains from about 4 to 18, preferably 10-14, carbon atoms, e. g., sodium dodecyl aryl derivatives derived from propylene tetramer or kerosene fractions (keryl) averaging 12 carbon atoms.
  • a specific preferred alkyl aryl sulfonate is sodium dodecyl benzene sulfonate.
  • Such a material is available commercially as Ultra-Wet 35 KX which typically comprises an aqueous solution of 68% by weight water and 32% by weight sodiumdodecyl benzene sulfonate.
  • alkyl aryl polyether alcohol as used throughout the specification and claims is intended, of course, to refer to various alkyl aryl polyether alkanols,
  • alkyl benzene polyoxyethylene hydroxides These compounds can be prepared by constituent isocyclicw hydroxy compounds having as a substituent in the nucleus at least one hydrocarbon or acyclic radical of at least 4 carbon atoms, withethylene oxide. Suitable isocyclic compounds are normal butyl phenol, 'diisobutyl phenol, dodecyl phenol, and the like. The condensation can be carried out at an elevated temperature in the presence of an alkali. For example, 206 parts by weight of p-isooctyl phenol are melted and combined with 2 parts by weight of a 40% caustic soda solution. To this mixture there is introduced ethylene oxide at 130 C. until a total of 10 molecules have been adsorbed for each molecule of the phenol. A commercially available product of this type is Triton X-lOO.
  • alkanolamide as used throughout the specification and claims is intended to refer to various alkanolamides, especially monoand dialkanolamides such as monoand diethanolamides, dimethanolamides, ethanol-' amides, methanolamides, and the like, although a diethanolamide is preferred at present, such as the commercially available product as Solar CO which is obtained by reacting coconutzoil with diethanolamine and typically comprises a mixture of 72% by weight diethanolamide, 1% by weight diethanolamine laurate, 21% by weight diethanolamine and 6% by weight glycerine.
  • Solar CO which is obtained by reacting coconutzoil with diethanolamine and typically comprises a mixture of 72% by weight diethanolamide, 1% by weight diethanolamine laurate, 21% by weight diethanolamine and 6% by weight glycerine.
  • polyoxyalkylene alkanol as used throughout the specification and claims, is intended to refer to various compounds of this type, especially polyoxyalkylene ethanols.
  • An illustrative and preferred polyalkylene ethanol compound is tridecyl polyoxyethylene ethanol.
  • a commercially available material of this type is the product known as Emulphor BC-840 which is a liquid, 100% active polyoxyalkylene ethanol.
  • antifreeze as used throughout the specifi- I cation and claims generally refers to organic compounds which may be added to prevent freezing of the liquid detergent composition. At present, it is preferred to employ a mixture of antifreeze compounds, notably a mixture of about equal proportions of (1) an alkylene glycol such as hexylene glycol and (2) an'alkanol such as methanol, ethanol, or the like. It will be appreciated, of course, that in certain instances, antifreeze'compounds need not be added whenthe intended application does not involve exposure to freezing temperatures.
  • sequestrant as used throughout the specification and claims, is intended to refer to additives capable of preventing sludge formation in hard water or other undesirable clouding.
  • a preferred type of Sequestrant at present is the commercially available material known as Sequesterene or Nullapon, which istetrasodium salt of ethylene diamine tetra-acetic acid.
  • Liquid detergents embodying the present invention can be prepared by mixing the specified ingredients in the indicated amounts.
  • the proportion ranges specified are critical and should be mentioned if the advantageous results characterizing the practice of this invention are to be obtained.
  • Example I An illustrative liquid detergent in accordance with the present invention is as follows:
  • a liquid detergent composition characterized by a high degree of clarity and absence of a cloud point up to C. and capable of providing clear solutions in water having hardness values ranging from 10 to 100 grains, said detergent comprising in admixture the following ingredients:
  • a liquid detergent composition characterized by a high degree of clarity and absence of a cloud pointup to 100 C. and capable of providing clear solutions'in. water having hardness values ranging from' 10 to 100. grains, said'detergent comprising in admixture the follow-' ing ingredients:

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  • Chemical & Material Sciences (AREA)
  • Life Sciences & Earth Sciences (AREA)
  • Engineering & Computer Science (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Oil, Petroleum & Natural Gas (AREA)
  • Wood Science & Technology (AREA)
  • Organic Chemistry (AREA)
  • Detergent Compositions (AREA)

