JP3504595B2 - Pretreatment method and pretreatment device for spent nuclear fuel - Google Patents

Pretreatment method and pretreatment device for spent nuclear fuel

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Publication number
JP3504595B2
JP3504595B2 JP2000228794A JP2000228794A JP3504595B2 JP 3504595 B2 JP3504595 B2 JP 3504595B2 JP 2000228794 A JP2000228794 A JP 2000228794A JP 2000228794 A JP2000228794 A JP 2000228794A JP 3504595 B2 JP3504595 B2 JP 3504595B2
Authority
JP
Japan
Prior art keywords
nuclear fuel
spent nuclear
pipe
pulverized
crushed
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Expired - Fee Related
Application number
JP2000228794A
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Japanese (ja)
Other versions
JP2002040189A (en
Inventor
義明 鈴木
忠博 鷲谷
務 小泉
Original Assignee
核燃料サイクル開発機構
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Priority to JP2000228794A priority Critical patent/JP3504595B2/en
Publication of JP2002040189A publication Critical patent/JP2002040189A/en
Application granted granted Critical
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Classifications

    • YGENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02EREDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E30/00Energy generation of nuclear origin
    • Y02E30/30Nuclear fission reactors
    • YGENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02WCLIMATE CHANGE MITIGATION TECHNOLOGIES RELATED TO WASTEWATER TREATMENT OR WASTE MANAGEMENT
    • Y02W30/00Technologies for solid waste management
    • Y02W30/50Reuse, recycling or recovery technologies

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  • Processing Of Solid Wastes (AREA)

Description

【発明の詳細な説明】Detailed Description of the Invention

【0001】[0001]

【発明の属する技術分野】本発明は、高速炉または高速
増殖炉における使用済核燃料からウラン・プルトニウム
等を回収する再処理工場において、使用済核燃料に再処
理を施す際に、使用済核燃料を細かくせん断して硝酸溶
液または溶融塩に溶解する前処理方法およびこの方法を
実施するための前処理装置の改良に関するものである。
TECHNICAL FIELD The present invention relates to a reprocessing plant for recovering uranium, plutonium, etc. from spent nuclear fuel in a fast reactor or a fast breeder reactor. The present invention relates to a pretreatment method of shearing and dissolving in a nitric acid solution or a molten salt, and an improvement of a pretreatment apparatus for carrying out this method.

【0002】[0002]

【従来の技術】高速炉または高速増殖炉で用いる核燃料
(以下、単に「燃料」と称す)は、燃料物質をペレット
形状に成形し、これをオーステナイト系ステンレス鋼製
の被覆管(直径約6mmの円筒管)に充填して燃料棒と
し、燃料棒同士の間隔を適切に設けるためのスペースワ
イヤを被覆管外周に巻いた後に複数の燃料棒をひとまと
めにした燃料集合体として原子炉に装荷され、炉内で燃
焼される。
2. Description of the Related Art A nuclear fuel (hereinafter simply referred to as "fuel") used in a fast reactor or a fast breeder reactor is formed by forming a fuel material into a pellet shape, which is then formed into an austenitic stainless steel cladding tube (having a diameter of about 6 mm). (Cylindrical tube) to be a fuel rod, and a space wire for appropriately providing a space between the fuel rods is wound around the outer periphery of the cladding tube, and then a plurality of fuel rods are bundled into a fuel assembly to be loaded into the reactor. Burned in the furnace.

【0003】燃焼し終えた使用済燃料からは、新たな燃
料棒を製作するために再処理により燃え残りのウランと
プルトニウムが抽出される。この再処理において、使用
済燃料棒をせん断し硝酸溶液または溶融塩に溶解する工
程を前処理と呼ぶ。
From the burned spent fuel, unburned uranium and plutonium are extracted by reprocessing to produce new fuel rods. In this reprocessing, the step of shearing the spent fuel rod and dissolving it in the nitric acid solution or the molten salt is called pretreatment.

【0004】硝酸に溶解する従来の湿式前処理において
は、使用済燃料棒は、せん断機によって3cm程度の長
さにせん断(チョップ)され、せん断機の下部に設けた
傾斜配管を経由して溶解槽にて硝酸溶解(リーチ)され
る。せん断された使用済燃料棒をハルと呼ぶが、ハル内
に含まれる使用済燃料は、溶解槽内でハルのせん断切り
口面から硝酸に溶解し、不溶解性の核分裂生成物(不溶
解残渣)をスラリーの形で含んだ硝酸溶解液となる。ま
た、ハルおよびスペースワイヤ等のせん断金属片は、硝
酸に溶解せずに溶解槽内に残存するので、これらはそれ
ぞれ別個に溶解槽より取り出される。硝酸溶解液は、後
工程にて不溶解残渣を分離除去した後にウランとプルト
ニウムに分離される。また、ハル及びスペースワイヤ等
のせん断金属片は、固体廃棄物としてハル缶に回収され
る。
In the conventional wet pretreatment which dissolves in nitric acid, a spent fuel rod is sheared (chopped) into a length of about 3 cm by a shearing machine, and is melted via an inclined pipe provided under the shearing machine. Nitric acid is dissolved (reach) in the tank. A sheared spent fuel rod is called a hull. The spent fuel contained in the hull is dissolved in nitric acid from the shear cut surface of the hull in the dissolution tank, resulting in an insoluble fission product (insoluble residue). To form a nitric acid solution containing slurry in the form of a slurry. Further, the shear metal pieces such as the hull and the space wire are not dissolved in nitric acid and remain in the dissolution tank, so that they are separately taken out from the dissolution tank. The nitric acid solution is separated into uranium and plutonium after separating and removing the insoluble residue in a later step. In addition, sheared metal pieces such as hulls and space wires are collected in hull cans as solid waste.

