PT105566A - PROCESS FOR THE SELECTIVE ELECTROCHEMICAL CONVERSION OF CARBON DIOXIDE - Google Patents

PROCESS FOR THE SELECTIVE ELECTROCHEMICAL CONVERSION OF CARBON DIOXIDE Download PDF

Info

Publication number
PT105566A
PT105566A PT105566A PT10556611A PT105566A PT 105566 A PT105566 A PT 105566A PT 105566 A PT105566 A PT 105566A PT 10556611 A PT10556611 A PT 10556611A PT 105566 A PT105566 A PT 105566A
Authority
PT
Portugal
Prior art keywords
pare
όττ
formula
compound
tal tal
Prior art date
Application number
PT105566A
Other languages
Portuguese (pt)
Inventor
Tiago Da Costa Duarte Pardal
Marta Catarina Martins Ramos Goncalves
Jose Augusto Damaso Condeco
Joaquim Miguel Badalo Branco
Tomas Rei Fernandes
Anabela Beatriz M Gomes Boavida
Original Assignee
Omnidea Lda
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Omnidea Lda filed Critical Omnidea Lda
Priority to PT105566A priority Critical patent/PT105566A/en
Priority to PCT/PT2012/000008 priority patent/WO2012125053A2/en
Priority to EP12715237.9A priority patent/EP2686464B1/en
Publication of PT105566A publication Critical patent/PT105566A/en

Links

Classifications

    • CCHEMISTRY; METALLURGY
    • C25ELECTROLYTIC OR ELECTROPHORETIC PROCESSES; APPARATUS THEREFOR
    • C25BELECTROLYTIC OR ELECTROPHORETIC PROCESSES FOR THE PRODUCTION OF COMPOUNDS OR NON-METALS; APPARATUS THEREFOR
    • C25B3/00Electrolytic production of organic compounds
    • C25B3/20Processes
    • C25B3/25Reduction
    • CCHEMISTRY; METALLURGY
    • C25ELECTROLYTIC OR ELECTROPHORETIC PROCESSES; APPARATUS THEREFOR
    • C25BELECTROLYTIC OR ELECTROPHORETIC PROCESSES FOR THE PRODUCTION OF COMPOUNDS OR NON-METALS; APPARATUS THEREFOR
    • C25B11/00Electrodes; Manufacture thereof not otherwise provided for
    • C25B11/02Electrodes; Manufacture thereof not otherwise provided for characterised by shape or form
    • C25B11/03Electrodes; Manufacture thereof not otherwise provided for characterised by shape or form perforated or foraminous
    • C25B11/031Porous electrodes
    • CCHEMISTRY; METALLURGY
    • C25ELECTROLYTIC OR ELECTROPHORETIC PROCESSES; APPARATUS THEREFOR
    • C25DPROCESSES FOR THE ELECTROLYTIC OR ELECTROPHORETIC PRODUCTION OF COATINGS; ELECTROFORMING; APPARATUS THEREFOR
    • C25D7/00Electroplating characterised by the article coated
    • C25D7/06Wires; Strips; Foils
    • C25D7/0614Strips or foils

Landscapes

  • Chemical & Material Sciences (AREA)
  • Organic Chemistry (AREA)
  • Engineering & Computer Science (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Electrochemistry (AREA)
  • Materials Engineering (AREA)
  • Metallurgy (AREA)
  • Electrolytic Production Of Non-Metals, Compounds, Apparatuses Therefor (AREA)
  • Electrodes For Compound Or Non-Metal Manufacture (AREA)
  • Organic Low-Molecular-Weight Compounds And Preparation Thereof (AREA)

Abstract

A INVENÇÃO DIZ RESPEITO A UM PROCESSO PARA A REALIZAÇÃO DA CONVERSÃO ELECTROQUÍMICA SELECTIVA DE DIÓXIDO DE CARBONO (CO2) EM HIDROCARBONETOS E MAIS ESPECIFICAMENTE EM HIDROCARBONETOS COM DOIS ÁTOMOS DE CARBONO C2. O PROCESSO É EFECTUADO NUMA CÉLULA ELECTROQUÍMICA EM QUE O CÁTODO É UM ELÉCTRODO MODIFICADO COM UM ELECTRODEPÓSITO DE COBRE DE MODO A MELHORAR A ACTIVIDADE CATALÍTICA E SELECTIVIDADE DO SISTEMA. A FORMACÃO DE UMA MISTURA DE HIDROCARBONETOS RICA EM C2 (C2H1 E C2H6) ISENTA DE METANO É OBTIDA COM SUCESSO COM ELECTRODEPÓSITOS DE ELEVADA ÁREA SUPERFICIAL ESPECÍFICA. ALÉM DISSO, O ETILENO É PRODUZIDO SELECTIVAMENTE EM DETRIMENTO DO ETANO. OS ELECTRODEPÓSITOS DE COBRE OBTIDOS POR ELECTRODEPOSIÇÃO EX-SITU CONDUZEM À ESTABILIDADE DO PROCESSO DE REDUÇÃO DO CO2, I.E., À ESTABILIDADE DA PRODUÇÃO DE HIDROCARBONETOS DEVIDO À FRACA DESACTIVAÇÃO DO CÁTODO.The invention relates to a process for the realization of the selective electrochemical conversion of carbon dioxide (CO2) in hydrocarbons and more specifically in hydrocarbons with two atoms of carbon C 2. The process is carried out in an electrochemical cell in which the cell is a modified electrode with a copper electrodeposite so as to improve the catalytic activity and the selectivity of the system. THE FORMATION OF A RICH HYDROCARBONS MIXTURE IN C2 (C2H1 AND C2H6) METHANE-FREE IS OBTAINED WITH SUCCESS WITH ELECTRODEPOSTS OF HIGH SPECIFIC SURFACE AREA. IN ADDITION, ETHYLENE IS PRODUCED SELECTIVELY IN DEATH OF ETHAN. COPPER ELECTRODEPOSITES OBTAINED BY EX-SITU ELECTRODEPOSYTION LEAD TO THE STABILITY OF THE CO2 REDUCTION PROCESS, I.E., TO THE STABILITY OF HYDROCARBON PRODUCTION DUE TO THE LOW DEACTIVATION OF THE CÁTODO.

Description

|«s m. oloobxoquissieo. s*l*et£va do dódãodo da c&rhoxas 0Sd«fÍS>| «S m. oloobxoquissieo. s * l * ethnicity of the dendron of the lungs.

Ostopso da Xm^oopàs .2 p.r o cas o c o· .Ιοοροροο alia? roopaiaico d fee-a càa ao; ca-1 avo q o 1 rosasa e, asc gar-ai, a uo proaosauso cie ccsasoerBâta; da 002 «a. 2Xdr oca sdãoasss toas aas ascooi oopocXi rcataonio ear hidxooopbonotoá. acaa dois dtoasoa daí coriaoaao €2 '(-etliana aOstopso da Xm ^ oopàs .2 para o o o o o o o o o o o o? roopaiaico d fee-a càa ao; ca. 1 avo q the 1 rose and, as a consequence, a proaosause cie csasoerBâta; of the invention. For all three purposes, the title compound is hydroxylated. two days later, € 2 '(-

Bta&amp;as.aa| - W«am£»ES DA nryraçâ© 2. cootoaoâs; oiocttoqaaiísica do €02 o o Mdaaocarbaiósotoo Casais aaabo ssastiadoda ir:ataáí:ooi:oãoaaaaia&gt;a dai «saia da 25 anos? ;Ha&gt;rl a?; o o a, &lt;,·. à d a $ y; Coo o a 0· s&amp; .1 - ,· i o aa ;a 1 &lt; doo ο o o aa a . {a, d o oi pasitootoq raio. a j rodp ciο ο I o o t r pato loai asa do €02 a po t aaa.ô o otilosao o ropootãoãsx aafioidooloo Carâdrooo do 7 31 o 251.: roaspoao.iva-i:onáo! οορ ptisaseiroo 15 minotoa? , .Oqcaeiao: totasasa av; ai I. c X o o.c i a ;v f as r 24 i ca o assai o a? .1 ooodo. as r ορ o r t a a! a. a a? t ô a o asoiaiOiai:o cora o reooaa-lo do roròscoaa do €02. coroo .autoreo soaX.€ãO:t.oxaaa a a Xispop tineia asas as? diopasoiM 11, ;::ai a' ssobro q ratao io r do ooo ii ocio cor oo ronco o t o Xo &quot; o; ir o -a o : 1 o o qo do ãa o da a osspisriicai e i a? o cátodo par a? obrar o ai o 0:bXaaX2:aasiasai farodloao &gt;aieaí:ada,a&gt; Contnd.co aaPo ooci voa: r assa tosai aiiXoca:araa 4o b rd r o co tb on as t oa .1. atoa ta das &lt;2X4 ·, € cobra- 2; o òolaso soai Cassai aX das saidotrobo Pot&amp;Iido atao c r Ooo Si ta .14r4 c á aafooaa o to ã c ocsas b t oslaa t a? as or ia o c a. c a i, a i Ga t C r a- X a. ast aai.: f 2005., sJXtsartq 20071, Oss aootdc cosas a Xiacraisiro,· as ásaiot.cra do hidrssoaabcssoboc praderida por asloecrcrodasçoas das &lt;232 é asaloaastaCSspidsa assas assattCr casa:'tas adsrs se o a-as pop as ot asas a? c Pti:a,spo, Eo. qptoi, ã saficXôcoXã iaaaodãioa 4o (2X4 0 sslala clOacído do psao as. alo €204.. Kyriaaaoo o oasaaosoàstcprisaXos {Kosaiãccti o 2o op aao a t cocaa X o o 1353:1 aaaapaittaijaaas oc o optai.o too aii;eiaacisa Os; iptstsgso ptdíS e te:ed.:eao ®l-SutroquIníi ca. de 002 .se oefe,ss suas soloadc de Cp S 0 d:a 220:03 d 203 d; 161 pa:s o tsataso s 13% para d et2isso, dsutsa st al, : Orces::. st ae,: lOSO; inscsaigaraa s rsdsjpis de: CQ2 asais selsção aquosa Os 0,s)a 0 23(003 e 2 3 3 0 a abtiacarasí ssátara, atilado e- etsas cae. afiei inalas .tarâdsiaaxi àé 17,2; 12,1 s d,0:30%,Bta &amp; as.aa | - - - - - - - - - - -. oiocttoqaaiÃsica of € 02 o the Mdaaocarbaiósotoo Couples aaabo ssastiadoda go: ataáí: ooi: oãoaaaaia &da; a dai «skirt of 25 years? ; Ha &gt; rl a &; or o to, <, ·. à d a $ y; As with 0 · s & .1 -, • i or aa; a 1 < doo ο oa aa. (a, d, o, pasitootoq radius. The composition of the formula (II) is prepared by the procedure of the formula (II): The compound of formula (II) οορ ptisaseiroo 15 minotoa? , Proc. The compound of formula (I) is prepared as described above. .1 ooodo. the r ô r o r t a! The. aa It is the heart of it, which makes it the heart of the € 02. X-ray diffraction. The composition of the present invention comprises the following steps: (a) the composition of the colorant (s) O; go to the oo: o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o? the cathode pair a? to work out the 0: bXaaX2: aasiasai farodloao &gt; aaa: ada, a &gt; Contnd.co aaPoo oo v alue: a b a ck a ck: a nd 4 o b b a c tb e o t. lt; 2x4, &lt; / RTI &gt;cobra-2; the coupling of the coupling to the coupling is effected by the coupling of the coupling agent to the coupling agent. the ora c a. c a i, a i Ga t C r a - X a. Asterisks of the present invention are shown in Figures 1 and 2 in the following table showing the adsorbed adsorbents of the &lt; 232 &gt; ? c Pti: a, spo, Eo. (2X40%) of chloroacetoacetic acid (20% by weight). The compound was prepared according to the procedure described in Example 1, which was prepared in the same manner as in Example 1. and the ratio of CpS02 to 220: 03d 203d: 161 to 13% for this, after this step. The compositions of the present invention may be prepared by the following methods: (1) to (2) to (2) to (3) to (5) to (5) to (5) to (5) to (8) to (8). tarasia at 17.2, 12.1, sd, 0.30%,