Description

United States Patent LIQUID DETERGENT COMPOSITIONS Daniel A. Cook, Mentor Township, Lake County, Ohio, assignor to Diamond Alkali Company, Cleveland, Ohio,
a corporation "of Delaware This invention relates to a novel liquid detergent composition, and more particularly relates to a new and improved liquid detergent characterized by excellent cleansing power" and larity throughout a wide range of temperatures' and with water of varying "degrees of hardness.
Until fairly recently, general purpose detergents frequently have been solid powders comprising mixtures of alkali andsoap adapted to be dissolved in water and applied as solutions. Various liquid organic substances, notably liquid non-ionic wettable agents, have demonstrated superiority in soil removal, sudsing ability and other desirable properties and have been proposed as additives to powdered detergents. These liquids are, of course, limited inthe amount in which they can be incorporated into a powder or granular material without destroying its particulate nature. Moreover, dusting and caking of dry detergents are frequently difficult to control so that considerable interest has been directed toward liquid detergents. v
Liquid detergents have found application in a variety of washing andcleansing operations, e.g., in dishwashirig, windowwashing, hand cleaning, machinery cleansing and a variety of applications in the dairy. industry in cleaning milking machines, inflations, utensils, milk tanks, pipelines, milk cans, and the like.
' Prior liquid detergents 'comprising a major portion of liquid non-ionicadditives, or a mixture of non-ionic and anionic surface active agents have not been completely satisfactory. Anionic materials alone frequently do not provide desirable results in hard water. On the other hand, it has been found that a liquid non-ionic substance lay itself does not provide an entirely satisfactory material, notably because of a disadvantageous cloud point. Accordingly, there has been a continuing interest in seeking new and improved liquid detergents.
Accordingly, it is a principal object of the present invention to provide a new and improved general purpose liquid; detergent which avoids the difiiculties heretofore encountered.
A further object of this invention is to'provide a new and improved liquid detergent which is characterized by a desirable viscosity, color, film characteristics, hard water resistance, cold weather properties and excellent detergency.
These and other objects and advantages of the present invention will appear more fully from the following description-thereof,
The present invention contemplates a liquid detergent composition comprising 'in admixture the following ingiedients: J
.l l Parts (21) Alkyl-arylsul-fonate- (100% active) a 6-9 (b) Alkyl aryl polyether alcohol (100% active) 23-26 (0) At least one substance selected from the group consisting of:
"ice
A liquid detergent composition of the above type is found to have a desirable viscosity and yet is not thick enough to cause difliculty in pouring nor is it subject to freezing at any typically-encountered low temperature. Further, a liquid detergent of the above composition has a desirable color, excellent sudsing characteristics, and is characterized by clarity and an absence of cloud point up to C. and an excellent hard water resistance whereby clear solutions are provided in water having hardness values ranging from 10-100 grains or more.
The expression alkyl aryl sulfonate as used throughout the specification and claims is intended, of course, to refer to various alkyl aryl sulfonates and their alkali metal salts such as sodium salts, potassium salts, andthe like. Preferred alkyl aryl sulfonates are alkyl benzene, toluene, and/or naphthalene sulfonates where the alkyl group contains from about 4 to 18, preferably 10-14, carbon atoms, e. g., sodium dodecyl aryl derivatives derived from propylene tetramer or kerosene fractions (keryl) averaging 12 carbon atoms. A specific preferred alkyl aryl sulfonate is sodium dodecyl benzene sulfonate. Such a material is available commercially as Ultra-Wet 35 KX which typically comprises an aqueous solution of 68% by weight water and 32% by weight sodiumdodecyl benzene sulfonate.
The expression alkyl aryl polyether alcohol as used throughout the specification and claims is intended, of course, to refer to various alkyl aryl polyether alkanols,
, notably ethanol, such as alkyl benzene polyoxyethylene hydroxides These compounds can be prepared by constituent isocyclicw hydroxy compounds having as a substituent in the nucleus at least one hydrocarbon or acyclic radical of at least 4 carbon atoms, withethylene oxide. Suitable isocyclic compounds are normal butyl phenol, 'diisobutyl phenol, dodecyl phenol, and the like. The condensation can be carried out at an elevated temperature in the presence of an alkali. For example, 206 parts by weight of p-isooctyl phenol are melted and combined with 2 parts by weight of a 40% caustic soda solution. To this mixture there is introduced ethylene oxide at 130 C. until a total of 10 molecules have been adsorbed for each molecule of the phenol. A commercially available product of this type is Triton X-lOO.
The term alkanolamide as used throughout the specification and claims is intended to refer to various alkanolamides, especially monoand dialkanolamides such as monoand diethanolamides, dimethanolamides, ethanol-' amides, methanolamides, and the like, although a diethanolamide is preferred at present, such as the commercially available product as Solar CO which is obtained by reacting coconutzoil with diethanolamine and typically comprises a mixture of 72% by weight diethanolamide, 1% by weight diethanolamine laurate, 21% by weight diethanolamine and 6% by weight glycerine.