【0005】溶融塩に溶解する従来の乾式前処理におい
ては、使用済燃料棒は、被覆管を切り開き、管中の使用
済燃料のみを取り出して粉砕した後、溶融塩電解槽に供
給される。また、使用済燃料を被覆管ごと高温下にて酸
化させ、熱膨張等によって燃料を自然粉砕する前処理法
も提案されている。こうして粉砕された使用済燃料は、
電解槽内で溶融塩に溶解し、不溶解性の核分裂生成物
(不溶解残渣)をスラリーの形で含んだ溶融塩溶解液と
なる。また、被覆管は固体廃棄物としてハル缶に回収さ
れる。
In the conventional dry pretreatment of dissolving in a molten salt, a spent fuel rod is supplied to a molten salt electrolytic cell after the cladding tube is cut open and only the spent fuel in the tube is taken out and crushed. Further, a pretreatment method has also been proposed in which spent fuel is oxidized together with a cladding tube at a high temperature, and the fuel is naturally pulverized by thermal expansion or the like. The spent fuel crushed in this way is
It becomes a molten salt solution that dissolves in the molten salt in the electrolytic cell and contains insoluble fission products (insoluble residue) in the form of a slurry. In addition, the cladding tube is collected in a hull as solid waste.

【0006】[0006]

【発明が解決しようとする課題】従来の湿式前処理方法
では、使用済燃料を燃料集合体ごとに3cm程度の長さ
にせん断する方式のため、せん断機内に燃料集合体を横
置きにする必要があり、せん断機の設置スペースが大き
くなる結果につながっていた。
In the conventional wet pretreatment method, since the spent fuel is sheared to a length of about 3 cm for each fuel assembly, it is necessary to place the fuel assembly horizontally in the shearing machine. The result was that the installation space for the shearing machine became large.

【0007】また、溶解槽においてハルのせん断切り口
面のみが硝酸に接触することになり、せん断両端面から
使用済燃料が徐々に溶解していくため、すべての使用済
燃料が硝酸に溶解するまでには数時間の時間を要してい
た。これは、溶解槽の大型化につながり、機器製作コス
トを高騰させる原因となっていた。
Further, in the dissolution tank, only the shear cut surface of the hull comes into contact with nitric acid, and the spent fuel gradually dissolves from both end surfaces of the shear, so that all the spent fuel is dissolved in nitric acid. It took several hours. This has led to an increase in the size of the melting tank, which has caused a rise in equipment manufacturing costs.

【0008】さらに、せん断時に発生する粒状あるいは
粉状のせん断金属粉(数十μm〜数mm)は、不溶解残
渣と同様にスラリーとして溶解液に同伴して後工程に移
送されるが、不溶解残渣(数μm)に比較して大きな粒
径のため、途中の機器や配管内において堆積しやすいば
かりでなく、溶解槽内部にも堆積しやすい。かようなせ
ん断金属粉の堆積物は溶解槽からの除去が困難であり、
溶解槽自体や溶解槽以降の機器構造や運転方法を複雑に
する結果となり、運転コストや保守コストを高騰させる
原因となっていた。
Further, the granular or powdery sheared metal powder (several tens of μm to several mm) generated at the time of shearing is carried as a slurry to the dissolution liquid in the same manner as the undissolved residue and is transferred to the subsequent step. Since the particle size is larger than that of the dissolution residue (several μm), not only is it easy to deposit in the middle equipment and piping, but also easily inside the dissolution tank. Such shear metal powder deposits are difficult to remove from the melting tank,
As a result, the melting tank itself, the equipment structure after the melting tank, and the operating method are complicated, which causes a rise in operating costs and maintenance costs.

【0009】一方、従来の乾式前処理方法では、せん断
せずに被覆管を1本ずつ切り開き、内部の使用済燃料の
みを取り出す操作を行うため、単位時間当たりに処理で
きる量が少なく、前処理工程の肥大化につながってい
た。
On the other hand, in the conventional dry pretreatment method, the cladding tubes are cut open one by one without shearing and only the spent fuel in the inside is taken out. It led to the enlargement of the process.

