US2462018A - X-ray opaque marking means - Google Patents

X-ray opaque marking means Download PDF

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Publication number
US2462018A
US2462018A US546907A US54690744A US2462018A US 2462018 A US2462018 A US 2462018A US 546907 A US546907 A US 546907A US 54690744 A US54690744 A US 54690744A US 2462018 A US2462018 A US 2462018A
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US
United States
Prior art keywords
metal
blocking
colloidal
rays
wax
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Expired - Lifetime
Application number
US546907A
Inventor
William H Wood
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Harris Corp
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Harris Seybold Potter Co
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Publication date
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Priority to US546907A priority Critical patent/US2462018A/en
Application granted granted Critical
Publication of US2462018A publication Critical patent/US2462018A/en
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Expired - Lifetime legal-status Critical Current

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    • GPHYSICS
    • G03PHOTOGRAPHY; CINEMATOGRAPHY; ANALOGOUS TECHNIQUES USING WAVES OTHER THAN OPTICAL WAVES; ELECTROGRAPHY; HOLOGRAPHY
    • G03BAPPARATUS OR ARRANGEMENTS FOR TAKING PHOTOGRAPHS OR FOR PROJECTING OR VIEWING THEM; APPARATUS OR ARRANGEMENTS EMPLOYING ANALOGOUS TECHNIQUES USING WAVES OTHER THAN OPTICAL WAVES; ACCESSORIES THEREFOR
    • G03B42/00Obtaining records using waves other than optical waves; Visualisation of such records by using optical means
    • G03B42/02Obtaining records using waves other than optical waves; Visualisation of such records by using optical means using X-rays
    • G03B42/04Holders for X-ray films
    • G03B42/047Holders for X-ray films provided with marking means

Definitions

  • markings or blocking-out as desired may be applied on the film holder or casette or on a sheet of material laid thereon and can be easily and quickly removed therefrom after the exposure, the negative carrying the required markings or blocking, while the film holder is ready for re-use.
  • special markings not available in stock forms may be employed and areas may be circled or otherwise identified or blocked out, as desired, all with improved speed and facility.
  • the invention comprises the features hereinafter fully described, and particularly pointed out in the claims, the following description setting forth in detail certain illustrative embodiments of the invention, these being indicative however, of but a few of the various ways in which the principle of the invention may be employed.
  • a pencil or crayon comprising a material in fine particle size having metal atoms of high atomic weight, in a carrier or vehicle substance.
  • metal of high atomic weight is here meant a metal of atomic weight at least 184. and particularly conveniently available are such metals as lead, bismuth, thallium, etc.
  • the metal is in colloidal form, as may be provided by the known methods of preparing metals in colloidal condition.
  • the carrier or vehicle may be a wax, and if a water-soluble type of wax or material of wax consistency be employed, after using the crayon or blocking-marking on the film holder, such as a metal casette, it may be quickly removed by a damp cloth or like suitable means ready for the next use of the film holder. If
  • a non-water-soluble wax is used, the markings may be removed by use of naphtha or other vola tile wax solvent.
  • Desirable water-soluble waxes are for instance the solid waxy polyglycols, polyethylene oxide (commercially known as Carboinstances of such suitable plasticizers being polyglycols, glycol ethers and esters, glycerine ethers and esters, etc.
  • a normally solid water-soluble wax such as afore-noted, is melted, nad the heat is removed and as it begins to cool about 75 per cent of colloidal lead having about '70 per cent or more of its particles in the size range of 1 to 15 microns, is stirred in, together with 5 per cent of a polyglycol plasticizer to produce a rather thick paste.
  • the mixture is then formed into desired pencil or crayon shape, as by a mold or by extruding through a die, and allowed to cool and harden.
  • the final product may be in the form of a stick or rod either not covered or covered with wood, metal, paper'or other casing adapted to facilitate usage.
  • the wax is melted and about per cent colloidal lead or other metal if high atomic weight in finely divided form is incorporated in the wax together with about 15 per cent of a uranium salt such as uranium sulphamate.
  • salts or compounds of the metals of high atomic weight i.e. above 184, such as uranium, bismuth, thorium, lead, thallium, etc.
  • the colloidal metal usually of a lesser atomic weight and substituting a corresponding amount thereof.
  • These combinations including a heavier metal salt together with the finely divided metal having a lesser atomic weight, possess improved blocking power and are particularly useful for work in- VolVing gamma rays and hard X-rays but are also fully effective for the softer less penetrating X-rays.
  • Compositions omitting the heavier metal salt component may be satisfactorily used wherever their blocking power is sufficient, as for the softer, less penetrating X-rays.
  • a liquid base such as a cellulose ether or ester or an alkyd or Bakelite resin clear enamel or varnish dispersed in an organic solvent may have the desired amount of colloidal metal or mixture of colloidal metal and compound of heavy metal in proportions as aiore noted.
  • Such composition mayzbe used .with amarking brush or pen.
  • a marking material for blocking x rays and the-dike comprising colloidal. lead and'a compound of a metal of atomic weight atleast 184-,- and a vehicle;
  • a marking material for blocking X-rays and 1 the like comprising a colloidal. metal. of EtOmlCWElght-Elt least 184 and a normally solid water-soluble material o-f'wax. consistency; 5.
  • a marking material for blocking X-rays and the like comprising colloidal lead, and a normally solid water-soluble material of wax consistency.
  • a marking material for blocking X-rays and the like comprising colloidal lead, and a normally. solid" Wax.
  • a vmarking material for blocking X-rays and the like comprising a vehicle with incorporated'coll-oidal metal of atomic weight at least 184.
  • a marking material for blocking X-rays and. the like comprising a colloidal metal of atomic weight at least 184 in amount of at least 50 per cent,'and a water-soluble polymerized ali-' phatie material of wax consistency.