The expression polyoxyalkylene alkanol, as used throughout the specification and claims, is intended to refer to various compounds of this type, especially polyoxyalkylene ethanols. An illustrative and preferred polyalkylene ethanol compound is tridecyl polyoxyethylene ethanol. A commercially available material of this type is the product known as Emulphor BC-840 which is a liquid, 100% active polyoxyalkylene ethanol.
The term antifreeze as used throughout the specifi- I cation and claims generally refers to organic compounds which may be added to prevent freezing of the liquid detergent composition. At present, it is preferred to employ a mixture of antifreeze compounds, notably a mixture of about equal proportions of (1) an alkylene glycol such as hexylene glycol and (2) an'alkanol such as methanol, ethanol, or the like. It will be appreciated, of course, that in certain instances, antifreeze'compounds need not be added whenthe intended application does not involve exposure to freezing temperatures.
The term sequestrant, as used throughout the specification and claims, is intended to refer to additives capable of preventing sludge formation in hard water or other undesirable clouding. A preferred type of Sequestrant at present is the commercially available material known as Sequesterene or Nullapon, which istetrasodium salt of ethylene diamine tetra-acetic acid. Other polyamino polycarboxylic acids, salts and derivatives thereof, as well as difierent compatible sequestrants, also may be used.
Liquid detergents embodying the present invention can be prepared by mixing the specified ingredients in the indicated amounts. The proportion ranges specified are critical and should be mentioned if the advantageous results characterizing the practice of this invention are to be obtained.
In order that those skilled in the art may more completely understand the present invention and the preferred methods by which the same may be carried into effect, the following specific examples are offered:
Example I An illustrative liquid detergent in accordance with the present invention is as follows:
Percent by weight Alkyl aryl sulfonate (32% active) Ultrawet 35 KX 25.0 (8.0% active) Alkyl aryl polyether alcohol (100% active) Triton Polyoxyalkalene alkanol (100% active) Emulphor Hexylene glycol Ethanol (denatured) 3.0 Sequestrant (Sequestrene) 0.1 Water Balance Example 11 Another illustrative liquid detergent formulation in accordance with the present invention is the following: Percent by weight Alkyl aryl sulfonate (32% active) Ultrawet 35 KX 21.7 (7.0% active) Alkyl aryl polyether alcohol (100% active) Triton 0 25.0 Alkanolamide (72% diethanolamide)-Solar CO 5.0 Hexylene glycol 3.0 Ethanol (denatured) 3.0 Sequestrant (Sequestrene) 0.1 Water Balance It is to be understood that although the invention has been described with specific reference to particular embodiments thereof, it'is not to be so limited, since changes and alterations therein may be made which are -withini 4 the full intended scope of this invention as defined b the appended claims.
What is claimed is:
1. A liquid detergent composition characterized by a high degree of clarity and absence of a cloud point up to C. and capable of providing clear solutions in water having hardness values ranging from 10 to 100 grains, said detergent comprising in admixture the following ingredients:
Percent by weight.
2. A liquid detergent composition characterized by a= high degree of clarity and absence of a cloudpoint up to 100 C. and capable of providing clear solutions in Water having hardness values ranging'from 10 to 100 grains, said detergent comprising in admixture the following ingredients:
' Percent: by weight (a) Sodium dodecyl benzene sulfonate 7.
(b) Alkyl benzene polyether ethanol 25 (c) Diethanolamide mixture consisting essentially of 72% by weight diethanolamide, 1% by weight diethanolamine laurate, 21% by weight diethanolamine, and 6% by weight glycerine 5 (a') Hexylene glycol 3. (e) Ethanol 3' (f) Tetrasodium salt of ethylene diamine tetra-acetic acid 0:1 Balance 3. A liquid detergent composition characterized by a high degree of clarity and absence of a cloud pointup to 100 C. and capable of providing clear solutions'in. water having hardness values ranging from' 10 to 100. grains, said'detergent comprising in admixture the follow-' ing ingredients:
Percent by weight (a) Sodium dodecyl benzene sulfonate 8. (b) Alkyl benzene polyether ethanol 24 (c) Tridecylpolyoxyethylene alcohol 5 (d) Hexylene glycol 3 (e) Ethyl alcohol 3:
(f) Tetrasodium salt of ethylene diamine tetra-acetic acid (g) Water References Cited in the file of this patent UNITED STATES PATENTS Vitale et al. June- 15, 1954 Bloch et al Sept. 6,,1955' Epstein et al. Jan. 31, 1956 OTHER REFERENCESv Hexylene Glycol, Tech. Booklet SC: 50-1, 19.50. Shell- Chem. Corp., N.Y., pp. 8, 9 and 21.
Sequestrene, pub. of Geigy Ind. Chem., N.Y., 1952, pp. 42 and 43. j
0.1 Balance UNITED STATES PATENT OFFICE CETlFICATE OF CORECTION Patent Nor, 2343 058 June 28 1960 Daniel Cook It is hereby certified that error appears in the-printed specification of the above numbered patent requiring correction and that the said Letters Patent should read as corrected below.
Column 1 line 18 for "larity" read clarity line 25 for "wettable" read wetting =3 column 2, lines 36 and 37 for "constituent" read condensing =-=g line 58,, after product insert known =3 same column 2 line 66 for "p0ly=" read polyoxy column 4 line l4; at the end of the line under Percent by weight insert we 5 same column 4 lines 20 and 21 at the end of the line under Per cent by weightm strike out they-numerals "5% each occurrence,
Signed and sealed this 3rd day of January 1961.,
(SEAL) Attest:
KARL H, AXLINE ROBERT C. WATSON Attesting Ofilcer Commissioner of Patents