【0010】また、使用済燃料を被覆管ごと高温下にて
酸化させ、熱膨張等によって燃料を自然粉砕する前処理
法は、現在研究開発段階に至っているが、せん断金属粉
は発生しないものの、前処理装置の大型化、操作の複雑
化につながっているのが現状である。
The pretreatment method of oxidizing the spent fuel together with the cladding tube at a high temperature and naturally crushing the fuel by thermal expansion has reached the stage of research and development, but does not generate shear metal powder, The current situation is that the pretreatment device is becoming larger and the operation is complicated.

【0011】そのため本発明の目的は、上述した従来の
使用済燃料の前処理方法のもつ問題点を改善し、溶解槽
の溶解時間の短縮化やせん断時に発生するせん断金属粉
の堆積問題の解消を図り、これによって溶解槽自体や溶
解槽以降の機器構造や運転方法を簡略化して、機器製作
コスト、運転コスト、保守コストを大幅に低減すること
ができる新規かつ改良された使用済燃料の前処理方法お
よび前処理装置を提供することである。
Therefore, an object of the present invention is to improve the problems of the above-mentioned conventional pretreatment method for spent fuel, shorten the melting time of the melting tank, and solve the problem of accumulation of sheared metal powder generated during shearing. In addition to the new and improved spent fuel, the melting tank itself and the equipment structure and operation method after the melting tank can be simplified, and the equipment manufacturing cost, operation cost, and maintenance cost can be significantly reduced. It is an object of the present invention to provide a treatment method and a pretreatment device.

【0012】さらに本発明の目的は、装置自体をコンパ
クト化でき、機器製作コストの削減および設置スペース
の縮小も可能な使用済燃料の前処理装置を提供すること
である。
A further object of the present invention is to provide a spent fuel pretreatment apparatus which can make the apparatus itself compact, reduce the manufacturing cost of equipment, and reduce the installation space.

【0013】[0013]

【課題を解決するための手段】すなわち本発明の使用済
燃料の前処理方法は、高速炉または高速増殖炉における
使用済燃料棒をオーステナイト系ステンレス鋼製の被覆
管ごと粒状または粉状に粉砕する工程、粉砕物から被覆
管粉砕物を磁気的に捕集除去して使用済燃料粉砕物を分
離する工程、分離された使用済燃料粉砕物を硝酸溶解槽
または溶融塩電解槽に移送して処理する工程からなるこ
とを特徴とするものである。
That is, the method for pretreatment of spent fuel of the present invention is to pulverize spent fuel rods in a fast reactor or fast breeder reactor together with an austenitic stainless steel cladding tube into particles or powder. Process, step of magnetically collecting and removing clad tube crushed product from crushed product to separate spent fuel crushed product, transferred separated spent fuel crushed product to nitric acid dissolving tank or molten salt electrolytic tank for processing It is characterized by comprising the steps of:

【0014】かような前処理方法によれば、オーステナ
イト系ステンレス鋼製の被覆管は粉砕工程におけるせん
断応力によりマルテンサイト系ステンレス鋼に変態する
ため強磁性を帯びる。このため、粉砕物から被覆管粉砕
物を磁気的に効率よく捕集除去することが可能となり、
使用済燃料粉砕物を容易に分離することができる。その
結果、溶解槽または溶融塩電解槽へ被覆管粉砕物の移送
量が大幅に低減し、溶解槽または溶融塩電解槽での被覆
管粉砕物の堆積を防止することができる。また、使用済
燃料粉砕物は、従来のせん断処理によるせん断物と比べ
て細かい粒状または粉状とされるため、硝酸や溶融塩に
対する溶解時間を短縮することが可能となる。
According to such a pretreatment method, the austenitic stainless steel cladding tube is transformed into martensitic stainless steel by the shearing stress in the crushing process, so that it becomes ferromagnetic. Therefore, it becomes possible to magnetically and efficiently collect and remove the pulverized product of the coated tube from the pulverized product.
The spent fuel pulverized product can be easily separated. As a result, the amount of crushed coated tube pulverized material transferred to the melting tank or the molten salt electrolysis tank is significantly reduced, and the accumulation of pulverized coated tube pulverized material in the melting tank or molten salt electrolysis tank can be prevented. Further, since the spent fuel pulverized product is made into finer particles or powder than the conventional sheared product, it is possible to shorten the dissolution time in nitric acid or molten salt.

【0015】さらに本発明の使用済燃料の前処理装置
は、高速炉または高速増殖炉における使用済燃料棒を
ーステナイト系ステンレス鋼製の被覆管ごと縦方向に挿
入する挿入部と、挿入された使用済燃料を被覆管ごと下
端から順次粉砕する粉砕部と、所定寸法に粉砕された粉
砕物のみを通過させるフィルター部と、前記フィルター
部を通過した粉砕物中の被覆管粉砕物を磁気的に捕集除
去して使用済燃料粉砕物のみを硝酸溶解槽または溶融塩
電解槽へ移送する磁気分離部とからなることを特徴とす
るものである。
Furthermore pretreatment device of the spent fuel of the present invention, o the spent fuel rods in fast reactors or fast breeder reactor
-Insert part for vertically inserting the whole cladding tube made of austenitic stainless steel, crushing part for sequentially crushing the inserted spent fuel together with the cladding tube from the lower end, and a filter for passing only the crushed product crushed to a predetermined size Part, and a magnetic separation part for magnetically collecting and removing the crushed product of the cladding tube in the crushed product that has passed through the filter part and transferring only the spent fuel crushed product to the nitric acid dissolving tank or the molten salt electrolysis tank. It is characterized by that.