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  • Physics & Mathematics (AREA)
  • General Physics & Mathematics (AREA)
  • Radiography Using Non-Light Waves (AREA)
  • Inks, Pencil-Leads, Or Crayons (AREA)
  • Medicines Containing Antibodies Or Antigens For Use As Internal Diagnostic Agents (AREA)

Description

Patented Feb. 15, 1949 X-RAY ()PAQUE MARKING MEANS No Drawing. Application July 27, 1944, Serial No. 546,907
12 Claims.
In the use of highly penetrating radiations such as alpha, beta or gamma rays from radium or other radioactive substances, or where photographic plates or films are exposed, such as in metal inspections, medical and surgical practice, etc., it has been customary to mark the plate or film for identification by placing formed letters of sheet lead for the identifying data, such letters being laid on the casette or film holder, and by their shielding or blocking out the radiation, produce the desired identification markings in the developed silver image. Such procedure, while positive in results, is inconvenient and particularly awkward in many instances and not applicable to some purposes. In accordance with the present invention however, markings or blocking-out as desired may be applied on the film holder or casette or on a sheet of material laid thereon and can be easily and quickly removed therefrom after the exposure, the negative carrying the required markings or blocking, while the film holder is ready for re-use. Furthermore special markings not available in stock forms may be employed and areas may be circled or otherwise identified or blocked out, as desired, all with improved speed and facility. Other objects and advantages will appear from the following description.
To the accomplishment of the foregoing and related ends, the invention, then, comprises the features hereinafter fully described, and particularly pointed out in the claims, the following description setting forth in detail certain illustrative embodiments of the invention, these being indicative however, of but a few of the various ways in which the principle of the invention may be employed.
In accordance with the invent on, preferably a pencil or crayon is provided comprising a material in fine particle size having metal atoms of high atomic weight, in a carrier or vehicle substance. By metal of high atomic weight is here meant a metal of atomic weight at least 184. and particularly conveniently available are such metals as lead, bismuth, thallium, etc. Preferably, the metal is in colloidal form, as may be provided by the known methods of preparing metals in colloidal condition. With particular convenience, the carrier or vehicle may be a wax, and if a water-soluble type of wax or material of wax consistency be employed, after using the crayon or blocking-marking on the film holder, such as a metal casette, it may be quickly removed by a damp cloth or like suitable means ready for the next use of the film holder. If
a non-water-soluble wax is used, the markings may be removed by use of naphtha or other vola tile wax solvent. Desirable water-soluble waxes are for instance the solid waxy polyglycols, polyethylene oxide (commercially known as Carboinstances of such suitable plasticizers being polyglycols, glycol ethers and esters, glycerine ethers and esters, etc.
As an example: A normally solid water-soluble wax, such as afore-noted, is melted, nad the heat is removed and as it begins to cool about 75 per cent of colloidal lead having about '70 per cent or more of its particles in the size range of 1 to 15 microns, is stirred in, together with 5 per cent of a polyglycol plasticizer to produce a rather thick paste. The mixture is then formed into desired pencil or crayon shape, as by a mold or by extruding through a die, and allowed to cool and harden. The final product may be in the form of a stick or rod either not covered or covered with wood, metal, paper'or other casing adapted to facilitate usage.
As another example: In similar procedure, the wax is melted and about per cent colloidal lead or other metal if high atomic weight in finely divided form is incorporated in the wax together with about 15 per cent of a uranium salt such as uranium sulphamate.