Claims (1)

1. A LIQUID DETERGENT COMPOSITION CHARACTERIZED BY A HIGH DEGREE OF CLARITY AND ABSENCE OF A CLOUD POINT UP TO 100*C. AND CAPABLE OF PROVIDING CLEAR SOLUTIONS IN WATER HAVING HARDNESS VALUES RANGING FROM 10 TO 100 GRAINS, SAID DETERGENT COMPRISING IN ADMIXTURE THE FOLLOWING INGREDIENTS: PERCENT BY WEIGHT (A) SODIUM DODECYL BENZENE SULFONATE ------ 7-8 (B) ALKYL BENZENE POLYETHER ETHANOL ------- 24-25 (C) AT LEAST ONE SUBSTANCE SELECTED FROM THE GROUP CONSISTING OF: (1) DIETHANOLAMIDE MIXTURE CONSISTING ESSENTIALLY OF 72% BY WEIGHT DIETHANOLAMIDE, 1% BY WEIGHT DIETHANOLAMINE LAURATE, 21% BY WEIGHT DIETHANOLAMINE, AND 6% BY WEIGHT GLYCERINE ----------------------- 5 (2) TRIDECYL POLYOXYETHYLENE ALCOHOL ---- 5 (D) HEXYLENE GLYCOL ----------------------- 3 (E) ETHYL ALCOHOL ------------------------- 3 (F) TETRASODIUM SALT OF ETHYLENE DIAMINE TETRAACETIC ACID ------------------------------ 0.1 (G) WATER --------------------------------- BALANCE
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Cited By (17)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US3222201A (en) * 1962-12-28 1965-12-07 Union Carbide Corp Cleaning and coating formulation
US3232880A (en) * 1961-04-10 1966-02-01 Ultra Chemical Works Inc Liquid detergent composition
US3239468A (en) * 1961-05-26 1966-03-08 Colgate Palmolive Co Hard surface cleaning compositions
US3257479A (en) * 1961-11-13 1966-06-21 Monsanto Co Amino-di-alkylene phosphonic acid esters
US3264242A (en) * 1961-10-03 1966-08-02 Dow Chemical Co Aqueous dispersions containing alkylated diphenyloxidedisulfonic acid and a non-ionic surface active agent
US3265625A (en) * 1962-10-30 1966-08-09 C P Baker & Company Liquid detergent
US3282852A (en) * 1962-05-11 1966-11-01 Colgate Palmolive Co Heavy duty liquid detergents
US3383328A (en) * 1966-04-04 1968-05-14 Navy Usa Water displacing and rust preventive compositions
US3404004A (en) * 1965-03-08 1968-10-01 Jean R. Ake Final soak bath for processed silver halide prints
US3491027A (en) * 1966-02-28 1970-01-20 Us Navy Composition and method for cleaning salt residues from metal surfaces
US3642506A (en) * 1969-11-28 1972-02-15 Swift & Co Method for improving the properties of hydraulic cementitious mixtures
US3914185A (en) * 1973-03-15 1975-10-21 Colgate Palmolive Co Method of preparing liquid detergent compositions
US3931033A (en) * 1973-12-14 1976-01-06 Henkel & Cie G.M.B.H. Liquid foam-regulated nonionic detergent compositions
DE2527165A1 (en) * 1974-06-21 1976-01-08 Procter & Gamble LIQUID HEAVY DUTY DETERGENT
US3953380A (en) * 1970-10-28 1976-04-27 Colgate-Palmolive Company Liquid detergent
FR2563840A1 (en) * 1984-05-02 1985-11-08 Camp Sa Liquid detergents for hard surfaces
US4717507A (en) * 1985-05-04 1988-01-05 Henkel Kommanditgesellschaft Auf Aktien Liquid detergent with fabric softening properties