【0016】前記した粉砕部は、外周に複数のせん断刃
を取り付けた回転ロータを有する構造、あるいは、外周
に複数のハンマーを揺動可能に取り付けた回転ロータを
有する構造とすることができる。
The above-mentioned crushing section may have a structure having a rotary rotor having a plurality of shear blades mounted on the outer circumference, or a structure having a rotary rotor having a plurality of hammers swingably mounted on the outer circumference.

【0017】さらに前記した磁気分離部は、回転ドラム
の内部の片側に、回転ドラムとともに回転せずかつ回転
ドラムの略半周分に相当する固定磁石を配設してなる磁
気分離手段を有し、固定磁石配設側の前記回転ドラム下
方に使用済燃料粉砕物を硝酸溶解槽または溶融塩電解槽
へ移送するための移送管を設け、固定磁石を配設してい
ない側の前記回転ドラム下方に被覆管粉砕物を排出する
ための排出管を設けた構造、あるいは、配管途中に、配
管直径を横切るように配管外部から抜き差し可能に複数
の棒状磁石を配設し、前記配管下流に使用済燃料粉砕物
を硝酸溶解槽または溶融塩電解槽へ移送するための移送
管を連接し、前記配管から分岐させて被覆管粉砕物を排
出するための切替バルブ付排出管を設けた構造とするこ
とができる。
Further, the above-mentioned magnetic separation portion has a magnetic separation means, which is provided on one side inside the rotary drum, with a fixed magnet which does not rotate together with the rotary drum and which corresponds to approximately half the circumference of the rotary drum. Provided below the rotary drum on the side where the fixed magnets are provided is a transfer pipe for transferring the spent fuel pulverized product to the nitric acid dissolving tank or the molten salt electrolysis tank, and below the rotary drum on the side where the fixed magnets are not installed. A structure provided with a discharge pipe for discharging the crushed material of the cladding pipe, or a plurality of rod-shaped magnets that can be inserted and removed from the outside of the pipe so as to cross the pipe diameter in the middle of the pipe, and the spent fuel downstream of the pipe A transfer pipe for transferring the crushed product to the nitric acid dissolving tank or the molten salt electrolysis tank may be connected, and a discharge pipe with a switching valve may be provided for branching from the pipe to discharge the crushed product of the covering pipe. it can.

【0018】かような前処理装置によれば、粉砕部と磁
気分離部とを一連のプロセスとして一つの装置内にまと
めて配設することができるため、装置全体としてコンパ
クト化が可能となる。さらに、使用済燃料棒を縦方向に
挿入するようにしたため、従来の横に挿入するせん断装
置に比べて装置の設置スペースを大幅に低減することが
できる。
According to such a pretreatment apparatus, since the crushing section and the magnetic separation section can be collectively disposed in one apparatus as a series of processes, the apparatus as a whole can be made compact. Furthermore, since the spent fuel rods are inserted vertically, the installation space of the device can be significantly reduced as compared with the conventional shearing device that is inserted horizontally.

【0019】なお、本明細書における「被覆管粉砕物」
という用語は、被覆管のみでなく、スペースワイヤ等の
燃料棒に付属する他の金属粉砕物も包含する用語として
用いている。
The "crushed product of coated tube" in the present specification
The term is used as a term that includes not only the cladding tube but also other metal pulverized materials attached to fuel rods such as space wires.

【0020】[0020]

【発明の実施の形態】図1は、本発明の前処理装置の実
施例を示す説明図であり、挿入部A、粉砕部B、フィル
ター部Cおよび磁気分離部Dをこの順で縦型に配列して
構成されている。挿入部Aは、使用済燃料棒1を縦方向
に挿入して粉砕部B方向へ押し込む装置である。粉砕部
Bは、外周に複数のせん断刃2を取り付けた回転ロータ
3を有する構造であり、挿入された使用済燃料棒1を被
覆管ごとその下端から順次粉砕する装置である。
1 is an explanatory view showing an embodiment of a pretreatment apparatus of the present invention, in which an insertion part A, a crushing part B, a filter part C and a magnetic separation part D are vertically arranged in this order. It is arranged in an array. The insertion portion A is a device that inserts the spent fuel rod 1 in the vertical direction and pushes it toward the crushing portion B. The crushing unit B has a structure having a rotating rotor 3 having a plurality of shear blades 2 attached to the outer periphery thereof, and is a device for sequentially crushing the inserted spent fuel rods 1 together with the cladding tube from the lower end thereof.