a d s|td c't s.varru(nt o , .0 d 1. s a ri Os 1 ç a a da s p r a da t o a e d Si c 1 es o i a s tarádaioaa sác iu?: tocante 0 apeada o.t d s as est rctosas ds %íd:ddallldid do sléctróde d Cdddidddd: locais, ta 1 soro d pn, rose est rap-Oo de 23(003 s 00% (Odtárrsli dt si,, 2000 }, O forteiptlo Os etliaso è farorceide. est solaçOos ds 21(003 02 2 d: ida e ( slect a d· 12 toa ds s ias adea pd), em ao a o matas; o é prosssàde praiareruaiaisdstte ο;» (sslspsea Os 22(00 3: raiatlssatasyte sescstisredas (alscero li tos 0a: baixo pib , Este sa 2 ect itidada asa p r adiç % è 0s ti s: ad a das; 3} 3 &quot; ala s ta o gs a a d o s sa rededas catódica qae aia esstaaiiselkíS: seu tara:,a sesta; sas soa HdQ:0·' uaasds ests sapécie ed esédaers: alepaolaei, Olsri d ta dl. r, 1000, ; 10i0, 1007} , dst s rsoe s c assas e a, 2- a, 2 a Pa a s 1. st al, (2002 } tlidulddrdds d atsrits Os satratara criatssilps do oalasa sa seiectlvidade ala sisotrorodupãs dd- 002, Os aatstrss t afeeitSP. ede ; as tacas:· criatalisaa; d:oralde.dsa par Ocsisut da o arigad pa: .lacapai.eests s atlisas d se rscse atd.:stalJ.naa doer cacas per Cu (112) fesorac:ae: a aradsção o.e aatans dfassoasài st; ai &gt;, 20021,. élé:a 02 asa, tdseOsxrsiS gas- st aasaesPo da OsasiOsOs atOaisa do piaso cridadvisgráfies (1:10} adtisa a i'sr:daa2a; Os saltaaaa.eias cot! maia Os doi.a àtetsca d:a ca s'0as:st (02 (3 d aaeriSíS a fcrsíapOa dc; (2(3 , O a meã a n 2 saoe tdaccldnaia pcldci:;iarsa 0 a reduçdo dd 002 a hi d toca rc o set cr aogatlOcs por satieia aíttcree ase edtitrddsrdoa &lt; Ocr i d cdlaOoasvddtse (Hord: dt ai,, .1007} e f s dista raP (Md real ai o a o a}:eda((lamd prcgjdtlvd da 1080 e ptap(.s(erat( aos; a a sisa reaaci oásis caadttcsstos só eetscs a a a i I eco pedes di f s r 2r sa: p r i es2 r a. t r as.a t erasc 1 .a. a.1 ed t r ca i ca pa:rs d CO- Para ter iafcrísapt* acere as t?s,:ts rcasoionaia da C02 a saieatde:id:sdaa doa produtoo.j· doai. st; si, (Hosai sta ai,* Idlin isaaçesat igarapé a íSsXsasssata sooecOoôc sao CSSa esss, &gt;sd. siast. realce; da ao:h.raa, rs 1 qs.se 1 e iessaa, Oa ssstaarea sasassetasasiao; aua aasss eieaaessosao asa isobre assas; a Ssspeasiiíssla asap as saa origina, asas paspaa.ro ossaetidada a a et.aassa tiad , dal cossao ao. sléctssodo sle nia|;,sassl a i:a s: a: o .· voaissalOí o «taíio islo foi das sa sa t. a si o aaas a IdasrabaS: da Cs.s islBsase e isso is.r aspas lisalass; assa Sasaaosaalosa asaaas a:ss;a aolsipslo da- ad:l d. ii ass lds.· Be toe aasítoasasa sacsaasirassíS afae a sdaoraia- de s&amp;pèas.ea de hidrasgéoias á: esasoieei si estrastssras &lt; Paa;sspa.asa;:'am tasasOatos, ag.sas a a aapaloies sala hasadogasaio aoBspoetea pa a da ia átsossco ala Oidroedaio pneapotosspeae eaasoaied.dss as ar a des da- de C d a em ei ée t ar a disse d a; a ea se de as sao e t f 1 c 1 a X i s a # assiS|s,ssa.to o Msasarasgdaasla; ssasaisdoas asalassriiaias poda ests,r aassolesido rasa easpasrficiea arsagasaax do aiasedscossioa da cassoe; asSss ass i aas a assasas ;asae da· a 1 si e t r odea do d :1 aps a l i a as da as aa;· sso ss d arasgoai atada da ; a aspe ri leia liora.aca dafeitae de eaparfixsie tassUs aeesò d ass.raass e Xeaoaae fsesorâveie si araaeçda de átoasoa de is xôrogén í e t sasaiss; esr a t doa i E a ta s tilda et t dado a: e ss: c a sdd Iro 1 rases sgaas· as i e aessas sso a; ais e t .Usasses si asa Sara ras iasasasds a sssssda easaeta josssas sao afa.se &gt;ss do aeasaass daosldisa ao soossosssisasesaiio iisas.1 tosão ase is 1 d.r o gé a;d. e as d;a; o r v lassas, Ã í oaeasrar e câsaassosssíaaaisíssssãe asai esss íarsaiase passo da íaslaetrasassepiseitasaa: ala aiasisara ias a asas aas taissie da e ao a Mikolic ast ai, s d. ass&gt;l1 c aata asa.,* 1,001; , :ílaísasaasaadaoasa'iís,a, ea- e:ss:r,sraais.s rasas :.: ss.as-sia vas C.sai SPPP, ,raS’sssasa’:ssíSSS; as·;:: a às;.:. a.ss:a.·ss·as:S. ss;ss:ssssss.ss asss; sas e«árasadas:ietioae prlsscipaisa dee aastasssasarasa ass; fasea aàe asei assas as esaieoeoaais de assasà.a aasaaspoa asse Sásssasstasrasa ea; peassas assas soaigasas. asi à iisosooi, ids sssssas.spe das ísscatesaaso; aas psarasa si iosasssissdo asses tala á iaisssaSsSiass alas: dasii lséa alas Psiaiss apásssiasí ssaao altsssiea ais eeiat|sas:c.is ase; s.s.;s;as ,isssss.iss.ssass r«saaass(.:esss de lssPsss.rtsa.pso de hidacoéeio aa.;.;: ssspsa s depeelç!ex tara raaapoa iosapae ale alapas a i a e as pa dep, i e a ses r - a e assaa t e e a e i aa el, e a a e das e r e Is ass as: a a assa peasses, o is aasaéss ala csosaseiesasaiao da a csasslsaasee das a aiassse pss.i.sBaa.i ;:oa passpee., d l.io li ai ass asa.., (Psi assas i isi sSa sl,, iOalel aslsa refere &amp; qpXsId-açlo doolssao ti |?&gt;ag dsss o.Iqctcrobopboi.t-OB· π O e 1 as- a? t; ra? r easdica o ;dp CPd :¾¾¾ forsssoco; ssioPo-o quo porroltosio p;rovò| o íSiassssiiasrtnoiO assiso: doaste tipo da? olddt::£Obep-6di.P-o.a ta rsssPsdtlasdi roossagdsv. cdsssss das; a|s.soaslidaa asa is insportasaítsssa: do pinto do vias t a do ssísíss pttsgoiiíB oiootrolitioo coiscss lasca-o é: a iotâíbiiidodo o is ds.i.sseit assa psssisdaçsPi te gasaasti Isatellcsiosenssass tocloo os odissaiàdssoioso i&amp;réd.toçsa r o .12; r i das o: asso isitósoaturo aiiooisssdOia rsspsiasrdasissioento -ipéo: Par too po; ri. o doo do soou.: coo ois;-a:l ;: a;sao.s.ns.i.srss, o ss; eiéetrodo tio sssoPto poraisss a osso &lt;s;Iovodo Oírtd,vJ:do.bg iaotoJ.itl&lt;sa aos rol aipis ο o &lt;s:&gt;síiSss?'or;s;idsí do 5102 OCaols or o x, - slBaidl; gv5vr«so;5?s:s sa: :%rsOít|ío.oi&gt; o CipíOtã-·. os&gt; .ciar ; *(1) (1) (1) (1) (1) (1) (1) (1) (1) (a) (d) Sodium dodecylsiloxazole (dibromoethane), dibromoethane (dibromoethane), sodium hydroxide, sodium bicarbonate, sodium bicarbonate, (s) and (s) to (d) to (d) to (d) to (d) to (d) in the forest is prossiàde praiareruaiaisdstte ο (sslspsea The 22 (3: 2, 3, 4, 5, 6, 7, 8, 8, 9, 10, 12, 13, 13, 13, 13, 13, 13, (2002), which is to be found in the present study, and the results obtained in the present study are shown in Table 1. The satellites OAOs are of the same quality as those of the SISOTRODUCTOPS-002. P. ede; the tacas: · criatalisaa; d: oralde.dsa pair of the arigad pa: .lacapai.eests s atlisas d se rscse atd.:stalJ.naa doer cacas per Cu (112) fesorac: ae: the collection o.e aatans dfassoasài st; ai &gt;, 20021 ,. (2: 1), as well as in the case of the population of the high population density (1:10), followed by the following: ts (02 (3 d aaeriSíS the fcrsíapOa dc; (2- (3, the MEA n 2 saoe tdaccldnaia pcldci:; iarsa 0 to reduçdo dd 002 hi d touches rc the set cr aogatlOcs by satieia aíttcree ase edtitrddsrdoa &lt; OCR id cdlaOoasvddtse (Hord dt al ,,} .1007 EFS is distant rAP (real Md al oaoa}: eda ((prcgjdtlvd the lamd 1080 and PTAP (.s (erat (to; aa SISA reaaci caadttcsstos oasis only ask eetscs aaai I echo di fsr 2r sa: pri es2 r a. tr as.at erasc 1 .aa1 ed tr ca i ca pa: rs d CO- In order to have access to the following, the case of CO 2 is absent: id: sdaa The present invention relates to a method for the preparation of a compound of formula (I) in which the compound of formula (I) is selected from the group of compounds of the general formula (I). , Oa ssstaarea sasassetasasiao; his aasss eieaaessosao asa aso asas baas; s saa origina, paspaa.ro wings ossaetidada a et.aassa tiad, dal cossao ao. The first step was to take the necessary steps to ensure that the necessary measures were taken. to each other at the end of the year, and this is the final quotation; Assa Sasaaosaalosa asaaas a: ss; aolsipslo da- ad: l d. • Beacons of the earthquake occur in the area of water and sanitation. Paa; sspaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaa and if and only if they are the same as the previous one. sasses of the asalassriiae prostrate, the aesthetised rasa easpasrficiea arsagasaax of aiasedscossioa cassoe; as well as the first and second quarters of the year following the year 2000; as well as for the removal of plaque and plaque from the bone and bone marrow and from the bone marrow. The following is a list of the three types of services provided: a) ai and t. If you wish to do so, you will be able to do so at the time of your application. and the d; a; and in the same way as this, at the same time, it would be possible to use the wings in such a way as to make the wings of the Mikolic ast. ass> 11a astat., * 1,001; The following are examples of the most common forms of SADS. as in a.ss: a · ss · as: S. ss; ss: ssssss.ss asss; sas and «arasadas: ietioae prlssentiala dee aastasssasarasa ass; (a) to carry out the tasks of the Member States; some soaigaas assas. thus to the iisosooi, ids sssssas.spe of the íscatesaaso; to the parasites if they were to be killed in the next years. (s), and (b) the water and wastewater treatment plants are to be exported to the districts, - is hereby approved on behalf of the European Parliament and of the Council, acting in accordance with the regulatory procedure with scrutiny referred to in Article 16 The compounds of the present invention may also be used in the preparation of the compounds of the general formula (1) in which the compounds of formula (I) are in the form of a pharmaceutically acceptable carrier. The Committee endorsed the assent of the European Parliament and of the Council of the European Union to the European Parliament and to the Council of the European Union for the sixth session of the European Parliament and of the Council of the European Union. In the case of the foot of the head of the head and neck of the head, the head and neck of the head is the head of the head and head of the head. rssps iasrdasissioio -ipéo: Par too po; ri. the donation of the donation is as follows: a. and the bone is removed from the bone and the bone is removed from the bone and the bone is removed from the bone. ; gt; 5: 5: ss: &lt; / RTI &gt; the. the &gt;.ciar; *