Citations (3)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
USRE23840E (en) * 1950-05-03 1954-06-15 Liquid anionic-dialkylolamide
US2717243A (en) * 1955-09-06 Non-caking alkyl aryl sulfonate
US2733212A (en) * 1956-01-31 Hair shampoo

Patent Citations (3)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US2717243A (en) * 1955-09-06 Non-caking alkyl aryl sulfonate
US2733212A (en) * 1956-01-31 Hair shampoo
USRE23840E (en) * 1950-05-03 1954-06-15 Liquid anionic-dialkylolamide

Cited By (18)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US3232880A (en) * 1961-04-10 1966-02-01 Ultra Chemical Works Inc Liquid detergent composition
US3239468A (en) * 1961-05-26 1966-03-08 Colgate Palmolive Co Hard surface cleaning compositions
US3264242A (en) * 1961-10-03 1966-08-02 Dow Chemical Co Aqueous dispersions containing alkylated diphenyloxidedisulfonic acid and a non-ionic surface active agent
US3257479A (en) * 1961-11-13 1966-06-21 Monsanto Co Amino-di-alkylene phosphonic acid esters
US3282852A (en) * 1962-05-11 1966-11-01 Colgate Palmolive Co Heavy duty liquid detergents
US3265625A (en) * 1962-10-30 1966-08-09 C P Baker & Company Liquid detergent
US3222201A (en) * 1962-12-28 1965-12-07 Union Carbide Corp Cleaning and coating formulation
US3404004A (en) * 1965-03-08 1968-10-01 Jean R. Ake Final soak bath for processed silver halide prints
US3491027A (en) * 1966-02-28 1970-01-20 Us Navy Composition and method for cleaning salt residues from metal surfaces
US3383328A (en) * 1966-04-04 1968-05-14 Navy Usa Water displacing and rust preventive compositions
US3642506A (en) * 1969-11-28 1972-02-15 Swift & Co Method for improving the properties of hydraulic cementitious mixtures
US3953380A (en) * 1970-10-28 1976-04-27 Colgate-Palmolive Company Liquid detergent
US3914185A (en) * 1973-03-15 1975-10-21 Colgate Palmolive Co Method of preparing liquid detergent compositions
US3931033A (en) * 1973-12-14 1976-01-06 Henkel & Cie G.M.B.H. Liquid foam-regulated nonionic detergent compositions
DE2527165A1 (en) * 1974-06-21 1976-01-08 Procter & Gamble LIQUID HEAVY DUTY DETERGENT
DE2527101A1 (en) * 1974-06-21 1976-01-08 Procter & Gamble LIQUID HEAVY DUTY DETERGENT
FR2563840A1 (en) * 1984-05-02 1985-11-08 Camp Sa Liquid detergents for hard surfaces
US4717507A (en) * 1985-05-04 1988-01-05 Henkel Kommanditgesellschaft Auf Aktien Liquid detergent with fabric softening properties

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