【0021】フィルター部Cは、粉砕部Bで所定寸法以
下に粉砕された粉砕物のみを通過させるメッシュをもつ
フィルター4から構成されている。また、所定寸法以下
に粉砕されなかった金属片5を排出するための排出管6
がフィルター4真上の粉砕部B側壁に設けてある。
The filter section C is composed of a filter 4 having a mesh which allows only the crushed material crushed by the crushing section B to have a predetermined size or smaller. In addition, a discharge pipe 6 for discharging the metal piece 5 that has not been crushed to a predetermined size or less.
Is provided on the side wall of the crushing section B directly above the filter 4.

【0022】磁気分離部Dは、内部に固定磁石7を配し
た回転ドラム8からなり、回転ドラム8は矢印で示す方
向に回転している。この固定磁石7は回転ドラム8とと
もに回転せず、回転ドラム8の略半周に相当する部分の
内部片側に配設されている。固定磁石7を配設してある
側の回転ドラム下方には、使用済燃料粉砕物9を硝酸溶
解槽または溶融塩電解槽(いずれも図示せず)へ移送す
るための移送管10が設けられている。また、固定磁石
7を配設していない側の回転ドラム下方には、被覆管粉
砕物11を排出するための排出管12が設けられてい
る。さらに、固定磁石7配設側の回転ドラム8に向けて
圧縮空気13を吹き付けるための圧縮空気吹き付け管1
4が、回転ドラム8の斜め下方に配設されている。な
お、固定磁石7は永久磁石であってもよく、あるいは電
磁石であってもよい。
The magnetic separation section D comprises a rotary drum 8 having a fixed magnet 7 arranged therein, and the rotary drum 8 is rotating in the direction indicated by the arrow. The fixed magnet 7 does not rotate together with the rotating drum 8 and is arranged on one side of the inner portion of a portion corresponding to substantially a half circumference of the rotating drum 8. A transfer pipe 10 for transferring the spent fuel pulverized material 9 to a nitric acid dissolving tank or a molten salt electrolytic tank (neither is shown) is provided below the rotary drum on the side where the fixed magnet 7 is arranged. ing. Further, below the rotary drum on the side where the fixed magnet 7 is not arranged, a discharge pipe 12 for discharging the crushed product 11 of the coated pipe is provided. Further, a compressed air blowing pipe 1 for blowing compressed air 13 toward the rotary drum 8 on the side where the fixed magnet 7 is disposed.
4 is disposed obliquely below the rotary drum 8. The fixed magnet 7 may be a permanent magnet or an electromagnet.

【0023】上記のごとき構成の本発明の前処理装置の
動作を述べるとともに、併せて本発明の前処理方法を説
明する。図1の挿入部Aに縦方向に押し込まれた使用済
燃料棒1は、その挿入下端が粉砕部B内で回転している
回転ロータ3方向に押し付けられ、回転ロータ3外周の
複数のせん断刃2によって、燃料棒1の被覆管はその内
部の使用済燃料ペレットと共に、直径約3mm以下の粒
状または粉状に粉砕される。本発明においては、従来の
せん断により得られる直径約3cm程度のせん断物に比
較して細かく粉砕する点が1つの特徴となっている。
The operation of the pretreatment apparatus of the present invention having the above-mentioned structure will be described, and the pretreatment method of the present invention will also be described. The spent fuel rod 1 vertically pushed into the insertion portion A of FIG. 1 has its insertion lower end pushed toward the rotating rotor 3 rotating in the crushing portion B, and has a plurality of shear blades on the outer periphery of the rotating rotor 3. 2, the cladding of the fuel rod 1 is pulverized together with the spent fuel pellets therein into a granular or powder form having a diameter of about 3 mm or less. One feature of the present invention is that it is finely pulverized as compared with a conventional sheared product having a diameter of about 3 cm obtained by shearing.

【0024】回転ロータ3により所定寸法以下に粉砕さ
れなかった金属片5は、フィルター部Cに設置したフィ
ルター4により除去されて、排出管6から排出除去され
固体廃棄物として処理される。
The metal pieces 5 that have not been crushed to a predetermined size or smaller by the rotating rotor 3 are removed by the filter 4 installed in the filter section C, discharged and discharged from the discharge pipe 6, and treated as solid waste.

【0025】フィルター4を通過した粉砕物は、磁気分
離部Dの回転ドラム8上へ落下する。粉砕物中のオース
テナイト系ステンレス鋼製の被覆管粉砕物は粉砕部にお
けるせん断応力により強磁性のマルテンサイト系ステン
レス鋼に変態しているため、回転ドラム8内部の固定磁
石7により回転ドラム8外周面に磁気的に捕集され、回
転ドラム8の回転とともに回動する。一方、回転ドラム
8上に落下した非磁性の使用済燃料粉砕物は、回転ドラ
ム8外周面に磁気的に捕集されることなく、回転ドラム
の回転方向側(図1の図面では右側)の下方に開口して
いる使用済燃料粉砕物移送管10へ落下し、硝酸溶解槽
または溶融塩電解槽へ移送されて処理される。
The pulverized material that has passed through the filter 4 falls onto the rotary drum 8 of the magnetic separation section D. The austenitic stainless steel cladding tube in the pulverized material has been transformed into ferromagnetic martensitic stainless steel due to shear stress in the pulverized portion. Therefore, the outer surface of the rotary drum 8 is fixed by the fixed magnet 7 inside the rotary drum 8. Are magnetically collected by the rotating drum 8 and rotate with the rotation of the rotating drum 8. On the other hand, the non-magnetic spent fuel pulverized material that has dropped onto the rotating drum 8 is not magnetically collected on the outer peripheral surface of the rotating drum 8 and remains on the rotating direction side (the right side in the drawing of FIG. 1) of the rotating drum. The spent fuel pulverized material transfer pipe 10 is opened downward, and is transferred to a nitric acid dissolving tank or a molten salt electrolytic tank for processing.