BiMáRio &amp;&amp; xm?ii:MÇÃD O procasadis doado, iaroiçâo; alio roaporto ò do«v oradas 0 i: ao? t r sida: i.ss i: co -.da' 5:tsS dx i a 5 i aSs o c o: rPas ssssSal 00? o d i. i ç o o asqs.s da; a$5 pSr &amp; da.o: sarlgOiO a iai:d.roos?rbon:gt:;??o g,. osasis 000000:^100^00.00,- o. dislrosiarPoiiitog ocos ;?;oi.o átoaoo do corPooo Cd (Otiloato o a; is? o o? 0 00. o í ssrarsssiO-s.· adi .00-?. or?o, ir iPtOisçidi tio os i odor o o as-issa aos tosssr nsn i.s 0.:.0-0.000 assss d.idrs:j&lt;s::5srP:ii0os:t\i:s; C2 ?: ο ρ o a· s o ít. s: *. sonsas iositassiaos. SSS50 00-10.0001 lo soisoOsiroo assaraPosrraàaa cio aso os do dos 't.éao.ioâp saosas ao o qro ;ssp5'5iooa.to.ssi: doidóialolMa asorssrssaãa i.ooa oaspotòosaao la íssiastoroa? sc-onotoudas ;ag;$sasisass paro igual toor oos hip.r&lt;&gt;pédio o i5rò.ast;.s:oiosás?sta 00, cassas o a osssoddtro passsasssrsrsss,. a atas -.cS:.na.ss:.oons ; torasas-r-ss; ss? 0.5..:, ssdisssooaissa asai a' adao:ssipi.;sa poro 00r aosi a: 1.11 i. a adoss o otíao o çasipu a t 1 :sass i 0, ò ρ r o as o as a o sã ai o c t ucsda asooio réisclo oioct rdspsios,!00. ost qpso a? copado a s,sçss oislrstrodo assodi :5? içadas ocas: ;i.l&gt;sí;otrodo:paãaai tasss asso caasaas? qae a ar e π 5s a as a a.o t la id.odo o: a a i ncs? i v?.d.r:.;o do p:aooo a;ssai asaoss s.sa$a acs5i.a‘or:oõa: Jc 002 as a: alva; a , d s::aa?;0'oraaas ala 510 i 0: olãsicauaala essas pacas: oBiMáRio &amp; xm? ii: MCD The procasadis donated, Iaroiço; In addition, The results are shown in Table 1 and Table 1 shows the results obtained from the results obtained. or d i. as the case may be; at $ 5 pSr &amp; From the beginning of the article, osasis 000000: ^ 100 ^ 00.00, - o. The composition of the present invention relates to a process for the preparation of the compounds of formula (I) in which the compounds of formula (I) are in the form of an aliphatic alcohol. to the tosses nsn is 0.:0-0.000 assss d.idrs: j <s: 5srP: ii0os: t \ i: s; C2?: ο ρ the so sits: * ssssssssss. -10.0001 it soisoOsiroo assaraPosrraàaa heat aso those of the 't.éao.ioâp saosas to the qro; ssp5'5iooa.to.ssi: doidóialolMa asorssrssaãa i.ooa oaspotòosaao it íssiastoroa sc-onotoudas; g; $ sasisass stop equal toor oos and the last one is the same as the last one, and the last one is the same as the previous one. .:, ssdisssooaissa Asai the "Adam,. ssipi; sa portion 00R AOSI to: 1:11 i to ADOSS the otíao the çasipu to 1: Sass i 0, ρ ro the AS to the sound al oct ucsda asooio réisclo oioct rdspsios,. And the other is the same as that of the air and π 5s at the same time as the id:The invention relates to a method for the preparation of a compound of the formula (I): wherein: (a) a, d s :: aa?; ooaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaah

assdco,- do fasass.11. aaassaasto dsss soa; cada o podo opoasoass I taasp-o rastear o osstii &lt;s-n?:.s:· o à pagarão Oitrssssoidãasioas.. õ riã;asr:aa- do 1 si íssassSi a; aia sia srppρ o a.a 0 pa i o c sa l o a; d o d ir; r 0 as: o r bop 0 p ps g sss r ors a as ρο-ίο aor -a ors t ra; 1 oaao poio sssiioaotó: ada assapsirlácio .00 a a as o aki assaiP.ro d.l a; psaaa .1 ο ο.I pirss; as aa .1. ar o tr'rr&gt;.r sa-asPo.ap P ao aio CC2 v Oa; pisLconasPoriatas proéaridoa podes; aor po:atardnaxaante: at íiJdddoa ando tdea:iias-x-pt 1¾¾¾. iodsadxioia .assdco, - fasass. aaassaasto dsss soa; each one of them may be used for the purpose of tracking the ossification of the ossicles. Aaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaa d or d ir; r 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 1 o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o oo psaaa .1 ο ο.I pirss; . The reaction mixture is cooled to -20 ° C to -20 ° C. pisLconasPoriatas proéaridoa podes; aor po: atardnaxaante: at iiJdddoa ando tdea: iias-x-pt 1¾¾¾. iodsadoxioia.

Oaacràpda dM FipnsaeOaacràpda dM Fipnsae

Fi qor-s 1 -- PaprasaotS o idSped Odtida and :aic;toacépio einatiéoicd da; var rtranseo da conéigardpio dandritica és sépn &gt;: XI.cie do eia o trode aé t iéo p&amp;r a 1aot rodepas.1 oao aa-&quot;·a i tu da d odre soera una saén da catere rafarido eu Esetípio I,:Fi qor-s 1 - PaprasaotS the idSped Odessa and: aic; The second part of the concomitance of the dandritic concomitant is in the form of the first step of the first step to the first step of the first step of the first step.

Fiaaxa 2 --- Eep se santa. a iasaaas· SOM da coniiiguxaçãd ao. fano a éa nai da ; sapo tirai a do s lá cisada ate ti da por a.1 rns t r-oéa p ;dti çde a a - ο r t a da a ate se a aiatá xasa sede da po&gt;ter s sai a.rido ae: E.aoaplo II en p:ao s: sxéasno ; X· ioilioa duas cr a. te r a s é i st r é ta e, sidoxa: 3 &quot;- Eepseeeota a idaeea Séé ria aettatxxna 30 da oPPta: e.si.reaaxrex:d.s paradas tipo aapeaja,· da ηχφοη tinia: da niéatrado oPtido por olíSotrosiapoáipãa ea-arito da onfere a ate ta osta to 1 ha da catere raoasido na Eaaap jas IV, aa que o sidras r o {21 iadi oa Co i s ao tas od sa.sddao dr.sr.ixtoas &gt; sigoxa 4 - Ãpsaaaata aas sernose;tfaaao ηορροηοχ iea ria célula eleat roqa 1 ar o a atai Irada ca a asaixaxlo-a I a IV, as-; pua· da asap.é/o,taa a-dra ros iixdscóxs: {és oesaósttiaaapta astèéioa;. (.4) oadpartiaarto adoclicn, {si assspartddioata para aadferaaa {aperoaoll, {d { entesada : da n-ls, 1 7{ oatxada da eléotxodo do: rof ar a λ:;- {.s, ; g I salda da aio td{ aaSsrada da aaasor da p.Ha figara S ; apresenta rara r a pr as a a t a a is p; r a ir ca da otiaiãaaia da. ao r rs n a { t { ara san çls; aa potencial do câtocla {e na éa/Paél; ;odt ida na aneapio X τ x: ,Fiaaxa 2 --- Eep if santa. the iasaaas · SOM of coniiguxation to. fano a da na; the frog is removed from the soil by the plant until the plant is harvested in the same place as E. in p: ao s: sxéasno; Xylation of two cr. ras te st i is r is ta, and sidoxa: 3 &quot; - Eepseeeota the idaeea would see the OPPTA aettatxxna 30: e.si.reaaxrex: ds aapeaja type stops, · the ηχφοη jingled: oPtido by the niéatrado and olíSotrosiapoáipãa-Arito from about 1 to about 1 ha of the esterase in Step IV, to which the cider is added to the esters of the esters. 4 - In the case of the cellular cell, the cell will be added to the cell to cell line 1 to IV, pua · of the asap.é / o, soa ds ds ds ds ds ds ds ds ds::::::::::::. (.4) the adipocyte adenylate, for the assay of the nucleotide sequence of the nucleotide sequence of the nucleotide sequence of the nucleotide sequence of the nucleotide sequence. the value of the value of the value of the value of the value of the value of the value of the value of the value of the value. is rare in the world. to go to the dairy industry. to r rs n a {t {ara san çls; the potential of the chase {e na éa / Paél; ; odt ida in the anaphase X τ x:

Daeoalgãa PdCdléaéa. da laaasrpàa 0 proceaoo doota leoensplo para: a couverale da COd «as blbaocarbcçatoa e maio eepeeif lcamo:ot;e ear rddroc.:odsonrooos eoo doie à tomos· d.o carbono Ca Ó afacauado rapta cdlelt elébtfòqúi&amp;ieòp A célooor oon.&gt;p.ato: praiaraíu-b^írl.aabda ouoa nel ai a d.a doia; corlpaxialânblcoa· oai cqia o cátodo 0 d ânodo aâo a opa;: abo a praãaaia:aoi.alao:n,aa par rasa iaeebrana. da portarta opa aca .* 0 ânodoi pode sá o decai qtcâr csoct orlai condator diadtricao-ontp: obaqaado pa.ro. n;oa operaçao af 1. ca?: da uoa. coiola 0:100x001100.00; por eaaopiOí plo:riooo qr.apioe o cardoao ed.rroco 0 material do cátodo poda eer qua 1 qoor p.a t o- r 1 a 1 coo do t or a 1 eco r i. ao: t o..1 coroa oob r oca rbooc v ϊr ra:;: . p. forma do oecdctirato do cátodo pode eer qualquer oonfrgo raçlo adecroada eporpr iodo para o lac ta odopocs iodo d p c Ibiiede podo; o do 1 da,................................................................................................................................... d superfície da cátodo é modificada por a 1 oct ro depo a i çâo iç™ a 1t u o o o a- :a i t n ao coe r e &lt; ma a p r o lo a p c ai:â: imoo e o po r e o·-' s 10 o pax a: f o r n a car taca c onrarcdi o oatáxel do COi apomae am bldrotartrooetoe d*. Foram, obtidoe o ido iro doa madi 1 Pctuioa com obaocrodopdadioo do oob ré coce a la a o tope f 1 loto alo o ot r eísamo o t a: d l doa d a s a ama tf da rd o i o t ôo cia moe i o J. co, 11 r d: voo de o 1 cot r odepo o i·qd o e;&lt; ~ o 1t o da cobro nlòlioaudo p r a .r o· r o η c i o c m o; &gt; c o cPrSOd domo fornooodor do cabida a de crebro a Bolem paro. aoçentax a: ooidor do pe.ndO: do depoo 1çio &lt;Daeoalgãa PdCdléaéa. The process of this process is as follows: the carbon dioxide and carbon dioxide emissions and the carbon dioxide production and the carbon dioxide emission of carbon dioxide and carbon dioxide. ................ The cathode is the cathode of the anode to the opaque layer of the solar panel. of the opaque part. The anode can only be decayed by the con- tact of the diadric-ontp: obaqaado pa.ro. The operation of the unit is carried out. coil 0: 100x001100.00; by eaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaaa crown: the crown of the crown; P. The cathode oxychloride form may be any suitable crosslinking agent for the lactate oxychloride powder; the 1 st day, ............................................. .................................................. .................................... the cathode surface is modified by 1 october depo ation (1) a) • The 10-speed manual is now on the rear panel and the rear panel is on the right side of the rear panel. The pyrrole-dicarboxylic acid was obtained in the same manner as the title compound as the title compound as the title compound as a colorless oil. of the 1 cot r odepo oi · qd oe; in the first quarter of the year. &gt; and the cPrSOd domo fornooodor from the brain to bolem stop. Amino Amino Amino Acid:

Po fiqordo 1; 2 o 1 ireatxam trinr cátodos oodi.fcondoo d la tintoa p rapo r o doo por oílcsodrorkrposipeo ox-xrboa de cobre. 0 catdlito pode eer qual coar aoi(talo aqooea de aai InOrqÉni.co ao ouo o (Pd: é aclderel,· 00.1. toais KiCOl , HaHCò-3 e Kld.,. profereneicimente EHC03,· em coneont raedo-o do coroa de p ; dO d 0 } O dp a pO p O 01 0 0 O;' 1CO. 0: ..i-SíO-í&quot; CU· O (.09 OOrCO Oí;í 0 O 1 o ddilito podo se.:: preleronoiolroíote o meomo que o cotdiitO;Po fiqordo 1; 2 to 1 will have trinr cathodes oodi.fcondoo d tintoa p rapo r o doo by oílcsodrorkrposipeo ox-xrboa copper. The catldate may be from which of the cells of the invention may be present in the presence of a nucleotide of the formula (I) or (I) of formula (I). The compounds of the invention may be prepared by reacting the compound of formula (I) with a compound of formula (I): ## STR1 ## in which: prealloyolytic or methylethyl alcohol;

Coa oaasPrana a.akaap.aa:ia eode eao: gaed agáaer èoséxríana gaia; aOáiáp pacaar p Xac did.aogéoi,o, tal oaaoo datiaio 117;. ou Haadleo 4 77, d r-ad\;çao ; eX,eat.eoaaxxOXaa da? *707 a h,ÍdrOaxe.aX7one:aoas Cd e coeoagoòds utilioaeCO aita adXXaala adaaadaaaKpaaaXoaa que papacal ao cátodo cos eXapèraídagaPaX to;;; de caiaraí ieerao ree ò:lee:trd:X.ito ee qaa o CCd a aoXeeeX, X5ede ser ati.l i aada qaáaXqoex oooeXpurapso ade-gaada d*; aare. cáIala diddtrdqaaid;id:a.. de flato da correote catre o oátodo a .o ioaaxc é .Xo .a coca do a? traeia da aoc Copta aat orna. de epprgia, O procesao de redução oleei ro0á:dtc.co poda aei etectaaakí d® acode oaaad i a no; o ai ea .at; a t â o iaao d a de i dta: xoxa t à t i a o ) ou atra via de nae eode eiean/oaXitioa; palaadaj,Coa oasPrana a.akaap.aa: ia eode eao: gaed agáaer èoséxríana gaia; The method of claim 1, wherein the compound of formula (I) is as hereinbefore defined. or Haadleo 4 77, d r-ad; tion; eX, eat.eoaaxxOXaa da? * 707 a hr, Oxydaxa. AX7one: at Cd and coeoagoos use and atorvastatin at the same time as papain at the cathode. The following is a list of the various types of information that can be used to determine whether the information is correct or not. aare. the cocaine of the aorta is the same as the one of cocaine. brings from the Coptic aat orna. The reduction process may be carried out by the process of the present invention; ai and a .at; The invention relates to a process for the preparation of a compound of the formula (I): palaadaj,

Ca ca tedox? oca; i i x coaxo a. aeraaaaaaataaXaa na Cia, 1; d a 3 çoa· d t XX: azados ; n d céi q: i a: &lt;a X e et i;a qu X rd: s a: pa r a a ceara a d a á:e: Cp CCd, d iteaseeòa da οΧοοόΧοΟΟρορΧΟο a a apperf icie do eiáaet daidaa raaxi s. f :. ca? f a; pXecaaato á; eoepo í'dedada Cai cartaX x ΐ: ieo 'dbg a? Xici rodara para a óoe al d® do db Cd 3a? X t .d rando coo ase qnenreeo?a a a a amapoe x cada da®. X:d.aXroosrPaiit:oa gaíaoecôa, praádaxtoo da? repcçlo, .3 oex r a au.aa aereas eterada, oa Fia, 1 ê caaxaaèiniXda par dapoeltoa da noanaa Penar it.àea&gt;a, Foi uPrltidadd aq.ua acate tipo íie aiactxodepéeit.oa proísoee a produção de et ilacao eo doer ice o. to de e.eaaca;, .3Xám dlaeco aaariiXooaa-ee qne ga:oodo maior for a ooPoetera. de otèefrodo oeo eXect redeeóeito® dindrifieoa miar d a acidei XçXdade para se atileaor 0 cátodo aaodif içado coe. aoa e ai. ratara de cobre: do 'tipo itero ale eo X âprooeatadá ;aa Fi.oe 2 pradao® a ptcejppâa aio ísperaa a· ?aad?:ec:a?roaa·; a;:aa? &lt;?a?; Ca {atilaíao a? a;ta:.ao5 aio aa dáaeaotacdo .petqpOv CaX?ía facto é i.apçedo:r o rstóplfa da etiX.i z&gt;ap.ãQ ;ò?a ç.ma eleóa.da. .área çpperf XcXaX ;.;&lt;&gt;a: i a??.a: .:xoa;í?ç?a,axa:a;a. e á a a; a mcaefòXoi^is./Xe.aÍea.tJiraá.v .3 oxkae aítaaaa do tipo favo aka dal doa aXaKdaaaaxa^daitaae pa,ss?.i.5. raia ρχθδ·!-·ί·0idade maia ?a.Xaoa;aC:a oax grio;?; da caCeO: pòr easl.aaae·, Báta CX' X OXX X' ÍS Ç :S O XiXXSSO &gt;X X. &lt;:&gt; a loac t xô c a 1a1. x ô X :Cô 3 ap t; X v&lt;&gt;s ,. aôxaooida 3 a dca::oa.çõoa do X&gt; IX :' l)XXCSXO X: -.XÇ XpX :.Ο O O 00 xpxo roXo.5 xxaxx m:Mè. prpXipxd, X IdadXíCa c tedox? the CA; i i x coax a. aeraaaaaaataaXaa na Cia, 1; d a 3 t · d t XX: hoes; n d c e: q a i i i i i i i i i i i i i i i i i i i i i i i i i i i i i i i i ii f:. here? f a; pXecaate; and the subject of the letter X x ΐ: ieo 'dbg a? Xici will run for the db o d® Cd 3a? X t .during each day. X: d.aXroosrPaiit: o gaiaoecôa, praádaxtoo da? repcçlo, .3 oex ra au.aa flights eterada, o AIF 1 is caaxaaèiniXda pair of dapoeltoa noanaa slaving it.àea &gt; A was uPrltidadd aq.ua abide type IIe production aiactxodepéeit.oa proísoee et phosphorylation and the ice hurt . to the extent that it is greater than ooPoetera. and the epoxy resin is reduced in the presence of the acidity to form the cathode. aaa et al. copper ratio: from the alloy type and the X to the product and the product to be used in the production process. aa &lt; a &gt; Ca atilaíao a? The composition of the composition of the composition is determined by the method of the present invention. the area of the X-axis, where X, X, X, X, X, and a a a; The composition of the present invention comprises a compound of the general formulas (a) and (b) of the compound of the general formulas (a) and (b). ray ρχθδ · - · ί · Mayan reality χ Xaoa; aC: oax grio;?; of the cachet: for example, Xaa Xa Xa, Xaa Xa, Xaa, at 1 to 1. x δ X: Cô 3 to t; X v &lt; &gt; s. 3 &quot; X &quot; IX: 1) XXCXXXXXXXXXXXXXXXXXXXXXXXXXX: X-ray, X-ray

Ο ;Χ3:Ρ000.Χ:Ρ0 XXÔX C-;3 d:0 COdO ΧΟΧ; XHXXXS X χηχα-χχ:, O cá t calo xaxxXiXxicaxxxx ilxxsxrxXío a a Flor 3 b χ:χ:&gt;.χ xxsxbrrxtXíra atro ta 3 D da ροοχο p\3x 0 aatraáíaríxaxxtax poropa EáXxx cxxcXXlq-.;xacác porxaiaxo c trorapixxtax Xépxxòx d.a aaa o llapxixlco· o a ; opa eiodada área at;pe:o2X,ciai a: :aotraxaxxa POaáoxxxa boro : o:upor X rxtx a da:aaòáap.;. p;xra co χοΡΧΟρΟΟΡ s;33xPtX'PpPXíXÍPa:P, â: XíX.ix.xa:ap:Ío daaXxo aááaidxí para a xxoxx/xx· x oáo de COX: r oaxti ta ar axdxxx:aarlxoasPx:oxx €2 .ale- axxxxlc de Per Pado-X3a 4, Exax a reaxpi1 aa-x co.ai .loraa οχιο a: α X a pori b 11X, baba da exxparxivio astXxoa do cobro e a diotrlPuioio oepacl a i doa xxíxx.x?x xxiΧ5ΧΧΧ-Χ'\xca.xxxxxxxxíxoxí saio a coaxar ρχχχχχ xx xaxooraxxeax oxx (3X 2 erx Xo, P.r o a oa Pbxxo bo s (12 „ ad, èP 01 a o p o:o x X. 2 2.: c o «&quot; ae o o:«x ;x aΟ; Χ3: Ρ000.Χ: Ρ0 XXÔX C-; 3 d: 0 COOD ΧΟΧ; XHXXXS X χηχα-χχ:, The chastex xxxXiXxxxxxxxxxxXxxXxxXxxXxxXxxXxxXxxxxXxxXxxXxxxxXxxXxxXxxXxxXxxXxXxxXxxXxxXxxXxxXxxXxxXxxXxxXxxxXxxXxxXxXxxXxxXxxXxxxxxXxxxxXxxXxxXxxxxxxxqxxxxxqxxxqxxxqxxxqxxxqxxxxqxXxxxqxxxxqxXxXxqxXxXxxXxXxXxxXxXxXxxXxxXxxXxxxxxxxqxxxXxxxxxxqxxxqxXxxXxXxxxxxxqxXxXxXxxxxxxxqxxxxXxXxXxXxXxXxxxxxxxxqxXxxXxXxxxxxxxxXxxXxXxXxxxxxxxXxxxxxxxxxXx o llapxixlco · oa; the area of the area at the end of the line is the following: p; s xra co χοΡΧΟρΟΟΡ; 33xPtX'PpPXíXÍPa: P A: XíX.ix.xa: after Io daaXxo aááaidxí to xxoxx / xx · x COX OAO: rt r oaxti air axdxxx: aarlxoasPx: 2 € oxx .Ale - Per axxxxlc Pado 4-X3a, the Exax reaxpi1 aa-x co.ai .loraa οχιο to: α x b Pori 11X, slaver of the astXxoa exxparxivio stop and gives oepacl diotrlPuioio al xxíxx.x xxiΧ5ΧΧΧ x-Χ? (x, y, x, y, x, x, y), x, x, y, x, y, x, y, shah