In similar manner, salts or compounds of the metals of high atomic weight, i.e. above 184, such as uranium, bismuth, thorium, lead, thallium, etc., may be applied along with the colloidal metal usually of a lesser atomic weight and substituting a corresponding amount thereof. These combinations, including a heavier metal salt together with the finely divided metal having a lesser atomic weight, possess improved blocking power and are particularly useful for work in- VolVing gamma rays and hard X-rays but are also fully effective for the softer less penetrating X-rays. Compositions omitting the heavier metal salt component may be satisfactorily used wherever their blocking power is sufficient, as for the softer, less penetrating X-rays.
In some instances instead of a normally solid 3 carrier, a liquid base, such as a cellulose ether or ester or an alkyd or Bakelite resin clear enamel or varnish dispersed in an organic solvent may have the desired amount of colloidal metal or mixture of colloidal metal and compound of heavy metal in proportions as aiore noted. Such composition mayzbe used .with amarking brush or pen.
With compositions as herein provided, identificartion markings such as in light metalalloy inspection work and other metal inspectionx'canw bequickly and conveniently made, and identification or blocking out many extent-desired may be applied, and afterservingjitsipurp'osep may be quickly and easily removed," the finished photographic plate or film carrying. therdesired. Similarly in anatomical" marking or blocking. X-ray work, markings and blockings -may, be made as desired.
Other modes of applying the principle of the inventionmay be employed, change being made asnregards the details described; provided the' an'd the like, comprising colloidal lead and acompoundv of a metal of atomic: Weight at least 184 and a normally soli'dwaxi' 3. A marking material for blocking x rays and the-dike; comprising colloidal. lead and'a compound of a metal of atomic weight atleast 184-,- and a vehicle;
4. A marking material for blocking X-rays and 1 the like, comprising a colloidal. metal. of EtOmlCWElght-Elt least 184 and a normally solid water-soluble material o-f'wax. consistency; 5. A marking" material. for blocking. X rays andthes like; OOmPTlSLiIIgT: a: colloidal. metal of atomic" weight at least .1841-and a normally solid wax;
6:. A marking" material for blocking. X-rays and'.the-..like,z comprising; a: colloidal metal of atomic weight=atleast 184; and avehicle;
'7. A marking material for blocking X-rays and the like, comprising colloidal lead, and a normally solid water-soluble material of wax consistency.
8. A marking material for blocking X-rays and the like, comprising colloidal lead, and a normally. solid" Wax.
9; A marking material for blocking X-rays and the like, comprising colloidal lead, and a vehicle.
10. A vmarking material for blocking X-rays and the like, comprising a vehicle with incorporated'coll-oidal metal of atomic weight at least 184.
11. A marking .mat-erial for blocking X-rays and the-tlike,..comprising colloidal lead at least 50 per cent, polyglycol of wax consistency, and a small. percent of plasticizer.
12. A marking material for blocking X-rays and. the like, comprising a colloidal metal of atomic weight at least 184 in amount of at least 50 per cent,'and a water-soluble polymerized ali-' phatie material of wax consistency.
WILLIAM H. \VOOD.
REFERENCES CITED The following references are of record in the file of this patent:
UNITED STATES PATENTS Number Name Date 471,438 Schwarzwald Mar. 22, 1892 1,278,010 Poetschke Sept. 8, 1918 1,396,415 Fried Nov. 8, 1921 1,511,874 Eder Oct. 14, 1924 1,602,688 Lindsay Oct. 12, 1936 1,918,996 Weger July 18, 1933 2046,55? Holt July 7, 1936 2,162,178 Marasco June 13, 1939 FOREIGN PATENTS Number Country Date 305,209 Great Britain 19 30 OTHER... REFERENCES Synthetic Organic;Chemicals, 10th.'Ed. 1940- published. by' Carbide and Carbon Chemicals Corp., N. Y. C. pp. 66-68. (Copy in-Div. 64.)
US546907A 1944-07-27 1944-07-27 X-ray opaque marking means Expired - Lifetime US2462018A (en)