【0026】回転ドラム8外周面に捕集されて回転ドラ
ム8とともに回動する被覆管粉砕物は、移送管へ落下す
ることなく回転ドラム8最下端を通過するが、固定磁石
7を配設していない側へ回転してくると、固定磁石7に
よる磁気的捕捉から解放されて、回転ドラム8外周面か
ら落下し、回転ドラム8下方に開口する排出管12へ導
かれて除去され、固体廃棄物として処理される。
The crushed coated tube which is collected on the outer peripheral surface of the rotating drum 8 and rotates together with the rotating drum 8 passes through the lowermost end of the rotating drum 8 without falling into the transfer tube, but the fixed magnet 7 is provided. When it rotates toward the non-rotating side, it is released from the magnetic capture by the fixed magnet 7, falls from the outer peripheral surface of the rotating drum 8, is guided to the discharge pipe 12 opening below the rotating drum 8 and is removed, and the solid waste is discarded. Processed as a thing.

【0027】なお、回転ドラム8外周面に磁気的に捕集
された被覆管粉砕物には、細粒状または細粉状の使用済
燃料粉砕物が付着しており、かような付着物も使用済燃
料粉砕物として回収する必要がある。付着物の回収は、
回転ドラム8外周面に磁気的に捕集されている状態の被
覆管粉砕物に圧縮空気吹き付け管14から圧縮空気13
を吹き付けて被覆管粉砕物に付着している使用済燃料粉
砕物のみを払い落とすことによって効果的に行うことが
できる。
The crushed product of the cladding tube magnetically collected on the outer peripheral surface of the rotary drum 8 has a crushed product of the spent fuel in the form of fine particles or fine powder attached thereto. It is necessary to collect it as spent fuel pulverized products. The collection of deposits is
From the compressed air blowing pipe 14 to the compressed air 13 to the crushed product of the coated pipe in a state of being magnetically collected on the outer peripheral surface of the rotary drum 8.
This can be effectively carried out by spraying and blowing off only the spent fuel pulverized product adhering to the pulverized product of the cladding tube.

【0028】なお、圧縮空気13を吹き付けずに、回転
ドラム8に軽い衝撃を与えるノッカ装置(図示せず)を
設置して、回転ドラム8外周面に磁気的に捕集されてい
る状態の被覆管粉砕物に軽い衝撃を与えることによって
も、被覆管粉砕物に付着した使用済燃料粉砕物を払い落
とすことができる。
A knocker device (not shown) that gives a slight impact to the rotary drum 8 is installed without blowing the compressed air 13 to cover the outer peripheral surface of the rotary drum 8 magnetically. The spent fuel pulverized material adhering to the clad pipe pulverized product can also be removed by giving a light impact to the pulverized pipe product.

【0029】かくして、被覆管粉砕物のごとき金属粉は
その大部分が硝酸溶解槽または溶融塩電解槽へ移送され
ることなく、使用済燃料粉砕物の硝酸または溶融塩への
溶解処理を効率よく行うことができる。実際に行った実
験では、被覆管粉砕物捕集効率約70重量%を達成で
き、溶解槽への被覆管移送量を従来の1/3以下まで低
減させることができる。
Thus, most of the metal powder such as the crushed product of the cladding tube is not transferred to the nitric acid dissolving tank or the molten salt electrolysis tank, and the dissolution treatment of the spent fuel crushed product into nitric acid or the molten salt can be carried out efficiently. It can be carried out. In the actually conducted experiment, the efficiency of collecting the pulverized product of the coated tube can be achieved at about 70% by weight, and the amount of the coated tube transferred to the dissolution tank can be reduced to 1/3 or less of the conventional amount.

【0030】さらに、使用済燃料の溶媒への溶解時間
は、両者の接触面積が多くなるほど短縮できることにな
る。例えば、本発明における使用済燃料粉砕物が直径約
2mmの粒状物と考えた場合の接触面積(表面積)は、
従来のせん断により得られる直径約6mm、長さ約3c
mのせん断物の接触面積(表面積)の約50倍となり、
従って、溶解時間は最大約1/50に短縮化可能とな
る。
Further, the dissolution time of the spent fuel in the solvent can be shortened as the contact area between the two increases. For example, the contact area (surface area) when the spent fuel pulverized product in the present invention is considered as a granular product having a diameter of about 2 mm is
Approximately 6 mm in diameter and 3 c in length obtained by conventional shearing
About 50 times the contact area (surface area) of the sheared object of m,
Therefore, the dissolution time can be shortened to a maximum of about 1/50.