OxaxPxXxxdopáaxXXxXs x3x cbXbax obtidos por alxxxaxxxXdeppeXção eat'· tira otaxdaoaai a a ax adi Iodado do ρχροοοοο d&lt;a rodopio do. (332, X x. o x x 2 o at- ab1 X a da do da ρχοχΟχιρίχ o xXo X; X d :roca· r boxta t o a d o o· ido d :lraco doaaprXoaçõo do aòaxodxo X :o ta. 1. pxxxaoxxxxx X::aooxicxxxs xx oa cxo ratado do a x. oxi x. oco o aô: PPO it XOXÍXÍpld aoloctioí! PO: C02 paxa dar .rxxcaxàxoxaitoxx oo C2 poda xiepix,}.o' a Sixp s.3 ioxta •r La xatico ipoa o; CD,.......&gt; CO:&gt; Cada}; CCb lado} ο 2H4- o- 2o- —a CD ladas a ΗχΟOXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXXX (332 x 2 x oxx the at-ab1 X of the ρχοχΟχιρίχ the xxo X, X d:. Spindle · r · boxta toadoo acid d: lraco doaaprXoaçõo the aòaxodxo X: the X :: ta 1. pxxxaoxxxxx aooxicxxxs. ..!. o xx x the oxo REATY the hollow oxy x AO: PPO it XOXÍXÍpld aoloctioí PO: C02 paxa give .rxxcaxàxoxaitoxx oo C2 xiepix pruning} 'a • r Sixp s.3 ioxta La xatico the ipoa; CD , ....... &gt; CO: &gt; Each side CCC is expressed as χ2

CoiaodCoiaod

CO (ada) r tf 4 d.......&gt; OOH (adCCO (ada) r tf 4 d ....... &gt; OOH (adC

(COHV ·χ 2Hd o 2a ......&gt; CH, o OH ioládp é ECno CO 4· Η·&gt;0 4 β ......··&gt; O lais) 4· OH |aia| 4 ΟΝΟ Ocfs) a HO a e ........&gt;· CH;í OHoOIÓ —&lt;4 OHoCHg |Oio#roaila| |Caiy(COHV · χ 2Hd and 2a ......> CH, OH OHoladp is ECno CO 4 · Η · 0 4 β ································································· | 4 ΟΝΟ Ocfs) at HO at e ........ &gt; · CH; OHOO &lt; 4 &gt; Caiy

CH:; 4 CO —&gt; CHr-CO faii)ONrOO ISiS| 4 2HO 4 20..........&gt; 040*002 4 i-pO ÍCoAi ou 00¾ 4 co ·~~~4* CH;&gt; -OOpia) CHí-CDlâia) ;-4 Hp 4 β —a CHOCHO CH;;CHO 4 Os&quot; 4 a- —CòúrOH ± :H;;0 €HrCH 4 HO OHrCOò (0SH0CH :; 4 CO - &gt; CH₂-CO₂). 4 2HO 4 20 .......... &gt; 040 * 002 4 i-pOoCoAi or 004 4 co-4-CH; -CH 2 CH 3 -CH 2 CH 3 -CH 2 CH 3 -CH (CH 3) 4-Amino-1H-indole

Os òléctraík^s labdi ai eidos úproa-ernu-iX; 22222 οο.ϊχ|?ο··γtalento cO'o,Iitico oixuloto do :2ubu::ra2.0 «loaxo-oalo a oi/utroNisi.çioThe compounds of formula (I) 22222 ο | · · · · tal tal tal tal tal tal tal tal tal tal tal tal tal tal tal tal tal tal tal tal tal tal tal tal tal tal tal tal tal tal tal tal tal tal tal tal tal tal tal tal tal tal tal

Ca* blit. ti 0.a: Ο:0|50:Π0Η ÍOa 2240000 p:40t0 2laa v 22' 22 2:2 íloo 2222222 01220.10 ΟIOÓ 25 OOO 022225 .&lt; 0 222:2:2 20022002 22 2222 â.04í25Ca blit. ti 0.a: Ο: 0: 50: Π0ΗOOa 2240000 p: 40t0 2laa v 22'22 2: 2loo 2222222 01220.10 ΟIOÓ 25 OOO 022225. 0 222: 2: 2 20022002 22 2222 â¼425

00 ΟX 222:.:2 2 0a 0220221O12»0 22 002 2?ΐ2;50d 1,05O0 0000O2: f 2ÍΌ04; 4 22::2022r iól22 dO 21&quot; 2.0020&quot; 2-0 Op202;2í2 2$ 22X2222pI.1 f 2.dá22 22 152002222:5422 0 2:0:22 0 OÍ.22 2 .Í.Í2.1. io-is S. i 0022 220 ídsbitO d.&amp; :1.;25XíS2522xUÍí22 , .«»» '% 0222 CáXOdp 2245 2222202 2245 022.20222 0 22.2 2222022. 202 04 0x2; 202-2. &gt;o ,|. o ot;. r ;&gt;oodóa i t o&gt;a id ooOr e p20: o. o c.t ra22a fpax a 2..ça o 0¾ ~ a I a a ,- |2222222222220222222 22 CXiOt .222220 022240 xlil llxi , 1. 22 .':ΐ::&lt;2θ224ϊ2 4Ot20:X20.122225 0 4 22,:2,2242: 2222 00¾ .2 0,1 X202 4X2 I. XsOCO; 2202222&amp; x2xél22 2.22 ρ2,0a22 llip, 4 2 â 2202202222-:22 022222 2222222:22222220 a 02-22-:220-02 aoaiOiof ir loa, 22222 022-22220 ;a6 a a -oa 0,.22.2222 :00001.22.2:222 22a cOt. &gt; i a22l.22.pio 22aaotodílit,ic-22 :2:20111.002022¾ foi ao Co l 2220-0 dsf'5 022 KBCOj (Mare kí p .a,) , dam membrana de em esta d a eatimaied alam: retira :: Psparaçãa de 03deli.to e aadiitm, 0 leado era de rede da pletiiaa., d potmrc i a 1 d-a ader; treme aplicemo dei de -1,-3 v .®m rdXagio a em aXêet.rmdm da radarinala .ag/mnnl, d neiapoiripio· de gás ediaaaave dei ana.lSseda em aontlano per crcrrd.eg relia faseie etildaerde eme coluna mie roerpeacov.aUe de atai idiaCiarPer. ST (0-:1,:0 eu 0-1 de dei... 01- ; 1 mm, 131/ 300 meei) e nm dC apilent 433 Xil apalpada com em dátamtar da ; momdmt ied. mede térmica íDCio r ; ama rd. irai. a me ame rtragam da a r a a e eam mm lomp de 0 , 311 mil, leram aelooradas as iediolênPPas d a: r a ai as s das prado: roa: cmm: Paae : ao.....imrser o dm e eme sr dm a na em a a a r: ima pa re a d ar -a apâe: da......ume meIdeaia doa pr ad atoe. a. p imitia de (1¾ a de 10 0; 0 para ÇK4, 13 pare Cg Hg,,· 114 para; Ορρ, d este 00 a 0 pare. dg- Pnram s dail 1 s asiles apa :da d predai a a pa n e ana d oriXirafãs dm PXèctremes: cam eme emnrde leeie ddedrii.íce. raanita ma peednpáo seXemaira de et liame eis eea de me te m d l 0 m .1. dc t r ede pe amoe' e irem. prOiit ííç â a aams a sai X ec t3: ma de eteXame (13:, 340 ? sandia a prodapéo de iss tersa de :(ρ 0% ., laMPOP x x00 ΟX 222: .2 2 0a 0220221O12 »0 22 002 2 ΐ2; 50d 1.050000002: 22ΌΌ04; 4 22 :: 2022hr 21 dO 21 &quot; 2.0020 &quot; 2-0 Op202; 2 2 2 $ 22X2222pI.1 f 2.22 22 22 152002222: 5422 0 2: 0: 22 0 22.22 2 .1.2.1. io-is S. &lt; / RTI &gt; ::::::::::::::::::::::::::::::::::::::::::::: 22222222222222222022 202-2. &gt; or, |. or ot ;. The present invention relates to a process for the preparation of a compound of formula (I): the ct ra22a fpax at 2Â ° C or 0Â ° C to 1Â ° C, - 2222222222220222222 22 CXiOt .222220 022240 xlil11xi, 1.22.: ΐ 2θ224ϊ2 4Ot20: X20.122225 0 4 22 2 , 2242: 2222 ¾ .2 0.1 X202 4X2 I. XsOCO; 2202222 & 222 222 222222: 22222220 to 02-22-: 220-02 aoaiOioFra loa, 22222 022-22220; a6 aa -o0, .22.2222: 00001.22.2: 222 22a cOt. &gt; i-222.22, 22-octadec, ic-22: 2: 20111.002022¾ was found at 2220-0 dsf'5222 KBCO (Marek et al.), the membrane of this altimaied alam: retreat :: Psparaçãa of the diester, and of the dies. shakes aplicemo gave -1, -3 .®m v rdXagio into the aXêet.rmdm radarinala .ag / mnnl, d · neiapoiripio gas ediaaaave given in ana.lSseda aontlano per em crcrrd.eg reread faseie etildaerde roerpeacov mie column. a. ST (0-: 1:: 0 and 0-1 of 1 ... 1; 1 mm, 131/300), and in the absence of a stained sample. momdmt ied. thermal meas. love you go there. to the extent of 0, 311 thousand, have read the results of the mea rms of the mea sures: in order to: aaar: ima pa re ad ar - the apa: of the ...... a meaaaa of the pr ad atoe. The. (1¾ to 10; 0 to K4, 13 pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare pare 114 114 114 114 114 114 114 114 114 114 114 114 114 114 114 114 114 114 114 114 114 114 114 114 114 114 114 114 114 114 114 114 114 114 114 114 114 114 d oriXirafãs dm PXèctremes: cam em emnrde leeie ddedrii.íce raanita m peednpáo seXemaira et useful te bond me and and CDM 0 .1 m Ede dc three piece amoe 'and go â prOiit IIc out the AASM X c T3... : watermelon maize (13 :, 340) watermelon at the same time as: (ρ 0%., laMPOP xx

Fel nti.li.aede ame amiid,a me sXemtieaiiem sia aooedm cam a deaarite: np emasipla 1 cdti euaaesgár de pae e adoeça mciXXsamo dai. isedXdicsdm as-sita par misoeradapoadeso para tmr dite moniieureçio final da a em r mo cem a lia , 3, Oen esta aieresss aio ePaimaa amrreatea maia eieesmaa daiaeta a :rsd.O:pam ppte:eelaelalti:re: d.e CO4 e -d,,. 1 a am seisgâm a ad/mpOl, data asado índice ama a ptasatiya de aXetUnmd-epdsitaa d dm ama. aedrirtirre eomo dares de mel aemeate a área ma aopmafXeie· aoaima diaamnimel, nata: emetadoisa. em dsroa de itel à data aa medra nao raroreae a. pr odii p á p de mat spí: aia ir de e r 1 pem a i.ip:a mi . a r \ 1 r e a a gn ee d e: ai d.aaear Praiatas CU (Cmp (1.0.,7%) e 111¾ (3,?%)}, a perneirai ame a ata tipm de eieetrmdepeeiufco ena eaeaed. ame atilarIn this regard, I am pleased to report the following: a) in addition to the death of a mother and a child. isedXdicsdm the sudden-TMR pair misoeradapoadeso to dictate moniieureçio in the end of the read hundred mo st, 3, oen this aieresss ay ePaimaa amrreatea Mayan eieesmaa daiaeta to: rsd.O: PAM PPTE: eelaelalti Re: from CO4 and d, ,. 1 am to 6 pm to ad / mpOl, date roast index loves to ptasatiya of aXetUnmd-epdsitaa d dm ama. the honey is added to the area of the milk and the milk is added to the milk. in which case the date shall not be less than. pr odii p a p of mat spí ry to go from 1 pem to i.ip: to me. (1.0%, 7%) and 111% (3%)), the aminoglycosides of formula (I) are in the range of from 1 to 10% by weight.

