PL434810A1 - Catalyst for selective reduction of NOx, in particular with ammonia, in the tail gases of the nitric acid plant, and method for its production - Google Patents

Catalyst for selective reduction of NOx, in particular with ammonia, in the tail gases of the nitric acid plant, and method for its production

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Publication number
PL434810A1
PL434810A1 PL434810A PL43481020A PL434810A1 PL 434810 A1 PL434810 A1 PL 434810A1 PL 434810 A PL434810 A PL 434810A PL 43481020 A PL43481020 A PL 43481020A PL 434810 A1 PL434810 A1 PL 434810A1
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PL
Poland
Prior art keywords
catalyst
optionally
range
precursor
nox
Prior art date
Application number
PL434810A
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Polish (pl)
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PL244075B1 (en
Inventor
Monika Ruszak
Marek Inger
Marcin Wilk
Katarzyna Antoniak-Jurak
Jakub Rajewski
Magdalena SARAMOK
Paweł KOWALIK
Original Assignee
Sieć Badawcza Łukasiewicz - Instytut Nowych Syntez Chemicznych
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Application filed by Sieć Badawcza Łukasiewicz - Instytut Nowych Syntez Chemicznych filed Critical Sieć Badawcza Łukasiewicz - Instytut Nowych Syntez Chemicznych
Priority to PL434810A priority Critical patent/PL244075B1/en
Publication of PL434810A1 publication Critical patent/PL434810A1/en
Publication of PL244075B1 publication Critical patent/PL244075B1/en

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Abstract

Przedmiotem zgłoszenia jest katalizator, który charakteryzuje się tym, że prekursor nośnika katalizatora jest złożonym hydroksytlenkiem żelazowo-glinowym, w którym stosunek molowy Fe/Al mieści się w zakresie od 1,5 do 3,0, korzystnie od 1,6 do 2,0, a finalny katalizator zawiera tlenek wanadu V2O5, którego stężenie mieści się w zakresie 1 — 10% wag. i ewentualnie tlenek lantanu La2O3 o stężeniu w zakresie od 0,1 do 5% wag., korzystnie w zakresie od 1 do 3% wag. Przedmiotem zgłoszenia jest także sposób otrzymywania katalizatora wg wynalazku, który charakteryzuje się tym, że z roztworu zawierającego co najmniej jeden glinian i co najmniej jedną rozpuszczalną w wodzie sól żelaza(II) wytrąca się złożony hydroksytlenek żelazowo - glinowy stanowiący prekursor nośnika, który poddaje się kolejno starzeniu w roztworze macierzystym, filtracji, odmywaniu wodnej zawiesiny prekursora, suszeniu, formowaniu w kształtki i kalcynacji kształtek, po czym uzyskany nośnik tlenkowy ewentualnie impregnuje się wodnym roztworem azotanu lantanu, suszy, kalcynuje a następnie impregnuje wodnym roztworem metawanadanu amonu, suszy, kalcynuje i ewentualnie powtarza się operacje impregnacji, suszenia i kalcynacji w wyniku czego uzyskuje się katalizator.The subject of the application is a catalyst characterized in that the catalyst support precursor is a complex ferro-aluminum hydroxide in which the Fe / Al molar ratio is in the range from 1.5 to 3.0, preferably from 1.6 to 2.0 and the final catalyst contains vanadium oxide V2O5, the concentration of which is in the range 1-10 wt%. and optionally La2O3 lanthanum oxide with a concentration ranging from 0.1 to 5 wt.%, preferably in the range of 1 to 3 wt.%. The subject of the application is also the method for the preparation of the catalyst according to the invention, which is characterized in that a complex iron-aluminum hydroxide precursor is precipitated from a solution containing at least one aluminate and at least one water-soluble iron (II) salt. aging in the mother liquor, filtration, washing off the aqueous suspension of the precursor, drying, forming into shapes and calcining the shapes, and then the obtained oxide carrier is optionally impregnated with an aqueous solution of lanthanum nitrate, dried, calcined and then impregnated with an aqueous solution of ammonium metavanadate, dried, calcined and optionally the impregnation, drying and calcination operations are repeated to obtain a catalyst.

PL434810A 2020-07-27 2020-07-27 Catalyst for selective reduction of NOx with ammonia in residual gases from nitric acid installations, and method of its production PL244075B1 (en)

Priority Applications (1)

Application Number Priority Date Filing Date Title
PL434810A PL244075B1 (en) 2020-07-27 2020-07-27 Catalyst for selective reduction of NOx with ammonia in residual gases from nitric acid installations, and method of its production

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
PL434810A PL244075B1 (en) 2020-07-27 2020-07-27 Catalyst for selective reduction of NOx with ammonia in residual gases from nitric acid installations, and method of its production

Publications (2)

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PL434810A1 true PL434810A1 (en) 2022-01-31
PL244075B1 PL244075B1 (en) 2023-11-27

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PL434810A PL244075B1 (en) 2020-07-27 2020-07-27 Catalyst for selective reduction of NOx with ammonia in residual gases from nitric acid installations, and method of its production

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Families Citing this family (1)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
PL448759A1 (en) 2024-06-04 2025-12-08 Sieć Badawcza Łukasiewicz - Instytut Nowych Syntez Chemicznych Radial-axial reactor for the SCR-deNOx or deN2O process

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