【0031】図2は、本発明の前処理装置の別な実施例
を示す説明図であり、図1の実施例とは磁気分離部Dの
みが相違し、他の部分は図1の実施例と同じである。従
って、図1と同じ構成部分については図1と同じ参照番
号を付すことにより説明を省略する。図2の実施例にお
ける磁気分離部D′は、フィルター部Cの下から下方へ
延びる配管15を若干斜めに傾斜させ、この配管15途
中に、配管直径を横切るように配管外部から複数の棒状
磁石16を抜き差し可能に配設してある。さらにこの配
管15の棒状磁石配設部分の下流には、使用済燃料粉砕
物9を硝酸溶解槽または溶融塩電解槽へ移送するための
移送管10が連接されている。また、棒状磁石配設部分
下流の配管15には、被覆管粉砕物11を排出するため
の排出管12が略垂直方向に延びるように分岐させてあ
り、この排出管12の分岐個所には切替バルブ17が設
けられている。
FIG. 2 is an explanatory view showing another embodiment of the pretreatment apparatus of the present invention. Only the magnetic separation part D is different from the embodiment of FIG. 1, and other parts are the same as those of the embodiment of FIG. Is the same as. Therefore, the same components as those in FIG. 1 are designated by the same reference numerals as those in FIG. In the magnetic separation part D'in the embodiment of FIG. 2, the pipe 15 extending downward from the bottom of the filter part C is slightly inclined, and a plurality of bar-shaped magnets are provided in the middle of the pipe 15 from outside the pipe so as to cross the pipe diameter. 16 is arranged so that it can be inserted and removed. Further, a transfer pipe 10 for transferring the spent fuel pulverized material 9 to a nitric acid dissolving tank or a molten salt electrolytic tank is connected downstream of the portion of the pipe 15 where the rod-shaped magnets are arranged. Further, a discharge pipe 12 for discharging the crushed product 11 of the coated pipe is branched in the pipe 15 downstream of the bar magnet arranging portion so as to extend in a substantially vertical direction. The discharge pipe 12 is switched to a branch point. A valve 17 is provided.

【0032】かような磁気分離部D′においては、フィ
ルター4を通過した粉砕物は配管15へ導かれ、棒状磁
石16配設部分を通過する際に、粉砕物中の強磁性の被
覆管粉砕物は棒状磁石16表面に磁気的に捕集され、非
磁性の使用済燃料粉砕物は棒状磁石16に磁気的に捕集
されることなく、移送管9へ導かれて硝酸溶解槽または
溶融塩電解槽へ移送されて処理される。このとき、配管
15から分岐する排出管12分岐個所に設けた切替バル
ブ17は分岐個所を閉として、使用済燃料粉砕物が排出
管12へ落下しないようにしてある。
In such a magnetic separation section D ', the crushed material that has passed through the filter 4 is guided to the pipe 15, and when it passes through the portion where the bar-shaped magnet 16 is disposed, the crushed material of the ferromagnetic coating tube in the crushed material is crushed. The substance is magnetically collected on the surface of the rod-shaped magnet 16, and the non-magnetic spent fuel pulverized product is guided to the transfer pipe 9 without being magnetically collected by the rod-shaped magnet 16 and is fed into a nitric acid dissolving tank or a molten salt. It is transferred to the electrolytic cell and processed. At this time, the switching valve 17 provided at the branch point of the discharge pipe 12 branched from the pipe 15 closes the branch point so that the spent fuel pulverized product does not drop into the discharge pipe 12.

【0033】棒状磁石16表面に電磁的に捕集された被
覆管粉砕物に付着している細粒状または細粉状の使用済
燃料粉砕物は、圧縮空気13を圧縮空気吹き付け管14
から被覆管粉砕物へ向けて吹き付けることによって払い
落とすことができる。圧縮空気13を吹き付けずに、棒
状磁石16に軽い衝撃を与えるノッカ装置(図示せず)
を設置して、棒状磁石16に捕集されている状態の被覆
管粉砕物に軽い衝撃を与えることによっても、被覆管粉
砕物に付着した使用済燃料粉砕物を払い落とすことがで
きることは、図1の実施例と同じである。
The finely pulverized or finely powdered spent fuel adhering to the clad tube pulverized material electromagnetically collected on the surface of the rod-shaped magnet 16 is compressed air 13 into the compressed air blowing tube 14.
It can be wiped off by spraying the powder toward the crushed product of the cladding tube. A knocker device (not shown) that gives a light impact to the bar-shaped magnet 16 without blowing the compressed air 13.
It is also possible to remove the spent fuel pulverized product adhering to the pulverized product of the cladding tube by applying a light impact to the pulverized product of the coated pipe in a state of being collected by the rod-shaped magnet 16. This is the same as the first embodiment.