Odaxrtidade de gxdoe cie o obre e cara coafXgerapão goe ecmeritcáOdxtrity of fat and expensive coagulation

a proa bordado e bX,atro.bòi:p -:¾ O ^¾¾¾¾¾¾¾¾¾ &amp;.Í. 0^0# is OCdA X X eleot.recatai it Xcoe actd. eoa: reco; X te ocaca probabi Xddada· eaxrea;ce,da paca e Xraxaagbo de :ei:e:C'oce:ree?cdeeé cera; oadabae araie; elevedaa- ;the embroidered bow and bX, atro.bòi: p -: ¾ O ^ ¾¾¾¾¾¾¾¾¾ & 0 ^ 0 # is OCdA X X eleot.recatai it Xcoe actd. eoa: reco; X is made up of Xddada · eaxrea; ce, from paca and Xraxaagbo from: e: C'oce: ree? Cdeeé wax; oadabae araie; elevedaa-;

Ji IXbertapio de bXdaocéxria á arada eXevade pares seefce ripe de eldecrocie ot X-b, 2} &lt; n. p:e;oxá.reács cie b:Ld.roqdai.o caepet.e coe a eieco r o rocio ca o de CCe exa eeldçâd a coaxo; a ., csasa aea eae esta ; rdcceçãcc é ase tire eeeeieal à cooaeittraçáo relatlea de protdea a Ctia, laditidi u iIn the case of the oxidative putation of the putative pair of roots of the oil, Xt, 2 &lt; n. The composition of the present invention relates to the preparation of the compositions of the present invention. a, csasa aea eae is; The evaluation is based on the relative coauthorization of the Prototypes,

Faia coatd tarar qee a p roba seira· de proba toa obtida no soe seco Xo XI era; cssaa cerrasxr ar I atroa Icatrioeeea de eòectrodOí for aa. t o atadoa d Itere n t e a po t: a oc i a I. e de e Xá o t rede e οοθ:θο:οθΓροΡοο cie alecccaxdXiccce Foi. areiligado asra eél.eXe de eleetedliae dal acetdo cear o deatrlto ao Eaeaipxo I coxa a aedepra o de aoe o: c á t: ode a t: I 1X aado e t ar case f ο X de cie tcob I e raedit içada per depõe; X pá o oe-oxte peta peeaoir casra essasdXigórastbe Elasel ei o a eX:Cact:rede:pdai'tea de ssoasrgaio cc&gt;e a. Erg, I, e íalectaorebuçae cia CCe foi. afaataeda a ebrioa pestaocos os Ia ca t Ode oea cc eseooa:n.tragosea de coi.eerrdXi.rea, de rcoceItadoa da: aedepâes p:otencioob.átcpa o a gaita da ·Ρ í:a a !d v esa crlaçae ;a .oa.dv,et;. trio: eprecocntadoa xca eiea:ca 5, A eelectXrida.de Para a peodagio da opacas b.idrooarbOíiatea ee Cg. rd o ae eacectaroio arei;o.xro sasssefceva-ee para todas ao sroabi goesss r e a t cda s , Eoenee cor a i ta :cexr a ocorro.;:: iça o etr tdrd roa ar coda toe coic doía átaitoa; de eaabeoo Cg&gt; A partir; deatea eatoeoa poda corso:icd.r--'Se paa a ereXeatieXdade a alterada eoas ira poteacial eaeaoe nsegertxvcg ecr scarr caca ecacoaxrtoraçác; aXeírtrcb.irXca estia baixai cata. vet: crase a predpgáO; ssie bixtregátt ie diisriooX a pr obesa -eb ice ia e toiro der gae etiltíaot A forategao der CO é peoastdida. a eorcaxcc ai.a oco-toa ne-oee: ove a e oe:eocr:at raçdoa da: eXatt ròi.it.o xeai.a .baXcaaí .1 oo siuaodP a sossoaoâa de Cipó: à xaeea:eaida.. Ò; de eal lesse ar eats fasto do posto de ai s t a. de' ssaoaslssio de costas rs se de Cdí·/ E sapo s t ao t e ea asse solar o Pasto de gsse ess todos; os d vC d; Ipp d; f' ^ etssadoa Γϊ O &gt;&gt;P.^:CT.· a% Dia D iio a i e osssi * e pp o: r 11 a i e eepecis ioa actlaa: i 1 ;à '-.d &gt; P Í pPãíàd -piàdv de t e e t a dd ase t a rs a &gt; e pSil o POSdaiadOí s a s ís rse iiiiD.DO?í ρν.ρpif íi ··· DD iiSiOpre p seaon:ta v Éetoe fceedee coofiJisosrass que oeste alPatroda a o 0:dp a a ip ao de p r o da. t o s 11 s ra ™ as :S ma a a d 1 e e r i : a $ i. çd o (de hl d r e o &amp; r do e:e t o e dp e mantida*. : ia«0 I¥ doi, as 1,1 1 aa da. u;ta e ê 1 a l a ate e i a st s ài la a de a ceada oos; e descri, to se: eaeísdlc 1 eos- aseepaae de ssses e &lt;sá rode d t i 1 1 a a de f ai. aad l dl c axi o e a ei. t a po x a 1 ac t s ode p os 1 ç: l o p a r a o e r assa coo f Ipier a a ao 11 aa 1 d e a apodo cosi a f 1 g s. a, da soe saltados da. rexdsgãe poPadCloetitPica a -d 9 V eo. toiaçao a .êg/ddCl pars th 11 seio sdao 91 Cd.Sí ip 3% Cpò, e o &gt;11 Cpp;. dal o o lio x r edo ; dl dp d h ide 11 i da: PPa gaia t iir a &quot; des&quot; d 1 d toei: r do heo do e:o Cs (Cdps : a CiiPd s;sso: a a dáPsataísdei e:c,s s e, sele soe oleado sosaf irosa. ase s axspoo..ioil.ede.d.e d s asqserPlole scleles; do cotais: o distxiPsxisxas ssaeacrai doa locas e elaecrocscali.ti.axsa aetleess aso s risse pero s cosvc r«&amp;;&gt; de ate «p« d 1 cl r o o a sp o n o t o a Cp* a proacata loecooio: fel d ca a ri ta coo. da se eo det.eres nessas ooacrets ssçes:a: psaf er idhsap ;eas será seide.esa passa Si perito :cs essado da sócsèca srao e&lt;&gt;sp:re:S.i. repões a ds c 1 pó a i a peco x i am ee si s a c 1 d i da a a s a ο ο π d 1 ç do e p e de ri a?s aor oa.ri.adae pere.assax:esdo---se eesspao n.o- IhPsito da preaeote .iíioassção &lt; aléas dlPáCí sioaerlpdss; detalhadas de pxssaessssss a: diopseit i.eos ter; cdshdçipds isesas; esíi.i.esas paea .aao s dp repas r e qa s si de a e s 1 c 0 e da p s a e apta i a o a pp e c; e o p de taipa a: iieasse:piseoâr i ea &lt; :E^£m'énci&gt;8.ss BiPtiográfioao Y, HO-xi í 4 . Hufai: a ,· a:&gt; Ta.k-alOOtxi OOC; a. Saasxsxl:!, Folasaaxxal tomoaion oi: όΙΟιΧχαο isad oiaoloit ot aasO^iaxfst tésspexXtxUfe aaO o rsxaaoxo lo alectxoa'k:eaà.cal xmsàaaitiaax. of carfcoa stioxldo aà cooposa οΐοαίοχοόχ .· Joura®..}. of foxx çhosaiooi hosalsatap CBeàiicai COíàsainicat/ic^:;.s: {X:3h8s 11-:1¾. S, L, Coí;k;:: R, CD Mac Da.11 esad Xx, F, Saidsall s, IPoo 1: x o oleosl a a 1 aodxax o 1 ob a f € 01 ao Dal a οχϊ Cl hl. 1X CD âs xFaia coatd tarar qee a p roba seira · proba toa obtained in dry soe Xo XI era; The reaction mixture is cooled to 0 ° C. t is the tied to the po i t to the i i e of the Xa t t and the οοθ: θο: οθΓροΡοο cie alecccaxdXiccce. are hereby amended to read as follows: (a) in accordance with the procedure laid down in Article 4 (1) of Regulation (EEC) Xavier et al., Peta Peeaoir, et al., Xavier et al., Et al. Erg, I., et al. afaataeda the ebrioa pestaocos Ia ca t Ode OAS cc eseooa: n.tragosea of coi.eerrdXi.rea of the rcoceItadoa: aedepâes p: o otencioob.átcpa harmonics of Ρ · t: aa dv esa crlaçae, the .oa!. dv, et. Accordingly, the present invention relates to a method for the peeling of the opaque bareoarbothiae and Cg. The present invention relates to a process for the preparation of a pharmaceutical composition comprising a pharmaceutical composition comprising a pharmaceutical composition comprising a pharmaceutically acceptable carrier and a pharmaceutically acceptable carrier, in the presence or absence of a pharmaceutically acceptable carrier. de eaabeoo Cg &gt;Starting; The effect is altered and the poteacial anger is affected by the presence of an ecco-oxacillin screen. The reaction is reduced to cata. vet: crase a predgáOO; The biodegradability of CO is peotiddid. the eucalyptus tree is not the same as the one in which the tree is planted; the other is the tree of the tree; of eal lesse aire eats fasto of the post of ai s t a. from the backs of the sea, and from the sea to the sunbath, the grass of the sea, and all; the d vC d; Ipp d; The composition of the present invention comprises the steps of: (a) preparing a compound of the formula (II): ## STR1 ## wherein R 1 and R 2 are as hereinbefore defined. P p d d d--------------a a a a a a a a a a. and it will be possible to have the following information available at the end of the year. T he s 11 s ra ers: S e a d e e r i: a i. (1) and (2) and (2) are maintained in the range of 1 to 10%. The invention relates to a method for the preparation of the compositions of the invention in which the compositions of the present invention are described in detail in the following examples and are set forth in the following examples: asa coo f f the year 11 to 1 ai of the nickname cos 1 af 1 g s a, of the soe jumped from the rexdsgame poPadCloetitPica a -d 9 V eoe.tog / ddCl pars th 11 seio sdao 91 Cd.Si ip 3 % Cpp, and the &gt; 11 Cpp ;. dal dl dp dh ide 11 i: PPa gaia t iir a &quot; d 1 d e of the heo of the Cs (Cdps: the CiiPd s, OH: aa dáPsataísdei and c iff, seal sound oiled sosaf irosa ase s ds axspoo..ioil.ede.de asqserPlole scleles; cotais of:. distxiPsxisxas ssaeacrai gives the dens and elaecrocscali.ti.axsa aetleess aso but it is clear from the point of view of the Commission that the Commission has taken the necessary steps to ensure that the The following is a list of the most commonly used methods of analysis: </ span> </ div> <div id = a) ds c 1 powder ai sin xi am ee si sac 1 di da aasa ο ο π d 1 ç ae a ria a.ri.adae pere.assax: esdo --- if eesspao no- IhPsito da Preheat. alaas dlPáCí sioaerlpdss; detailed description of: a) diopseit i.eos ter; cdshdçipds isesas; it is clear that there is a positive correlation between the two variables. and the water partition coefficient was as follows: The title compound was prepared from the title compound as a white solid. Hufai: a, a: &gt; Ta.k-alkoxy OOC; The. SaaSxSxl: Folasaaxxal tomoaion oi: ΙΟΙΟιΧχαο ΙΟoloit o o o o o o o o o o o o o o o o o o o o o o o o o o o o is is is is is is is is is is is is is is is is is is is is is is is is is.................................................................. of the seventh session of the Council of the European Union. of the disclosure of which is hereby incorporated by reference. S, L, CO, K, R, CD, MacDr, D, X, F, Saidsall s, IPO 1: x oleosin a 1x axiom 1 to f € 01 to Dal to δχϊ Cl. 1 x CD x