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Cited By (22)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US2682476A (en) * 1950-05-11 1954-06-29 Staedtler J S Mixture for manufacture of pencil leads
US2702756A (en) * 1950-05-13 1955-02-22 Burgess Battery Co Electrically conductive wax compositions
US2807555A (en) * 1956-03-02 1957-09-24 Du Pont Ceramic color compositions
US2988523A (en) * 1958-05-12 1961-06-13 California Ink Company Inc Radiation shielding composition and method of manufacture
US3454765A (en) * 1965-10-23 1969-07-08 Pitney Bowes Inc Thermographic reproduction process using stencil laminate material with a layer of pressure spreadable and infrared reflective material
US3767441A (en) * 1968-07-01 1973-10-23 Rohr Industries Inc Hold-down composition for machining articles
US3994848A (en) * 1974-12-20 1976-11-30 Scm (Canada) Limited Solid paints
US3994849A (en) * 1974-12-20 1976-11-30 Scm (Canada) Limited Solid paints
US4710946A (en) * 1985-08-06 1987-12-01 Amoco Corporation Method and apparatus for X-ray video fluoroscopic analysis of rock samples
US4813062A (en) * 1986-08-13 1989-03-14 Milliken Research Corporation Radio-opaque marker and method
US5115461A (en) * 1991-03-04 1992-05-19 Kroy, Inc. Method and apparatus for labeling X-ray film
US5469847A (en) * 1992-09-09 1995-11-28 Izi Corporation Radiographic multi-modality skin markers
US5522921A (en) * 1992-10-23 1996-06-04 Custer; Peter Invisible, x-ray opaque fluorescent printing medium for multiplex reading
US5702128A (en) * 1996-07-18 1997-12-30 Beekley Corporation Radiographic marker system and method of making same
US20080009718A1 (en) * 2006-05-11 2008-01-10 Zohman Gary L Implements and methods for applying radiopaque markings
US20090253981A1 (en) * 2008-04-03 2009-10-08 Hamilton Brian H Skin Marking Tool for Radiological Imaging Material
US20100062909A1 (en) * 2008-09-08 2010-03-11 Hamilton Brian H Bicycle Trainer with Variable Magnetic Resistance to Pedaling
US20100062908A1 (en) * 2008-09-08 2010-03-11 Hamilton Brian H Bicycle Trainer with Variable Resistance to Pedaling
US20100200136A1 (en) * 2008-09-08 2010-08-12 Hamilton Brian H Modular Tire with Variable Tread Surfaces
US8439808B2 (en) 2008-09-08 2013-05-14 Brian H Hamilton Bicycle trainer with variable resistance to pedaling
US8979715B2 (en) 2008-09-08 2015-03-17 Brian H. Hamilton Portable and attachable bicycle trainer
US9980784B2 (en) 2016-01-28 2018-05-29 Raytheon Company X-ray ink pen

Citations (9)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US471438A (en) * 1892-03-22 Schwarzwald
US1278010A (en) * 1917-10-08 1918-09-03 Paul Poetschke X-ray-protective cement.
US1396415A (en) * 1920-05-01 1921-11-08 Fried Julius Identification of plates and films
US1511874A (en) * 1922-06-02 1924-10-14 Eder Josef Maria Method of protecting against light of short wave length and composition of matter therefor
US1602688A (en) * 1922-10-06 1926-10-12 Celluloid Co X-ray protective material and process of manufacturing same
GB305209A (en) * 1928-01-03 1929-09-26 Ig Farbenindustrie Ag Packing for rontgen photographic materials
US1918996A (en) * 1929-09-18 1933-07-18 Bakelite Gmbh Process of preparing molding substances and molded articles from synthetic resins and fillers
US2046557A (en) * 1934-04-30 1936-07-07 Thomas T Holt Filler, marking, and coating composition
US2162178A (en) * 1937-01-19 1939-06-13 Du Pont Film Mfg Corp X-ray shielding compound

Patent Citations (9)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US471438A (en) * 1892-03-22 Schwarzwald
US1278010A (en) * 1917-10-08 1918-09-03 Paul Poetschke X-ray-protective cement.
US1396415A (en) * 1920-05-01 1921-11-08 Fried Julius Identification of plates and films
US1511874A (en) * 1922-06-02 1924-10-14 Eder Josef Maria Method of protecting against light of short wave length and composition of matter therefor
US1602688A (en) * 1922-10-06 1926-10-12 Celluloid Co X-ray protective material and process of manufacturing same
GB305209A (en) * 1928-01-03 1929-09-26 Ig Farbenindustrie Ag Packing for rontgen photographic materials
US1918996A (en) * 1929-09-18 1933-07-18 Bakelite Gmbh Process of preparing molding substances and molded articles from synthetic resins and fillers
US2046557A (en) * 1934-04-30 1936-07-07 Thomas T Holt Filler, marking, and coating composition
US2162178A (en) * 1937-01-19 1939-06-13 Du Pont Film Mfg Corp X-ray shielding compound

