RO86086B1 - Process for butadyenestyrene elestomer blockcopolymer synthesis - Google Patents

Process for butadyenestyrene elestomer blockcopolymer synthesis

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Publication number
RO86086B1
RO86086B1 RO109544A RO10954482A RO86086B1 RO 86086 B1 RO86086 B1 RO 86086B1 RO 109544 A RO109544 A RO 109544A RO 10954482 A RO10954482 A RO 10954482A RO 86086 B1 RO86086 B1 RO 86086B1
Authority
RO
Romania
Prior art keywords
synthesis
coupling agent
catalyst
butadyenestyrene
elestomer
Prior art date
Application number
RO109544A
Other languages
Romanian (ro)
Other versions
RO86086A2 (en
Inventor
Elena Ceausescu
Radu Mihai Bordeianu
Paul Nicolae Ghioca
Irina Alexandra Cerchez
Emil Buzdugan
Mariana Cristina Barcov
Petre Ionescu
Cleopatra Schlet
Zoe Andreescu
Constantin Andrei
Gheorghe Horia Micu
Constanta Teodorescu
Gheorghe Aurel Pop
Vasile Murgu
Traian Stan
Andrei Breiner
Gheorghe Halmageanu
Original Assignee
Institutul De Cercetari Chimice
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Institutul De Cercetari Chimice filed Critical Institutul De Cercetari Chimice
Priority to RO109544A priority Critical patent/RO86086B1/en
Publication of RO86086A2 publication Critical patent/RO86086A2/en
Publication of RO86086B1 publication Critical patent/RO86086B1/en

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  • Silicon Polymers (AREA)
  • Other Resins Obtained By Reactions Not Involving Carbon-To-Carbon Unsaturated Bonds (AREA)

Abstract

Procedeul de sinteza a blocopolimerilor elastomeri termoplastici, conform inventiei se caracterizeaza prin aceea ca într-o prima faza se polimerizeaza stirenul în prezenta unui catalizator, organo-litic la temperatura de 30 degree C, din care, în faza a doua se initiaza polimerizarea butadienei la temperatura de 60 degree C cu homopolimerul activ format în prima faza a sintezei, iar în faza a treia, se cupleaza diblocopolimerul activ rezultat din faz a doua a reactiei cu un agent de cuplare di-sau polifunctional ales dintre iod dimetildiclorsilan, acetat de etil, dicetone, Si Cl4, CCl4,diesteri, dianhidride, în proportie sub stoichiometrica fata de catalizator, astfel încat cantitatea molara de agent de cuplare utilizata pt. un mod de catalizator efectivsa fie cuptinsa între 0,95/EF 0,45/EF, preferabil între 0,85/EF 0,50/EF, unde E este eficienta, F este functionalitatea agentului de cuplare.The process for the synthesis of thermoplastic elastomeric block copolymers according to the invention is characterized in that, in a first step, the styrene is polymerized in the presence of an organolithic catalyst at a temperature of 30 ° C, of which, in the second step, polymerization of the butadiene to the temperature of 60 degrees C with the active homopolymer formed in the first phase of the synthesis, and in the third step, the active diblocopolymer resulting from the second phase of the reaction is coupled with a di- or polyfunctional coupling agent selected from dimethyldichlorosilane iodide, ethyl acetate, diketone, SiCl 4, CCl 4, diesters, dianhydrides, in proportions below the stoichiometric to the catalyst, so that the molar amount of coupling agent used for an effective catalyst mode is either comprised between 0.95 / EF 0.45 / EF, preferably between 0.85 / EF 0.50 / EF, where E is efficient, F is the functionality of the coupling agent.

RO109544A 1982-12-30 1982-12-30 Process for butadyenestyrene elestomer blockcopolymer synthesis RO86086B1 (en)

Priority Applications (1)

Application Number Priority Date Filing Date Title
RO109544A RO86086B1 (en) 1982-12-30 1982-12-30 Process for butadyenestyrene elestomer blockcopolymer synthesis

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
RO109544A RO86086B1 (en) 1982-12-30 1982-12-30 Process for butadyenestyrene elestomer blockcopolymer synthesis

Publications (2)

Publication Number Publication Date
RO86086A2 RO86086A2 (en) 1985-02-25
RO86086B1 true RO86086B1 (en) 1985-03-01

Family

ID=20112462

Family Applications (1)

Application Number Title Priority Date Filing Date
RO109544A RO86086B1 (en) 1982-12-30 1982-12-30 Process for butadyenestyrene elestomer blockcopolymer synthesis

Country Status (1)

Country Link
RO (1) RO86086B1 (en)

Also Published As

Publication number Publication date
RO86086A2 (en) 1985-02-25

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