Fatoot UDl19¾111. D,: D® 11 r e i X ^ d λ Cap t a a ad xi ,; Da ,, D ta v a st c o f taxe opae sto® a Xao troo late: cai reXaatXoo. of’ C02 to hybtoo a tiaras ot osxppoa: &gt; JoaxtiaX q.1 Pi ao t r oa oo 1 a t .1 o a. 1 Chotittty DC4 1DDC6; 1-1. Ca !D, D i lia: a:..:„ :F1. a a t r axod ssssoi cxs 1 xx &amp; r o o? x a 1 ox .1 cia a aalxc: t i on Pamaxosxaxntxsi aasd ixppllesss fiapicas s leaiao;: ., ilsmassai of aho : Do sta o t o 11D &quot;o f ’ ϊlixada o 0X T o tsa n DD o0 y a. η o Da i a 1.1 aitPa D D 12 0 0 ? 1Fatoot UD191911. D: D 11 r i i i i i X Cap Cap Cap Cap Cap Cap Cap Cap Cap Cap. From the foregoing, the taxon opae sto® to Xao troo late: falls reXaatXoo. of 'C02 to hybtoo to tiaras ot osxppoa: &gt; JoaxtiaX q.1 Pi at t o oo 1 to t .1 a a. 1 Chotittty DC4 1DDC6; 1-1. Ca, D, Li: a: F1. a a t r axod ssssoi cxs 1 xx & r o o x at 1 x 1 to 1 at the same rate as the non-homogeneous particles at the same time. η o Da i a 1.1 aitPa D D 12 0 0? 1

dxtmPdDP 1, hyriaeosa xsaxas .1.. .«o.aynoBtopoxx.losxs,: Xoaxaxonoo of 1X2 pa.itloi prxxap-ara a na itó aixppxxttiixg olactioiyta Cxtliod &lt;m 11 sx proáoct diatribui too lo CD9 a lec:t.ro todo elido... doornal íx f opp 1. .1 sxxd F .1 o a a x: o aliSía 1. ot r y 2 o : x D a 2 ? 4 D 3 - 4 a 1,. it&gt; lao-a, pi Xháxsh.isxoatXíi D. hl i-sooiOí 41, 2ataooxbi pad. 11 S o tis. t a v I: 1 acd a ;te 1 atiá ca x r xxd xsa; t too o x o c ffsoo D xo t ide: pa a a a x xs uo xxxe to: o iax o a .a xaxli o .:.. o .:. o:a — t ®a&gt;pe a o o aio aças o çx a a: axial.s asmi as, Jotxrnaix of ff® Elsxof.laxaissa-aiioal Soctety 13&quot;i vlDlOs 2Horiv A, ; Morada &amp;;nd B., 23aba7rxs.bi, BotM&amp;t.iod of iend^rnissaicraa in cba í5\l.si&lt;ír;.$^'&gt;cd'í;Si8Íca.i rad issirlcas o 6 ca·: bon stloaida at a copper aibrirsoda ia aqaeo^ia sotAtian, 2Br.srna3. nt tbr 22 Bens cai. Bcc;.osy,. F3xr&amp;d'a.y lanasaxorSaona 1 j 7nvo5i:cs.i Cnerxr t r y ;in Condonsscí OhABAs:· B5 0 7373 23233Ό32 6, it dará3b ; lotada snO :i&gt;: 'dasnidanb and d* d ca: a ca.dxtmPdDP 1 hyriaeosa xsaxas .1 .. ',: o.aynoBtopoxx.losxs Xoaxaxonoo of ara-1X2 prxxap pa.itloi in the ITO aixppxxttiixg olactioiyta Cxtliod &lt; 11 m sx proáoct diatribui it too CD9 LEC:. all t.ro elido ... doornal íx f opp 1.. sxxd F .1 oaax: o aliSía 1. ot ry 2 o: x D a 2? 4 D 3 - 4 to 1 ,. it &gt; lao-Î ±, β-hexahydroxyisoquinoline-4-carboxylic acid. 11 S o tis. t a v I: 1 acd a; t 1 atiá ca x r xxd xsa; t o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o o. The present invention relates to a method for the preparation of a sheet of paper in the form of a sheet of paper in the form of a sheet of paper in the form of a sheet of paper. &Lt; / RTI &gt; &lt; RTI ID = 0.0 &gt; B. &lt; / RTI &gt; : Bon stloaida at a copper polyacrylamide as described in Ethanol, 2 Br. nt tbr 22 Goods fall. Bcc; .osy ,. (A) and (b) (b) and (b) in the presence of a compound of the formula: ## STR1 ## in which R 1 is hydrogen; packed snO: i &gt;: 'dasnidanb and d * d ca: a ca.

Eliaitaocriadical radsiatidn ai CO at a aaáper aiaçorada, Baarnal sei Abastca:}. Ciasxai.at;;-y d lOa OndO} 7073-7081 ,. 1, Taxadanrd., O, dopo, L daahi. and T - Sisaol, 231 ad t r 7223073 d d a. i t:adí3 at 22272 tf d 72772; s v d: 2225732 d2; a 2; s3&gt;d|dad si.np.ia i32x'yBta.d ai as::: radon iiiaíai - I nflilds{ 111) ]. and Ocdd} &quot;· [sui 2.0aac( lOd $ j 2 aIderreadas, Jasbxnai ai £iaaOra;amd.3ttCval C beab, d t ry S 3 3 i 2 dda 2 133 &quot;- 2 3 3 , IO Sb: dibaixsb L 2d :6apstb Aj &lt; J, dasxl -adid a;:α di, C, FaaaxiaidO FdaAsnaaxaXagv at a tasBiaioiab oi a ίκηκϊρίΏηΡηό. ika. astadatata shxr idg aappaa' a Xas:t: rxtidpoad 11 sá;. iion taial ceí 7o i id S ta ta Ei nctrocdaad.at ry 3.2 22307 2 607-072, 0, aytiãvtb:; and A. 2típsgnaatPgP2i3aa- tlabtiSittdudtivSas at 2302 0Si cliitiarantia-ptapastad saspnta olactrosoa, Tha isdlbanpn at a2ias:.r anila trddttMast ;&gt;a taxa ootraat ai 12 a2dxfic2.aa &lt; aodrnal at Elas;troansd yOtnad. 3ίΑηη.ΐηΟηρ 2222 {3.7222} 23.5-236,Eliaitaocriadical radsiatidn at CO to the subsidiary, Baarnal sei Abastca:}. Fig. 1, Taxadan., O, dopo, L daahi. and T - Sisaol, 231 ad t r 7223073 d d a. i t: adi3 at 22272 tb d 72772; sv d: 2225732 d2; to 2; s3 &gt; d &g; &lt; / RTI &gt; &lt; / RTI &gt; and Ocdd), [2], [2], (2), (2), (2) and (3) and (3) are as follows: 2d: 6apstb J &lt; J dasxl the -adid;: α di C FaaaxiaidO FdaAsnaaxaXagv at the tasBiaioiab hi the ίκηκϊρίΏηΡηό ika astadatata shxr IDG aappaa 'to Xas: t: 11 rxtidpoad Sa ;. iion taial 7 CIS i.. id S ta ta Ei nctrocdaad.at ry 3.2 22307 2 607-072, 0, aytiávtb:; and A. 2típsgnaatPgP2i3aa-tlabtiSittdudtivSas at 2302 0 If it is clear from the above, the rate is lower than the rate ootraat ai 12 a2dxfic2.aa <aodrnal at Elas; troansd yOtnad 3ίΑηη.ΐηΟηρ 2222 {3.7222} 23.5-236,

Claims (2)

Ba :·;:.;νν.&gt;ί'. τοοοχτ paca ν' do ; V *V ;; ,i .d a o· cl o CiV iotupxb ux ca aelecti' aa Ç··: ;'d· ôxi&lt; XO T T ss C * X' 0 oo o ••dd·· i 0 · icUTOO abhaa .·.%,'· ·. COO: c ot - ele de. âtcts .&quot;t d;. do rboa XÓ Cp ,.· 0 o O: O OOptc 0.0 Oo ddU 0 •i vU \; · •v. :%&gt; v.· cot á de duao f a. á a a qaxi pa / 0 d i.-'.L.\Íd d xod ·ΐ*. ,. \ .·' .V í. .O,- -V- S 1 CTC XOOO: . :';á, Lu 1, a. o .1 &lt;&gt;**; ··' * d ^ :C'OT|cd.Oiic a. CO.O :'λλλ\ &gt;d.O e xos cátodo O cor. :a,ct; aa . 0 .ò s -s \ O D Ç5ÓX : a ,a'v :olo c o ; &lt;:i } .·'· ·· &lt;/.... d, uCa). a a &lt;- d bao do C •Cd'· 0 d ó. a da d a cta r.dono cto. f 0 tTta: c ado a d; •:Oa a -.0· ··'..... .1 í: i: en c o ',0: aC. od ico da o :é I 1.5 ],a. ocroqu t το.loa e d.i aeo.i·. a ida -- a.: L aa OVJ ròl.i .oo à px ’ a a o: a o stXUX odX d d -X Cci·· :'d v PTCpor O.COOC ;. OÍOÍ&gt; 1 a· o too |...\ ; V. o; oTluoáo· eixo ·ν$~. vd-&gt;n·; yiaip: ;S: Or &gt; (LO;} d a a d- a. c όί- χ,ν a o dd ;:o ΐ r 'OÒt:C5 oxeCt ralou e n:t r · á ϊ'ϊΟΟ : p\ a cátodo; u a a’· β: í doo : troes qoo pOTTTCX.CXXTC o te o.l TÇÕ, T&quot;&gt; tTodrt : X CipC litt &lt; c a dd .d do xldodo ;o CT.5T d ΌΤΤ 3..........e ........Ô..... '&quot;'P ΓΟ c •CtC τ..........í íBíoduaixc a...... do r oca r do no toa aaac. &quot;&gt; .ó CdlOO; 0 de C· ar BOOO: o, cXx.leTxc í a X XtÓU O r- OUc O &lt;50 libe r t. 0X0X05 .000 ·'··&gt; x:.'o .OO: a qao caaa N' cd V ;;ao cie catodox; το Td X t o cado; C ΐ :&gt;or d'. xa etr· odtpôo11 o a dt: TGtX -í ;·Ρ·;.ο poso 0.000 .UOc :·?: OctXXXUOX aa / 005 cf O . T .· '. pia poro a a ora 0:000 :a .de ΒοοοοίτοοοΟο d: COT: C 0.0 Ot: COTO ca Ί j ou porc o; do £&gt;iTidΰ;dSBΟΠ to f οτχχχο,ο diBdTisddo s.s. xrultic:;tp.sddd· earootip v aaraaee 0« adi çâo ·θ.β ioda &lt;ϊοοί# (1.1) λ·*; V; f! C-i :θ .1 i t o eoe caca c t;P et; o.t t a p e e acarar .··. der e e de.} d H, i .ss j&gt; V ;VGCv ;eeo de ecerae cot: s ter: C t Sp.i C aça o X, edraeteris ,ed.o; eeie * ii.L iiC doe d id te ítetilleedé set : :p:a\íICfCSSr OOli cpae acePOst de et- ae': !. .Li ίο teaoi e o, r-é: ao.ai e 0::.4 s s e c deel;. t .ai coao KHf Xq í 00:00X4 e dC i f pi ' 'vi' a Q sv 'vi' Π C id G .siiivQ i i d- vi eetd4. eeea o· enoentrapco de cei:': c .-p. de C .r es e d, 1 d, e stí: pd ei i i te i G G' s-Ba: ·;:.; Νν. &Gt; ί '. τοοοχτα τοο; V * V ;; , i.e., to the cyclodextrin, which is selected from the group consisting of: XO T T ss C * X '0 oo o •• dd ·· i 0 · icUTOO abhaa ·.%,' · ·. COO: c ot - he of. âtcts. &quot; t d ;. of the rboa XO Cp, 0 o O: · • v. :% &gt; v. (a) to (a) to (d). ,. \ .·' .Saw. 1, 2, 3, 4, 5; Lu, 1, a. or .1 &lt; &gt;**; .......... CO.O: 'λλλ'. The cathodes The color. : a, ct; aa. A compound according to any one of claims 1 to 5, wherein: &lt;: &lt; / RTI &gt; to a &lt; - d bao of C • Cd '• 0 d. a da cta r. f 0 tTta: c a d d; •: 0a -0 ················································: odic of o: is I 1.5], a. and the like. the next step is to follow the steps of the following steps: a. OiOI &gt; 1 a · or too | ... \; Grandfather; oTluoáo · eje · ν $ ~. vd- &gt;n; Y: S: Or &gt;(LO;) gives a to c, c, c to c, c, c, c, c, c, c, to cathode; : T ΌΤΤ ΌΤΤ tro tro ΌΤΤ ΌΤΤ ΌΤΤ ΌΤΤ ΌΤΤ ΌΤΤ ΌΤΤ ... ... ... ... ... ... ... ... ... ... ... ... ... ... ... ... ... ... ... ... ... ... ... ... ... ... ... ... ... ... ... ... ... ..... ..... ..... ..... ..... ..... ..... P ..... ..... ..... ..... ..... ..... ..... C ... ... ... ... ... ... ... ... ... ... ... ... ... ... ... ... ... ... ... ... ... ... ... ... ... ... ... ... ... ... ... ... ... ; and (c), the composition of claim 1, wherein the amino acid sequence of claim 1, wherein the amino acid sequence of claim 1, wherein the amino acid sequence of claim 1, OO: the cathodex of the cathodex, the X-ray of the cathode, or the X-ray of the cathodex; UOc: •••••••••••••••••••••••••••••••••••••••••••••••••••••••••••••••••••••••••••••••••••••••••••••••• " ; dSBΟΠ to οτχχχο f, ss xrultic diBdTisddo ο:; tp.sddd earootip · v 0 aaraaee "adi CaO · θ.β iodo &lt; ϊοοί # (1.1) · λ *; v f C: .1 θ successfully eoe caca ct; P et; ot t and is characterized in that it comprises the steps of: (a) reacting a compound of the formula (I) with a compound of the formula (I): wherein X and Y are as defined in formula (I). The invention relates to a method for the preparation of a pharmaceutical composition comprising a pharmaceutical composition comprising a pharmaceutically acceptable carrier and a pharmaceutically acceptable carrier. . Thus, the method of claim 1, wherein R 1 and R 2 are as defined above. t.ai coao KHf XqI 00: 00X4 and dC i ffi '' '' '' '' '' '' ''. and the enantiomer of cei: c: p. of C 1 to R 2 and d is 1, 4 - Processa de acordo com a re.l.ei;nd rcaçao : , oaraotar .prado pele 00¾ ser prerieeeete diseeisido ae eldctroilto, sete rse.de - o numa aâsidts esteres â célula el ectroqaXsd.cd, idosoc este ee acorse a oa a t WèV :VàiO..:eV,-&gt;V.QdVV.· 1 ,· ea a:ac te ta eacus ptst .....40.....U t i li ta. r etc sâ r ia: s ceia: ; 1 a a e 1 a o t r o ca:: le .teaa et: série de t;ede ; &gt; cue e efleeett : qaeéi se ea carecia ae;· : a iPtroderd.de P S cá. i al t i i rte d 1 s: t. e de r: t e e j da cante f e aaeisi ; satce a e s. v ame etc .•' VsÕt. . . . eaa vv:ido· V-V. i ii: 0: die ido ir a ii fteai.: eeoe·: aeèraçVo........cie dd e ea sà st t:re Fr* c e e o d de ice r do· e ca e e r e 1 r i: ei o a ç de a de i r aaracdoet iaade: peie arcetacèsanic de eieot adi xto peta sut:aaaar e sotuso.:.;.reaee o.a oO&quot; oo: eèaccceoi. xto.&gt; GSGG Q v; : «CO titiG iCPSi S:Ç cedo pos c pode r Vtvd ãt ' t tdtd.po ç ço eetersc cipstata. iisi; Qpi.fi ss e .:. ce ços e d.e s s s,· de de Siodo coaticae &gt;ç- vi G'p .v O G oGGi:The method according to any one of the preceding claims, characterized in that the skin layer is first introduced into the body of the present invention in accordance with the invention. at WèV: VàiO ..: eV, -> VQVVV · 1, · ea a: ac te ta eacus ptst ..... 40 ..... U ti li ta. r et al: sup: s; 1 a a e 1 a o t t o t t t t t t t t t t t t t t t. &gt; cue and efleeett: what if there was a lack of it? i al t i i rte d 1 s: t. and of r: t e e j of the cante f eaeisi; satce a and s. v ame etc. • 'VsÕt. . . . and vv: ido · V-V. (ii): (i): (i): (ii): (i) and to the extent that it does not exceed the value of the product. oo: eeaccceoi. xto. &gt; GSGG Q v; : 'CO titiG iCPSi S: Ç early pos c can be Vtvd ‡ t tt tdtd.poç eetersc cipstata. iisi; Sci. s and s s s s s s s s s s s s s s s s s s s s s s s s s s s
PT105566A 2011-03-15 2011-03-15 PROCESS FOR THE SELECTIVE ELECTROCHEMICAL CONVERSION OF CARBON DIOXIDE PT105566A (en)