Cited By (33)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US2682476A (en) * 1950-05-11 1954-06-29 Staedtler J S Mixture for manufacture of pencil leads
US2702756A (en) * 1950-05-13 1955-02-22 Burgess Battery Co Electrically conductive wax compositions
US2807555A (en) * 1956-03-02 1957-09-24 Du Pont Ceramic color compositions
US2988523A (en) * 1958-05-12 1961-06-13 California Ink Company Inc Radiation shielding composition and method of manufacture
US3454765A (en) * 1965-10-23 1969-07-08 Pitney Bowes Inc Thermographic reproduction process using stencil laminate material with a layer of pressure spreadable and infrared reflective material
US3767441A (en) * 1968-07-01 1973-10-23 Rohr Industries Inc Hold-down composition for machining articles
US3994848A (en) * 1974-12-20 1976-11-30 Scm (Canada) Limited Solid paints
US3994849A (en) * 1974-12-20 1976-11-30 Scm (Canada) Limited Solid paints
US4710946A (en) * 1985-08-06 1987-12-01 Amoco Corporation Method and apparatus for X-ray video fluoroscopic analysis of rock samples
US4813062A (en) * 1986-08-13 1989-03-14 Milliken Research Corporation Radio-opaque marker and method
US5115461A (en) * 1991-03-04 1992-05-19 Kroy, Inc. Method and apparatus for labeling X-ray film
US5469847A (en) * 1992-09-09 1995-11-28 Izi Corporation Radiographic multi-modality skin markers
US5522921A (en) * 1992-10-23 1996-06-04 Custer; Peter Invisible, x-ray opaque fluorescent printing medium for multiplex reading
WO1997041179A1 (en) * 1994-10-11 1997-11-06 Peter Custer Invisible, x-ray opaque, fluorescent printing medium for multiplex reading
US5702128A (en) * 1996-07-18 1997-12-30 Beekley Corporation Radiographic marker system and method of making same
US20080009718A1 (en) * 2006-05-11 2008-01-10 Zohman Gary L Implements and methods for applying radiopaque markings
US20090253981A1 (en) * 2008-04-03 2009-10-08 Hamilton Brian H Skin Marking Tool for Radiological Imaging Material
US10004843B2 (en) 2008-04-03 2018-06-26 Brian H. Hamilton Radiopaque marker tool and method for use in a radiological medical imaging process
US8313419B2 (en) 2008-09-08 2012-11-20 Hamilton Brian H Bicycle trainer with variable magnetic resistance to pedaling
US9149702B2 (en) 2008-09-08 2015-10-06 Brian H. Hamilton Bicycle trainer with variable magnetic resistance to pedaling
US20100200136A1 (en) * 2008-09-08 2010-08-12 Hamilton Brian H Modular Tire with Variable Tread Surfaces
US20100298103A1 (en) * 2008-09-08 2010-11-25 Hamilton Brian H Bicycle Trainer with Variable Resistance to Pedaling
US7955228B2 (en) 2008-09-08 2011-06-07 Hamilton Brian H Bicycle trainer with variable magnetic resistance to pedaling
US20110212812A1 (en) * 2008-09-08 2011-09-01 Hamilton Brian H Bicycle Trainer with Variable Magnetic Resistance to Pedaling
US7766798B2 (en) 2008-09-08 2010-08-03 Hamilton Brian H Bicycle trainer with variable resistance to pedaling
US8439808B2 (en) 2008-09-08 2013-05-14 Brian H Hamilton Bicycle trainer with variable resistance to pedaling
US8162806B2 (en) 2008-09-08 2012-04-24 Brian H Hamilton Bicycle trainer with variable resistance to pedaling
US8979715B2 (en) 2008-09-08 2015-03-17 Brian H. Hamilton Portable and attachable bicycle trainer
US20100062909A1 (en) * 2008-09-08 2010-03-11 Hamilton Brian H Bicycle Trainer with Variable Magnetic Resistance to Pedaling
US9517376B2 (en) 2008-09-08 2016-12-13 Brian H. Hamilton Portable and attachable bicycle trainer
US9802099B2 (en) 2008-09-08 2017-10-31 Brian H. Hamilton Bicycle trainer with variable magnetic resistance to pedaling
US20100062908A1 (en) * 2008-09-08 2010-03-11 Hamilton Brian H Bicycle Trainer with Variable Resistance to Pedaling
US9980784B2 (en) 2016-01-28 2018-05-29 Raytheon Company X-ray ink pen

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