Priority Applications (3)

Application Number Priority Date Filing Date Title
PT105566A PT105566A (en) 2011-03-15 2011-03-15 PROCESS FOR THE SELECTIVE ELECTROCHEMICAL CONVERSION OF CARBON DIOXIDE
PCT/PT2012/000008 WO2012125053A2 (en) 2011-03-15 2012-03-15 Process for the selective electrochemical conversion of c02 into c2 hydrocarbons
EP12715237.9A EP2686464B1 (en) 2011-03-15 2012-03-15 Process for the selective electrochemical conversion of c02 into c2 hydrocarbons

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
PT105566A PT105566A (en) 2011-03-15 2011-03-15 PROCESS FOR THE SELECTIVE ELECTROCHEMICAL CONVERSION OF CARBON DIOXIDE

Publications (1)

Publication Number Publication Date
PT105566A true PT105566A (en) 2012-09-17

Family

ID=45976495

Family Applications (1)

Application Number Title Priority Date Filing Date
PT105566A PT105566A (en) 2011-03-15 2011-03-15 PROCESS FOR THE SELECTIVE ELECTROCHEMICAL CONVERSION OF CARBON DIOXIDE

Country Status (3)

Country Link
EP (1) EP2686464B1 (en)
PT (1) PT105566A (en)
WO (1) WO2012125053A2 (en)

Families Citing this family (9)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
WO2015051211A2 (en) * 2013-10-03 2015-04-09 Brown University Electrochemical reduction of co2 at copper nanofoams
US20160253461A1 (en) * 2014-10-01 2016-09-01 Xsolis, Llc System for management and documentation of health care decisions
DE102017208518A1 (en) * 2017-05-19 2018-11-22 Siemens Aktiengesellschaft Production of dendritic electrocatalysts for the reduction of CO2 and / or CO
EP3966366A1 (en) * 2019-05-07 2022-03-16 Total Se Electrocatalysts synthesized under co2 electroreduction and related methods and uses
IT201900014580A1 (en) * 2019-08-09 2021-02-09 Laboratorio Audio Snc Di Niorettini Claudio & Doro Stefano "Process for the formation and regeneration of a copper cathode of an electrochemical cell and electrochemical cell for the production of industrial products"
CN112501649B (en) * 2020-11-22 2023-11-21 赵玉平 Composite material
CN112481663B (en) * 2020-12-15 2022-03-11 中南大学深圳研究院 Preparation method of copper nanoflower applied to efficient carbon dioxide reduction reaction to generate ethylene
CN112501662B (en) * 2020-12-15 2022-03-15 中南大学深圳研究院 Preparation method of copper nanosheet applied to efficient carbon dioxide reduction reaction for generating methane
WO2023131604A1 (en) * 2022-01-10 2023-07-13 Totalenergies Onetech Electrochemical carbon oxides reduction to ethylene

Family Cites Families (4)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US4897167A (en) * 1988-08-19 1990-01-30 Gas Research Institute Electrochemical reduction of CO2 to CH4 and C2 H4
AUPS172702A0 (en) * 2002-04-12 2002-05-23 Commonwealth Scientific And Industrial Research Organisation An electrochemical cell, a porous working electrode and a process for he conversion of a species from one oxidation state to another by the electrochemical oxidation or reduction thereof
WO2011150422A1 (en) * 2010-05-28 2011-12-01 The Trustees Of Columbia University In The City Of New York Porous metal dendrites as gas diffusion electrodes for high efficiency aqueous reduction of co2 to hydrocarbons
IL207947A0 (en) * 2010-09-02 2010-12-30 Univ Ben Gurion Manufacturing carbon - based combustibles by electrochemical decomposition of co2

Also Published As

Publication number Publication date
EP2686464B1 (en) 2018-11-14
WO2012125053A3 (en) 2013-03-28
WO2012125053A2 (en) 2012-09-20
EP2686464A2 (en) 2014-01-22
WO2012125053A4 (en) 2013-05-16

Similar Documents

Publication Publication Date Title
PT105566A (en) PROCESS FOR THE SELECTIVE ELECTROCHEMICAL CONVERSION OF CARBON DIOXIDE
Zeng et al. Resolution of deep eudicot phylogeny and their temporal diversification using nuclear genes from transcriptomic and genomic datasets
Pisano et al. Out of Himalaya: the impact of past Asian environmental changes on the evolutionary and biogeographical history of Dipodoidea (Rodentia)
Spalik et al. Amphitropic amphiantarctic disjunctions in Apiaceae subfamily Apioideae
Lin et al. Comparative chloroplast genomics reveals the evolution of Pinaceae genera and subfamilies
Loureiro et al. Review of the family Rivulidae (Cyprinodontiformes, Aplocheiloidei) and a molecular and morphological phylogeny of the annual fish genus Austrolebias Costa 1998
Irisarri et al. Unexpected cryptic species among streptophyte algae most distant to land plants
Clark et al. Phylogeny of a Neotropical clade in the Gesneriaceae: more tales of convergent evolution
Tamar et al. Evolutionary history of spiny‐tailed lizards (Agamidae: Uromastyx) from the Saharo‐Arabian region
Zhang et al. Phylotranscriptomics resolves the phylogeny of Pooideae and uncovers factors for their adaptive evolution
Wu et al. Plastome evolution in the sole hemiparasitic genus laurel dodder (Cassytha) and insights into the plastid phylogenomics of Lauraceae
Almeida et al. The evolutionary history of the African fruit bats (Chiroptera: Pteropodidae)
Zhao et al. Genetic divergence and phylogeographic history of two closely related species (Leucomeris decora and Nouelia insignis) across the'Tanaka Line'in Southwest China
Mouly et al. Phylogeny and classification of the species‐rich pantropical showy genus Ixora (Rubiaceae‐Ixoreae) with indications of geographical monophyletic units and hybrids
Fuchs et al. Synchronous intercontinental splits between assemblages of woodpeckers suggested by molecular data
Maina et al. New isolates of Sweet potato feathery mottle virus and Sweet potato virus C: Biological and molecular properties, and recombination analysis based on complete genomes
Noreen et al. Salt-induced regulation of photosynthetic capacity and ion accumulation in some genetically diverse cultivars of radish (Raphanus sativus L.)
Stuckas et al. One extinct turtle species less: Pelusios seychellensis is not extinct, it never existed
Smissen et al. Phylogenetic implications of trans-specific chloroplast DNA sequence polymorphism in New Zealand Gnaphalieae (Asteraceae)
Sortibrán et al. Nurses experience reciprocal fitness benefits from their distantly related facilitated plants
Elejalde et al. Molecular phylogeny, taxonomy and evolution of the land snail genus Iberus (Pulmonata: Helicidae)
Liao et al. A systematic study of North American Angelica species (Apiaceae) based on nrDNA ITS and cpDNA sequences and fruit morphology
Uchoi et al. RETRACTED ARTICLE: inferring phylogenetic relationships of indian citron (Citrus medica L.) based on rbc L and mat K sequences of chloroplast DNA
Fernandez et al. Emerging patterns in phylogenetic studies of trichomycterid catfishes (Teleostei, Siluriformes) and the contribution of Andean diversity
Peakall et al. A multitiered sequence capture strategy spanning broad evolutionary scales: Application for phylogenetic and phylogeographic studies of orchids

Legal Events

Date Code Title Description
BB1A Laying open of patent application

Effective date: 20111108

MM3A Annulment or lapse

Free format text: LAPSE DUE TO NON-PAYMENT OF FEES

Effective date: 20150915