【0034】一方、棒状磁石16に捕集された被覆管粉
砕物は、粉砕部Cでの粉砕運転を一旦停止した後、排出
管12の分岐個所に設けてある切替バルブ17を開に切
り替え、次いで棒状磁石16を引き抜いてそれらの表面
から被覆管粉砕物を払い落とし、排出管12へ落下、排
出させることができる。被覆管粉砕物を払い落とした
後、棒状磁石16を再び配管15内部に挿入し、切り替
えバルブ7を閉に切り替えた後、粉砕部Cでの粉砕運転
を再開することにより、次回の操作を開始することがで
きる。
On the other hand, for the crushed product of the coated tube collected by the bar-shaped magnet 16, after temporarily stopping the crushing operation in the crushing section C, the switching valve 17 provided at the branch point of the discharge pipe 12 is switched to open, Then, the rod-shaped magnets 16 can be pulled out, the crushed products of the coated tube can be blown off from their surfaces, and they can be dropped into the discharge pipe 12 and discharged. After removing the crushed product of the coated tube, the rod-shaped magnet 16 is again inserted into the pipe 15, the switching valve 7 is closed, and then the crushing operation in the crushing unit C is restarted to start the next operation. can do.

【0035】図1および図2の前処理装置における粉砕
部Bでは、せん断刃2を外周に取り付けた回転ロータ3
を用いた実施例を示したが、図3に示すように、複数の
ハンマー22をピン21により外周に揺動可能に取り付
けた回転ロータ23を使用することもできる。
In the crushing section B of the pretreatment apparatus shown in FIGS. 1 and 2, the rotary rotor 3 having the shear blade 2 attached to the outer periphery thereof is used.
Although the embodiment using the above is shown, as shown in FIG. 3, it is also possible to use a rotary rotor 23 in which a plurality of hammers 22 are swingably attached to the outer periphery by pins 21.

【0036】上述した本発明の前処理方法においては、
被覆管粉砕物を磁気的に捕集除去して使用済燃料粉砕物
を分離する工程を施した後に、分離された使用済燃料粉
砕物を硝酸溶解槽へ移送して溶解処理する実施態様を説
明したが、粉砕工程で得られた粒状または粉状の粉砕物
をそのまま硝酸溶解槽へ移送して粉砕物中の使用済燃料
粉砕物のみを溶解処理した後に、溶解しなかった被覆管
粉砕物を溶解処理液中から磁気的に捕集除去するように
してもよい。本発明においては、粉砕工程で使用済燃料
棒の被覆管を、従来の被覆管せん断物(ハル)よりも細
かい粒状または粉状に粉砕しているため、ハルのような
比較的大きい被覆管せん断物が溶解槽内に堆積するおそ
れが少なく、硝酸溶解液から被覆管粉砕物を磁気的に分
離除去する頻度は、従来の被覆管せん断物を除去する頻
度に比べて圧倒的に少なくできる。
In the above-mentioned pretreatment method of the present invention,
An embodiment in which after performing a step of magnetically collecting and removing the crushed clad tube to separate the crushed spent fuel, the separated crushed spent fuel is transferred to a nitric acid dissolution tank to be subjected to dissolution treatment will be described. However, the granular or powdery pulverized product obtained in the pulverization process was directly transferred to the nitric acid dissolution tank to dissolve only the spent fuel pulverized product in the pulverized product, and the undissolved clad tube pulverized product was It may be magnetically collected and removed from the dissolution treatment liquid. In the present invention, the clad tube of the spent fuel rod is crushed into finer particles or powder than the conventional clad tube shearing material (hull) in the crushing process, so that a comparatively large clad tube shear such as hull is crushed. There is little risk of deposits of substances in the dissolution tank, and the frequency of magnetically separating and removing the crushed product of the coated tube from the nitric acid solution can be far less than the frequency of removing the conventional sheared product of the coated tube.

【0037】なお、粉砕工程で得られた粒状または粉状
の粉砕物をそのまま溶融塩電解槽へ移送して溶融塩によ
る溶解、電解処理を施こした後に、被覆管粉砕物を磁気
的に捕集除去する実施態様は、あまり適切ではない。な
ぜならば、被覆管粉砕物自体が電解槽の電解能力に影響
を及ぼす可能性があるためである。
The granular or powdery pulverized product obtained in the pulverization step is transferred as it is to a molten salt electrolysis tank for dissolution by molten salt and electrolysis, and then the pulverized product of the coated tube is magnetically captured. The embodiment of collecting and removing is not very suitable. This is because the crushed product of the coated tube itself may affect the electrolytic ability of the electrolytic cell.

【0038】[0038]

【発明の効果】以上詳述したところからわかるように本
発明によれば、使用済燃料棒を被覆管ごとせん断して硝
酸溶解槽または溶融塩電解槽で前処理する際に、従来の
せん断物より細かい粒状または粉状に粉砕し、粉砕物中
の被覆管粉砕物を磁気的に捕集除去した後、使用済燃料
粉砕物のみを硝酸溶解槽または溶融塩電解槽で前処理す
るようにしたから、溶解槽への被覆管粉砕物移送量を従
来より大幅に低減させることができる。その結果、溶解
槽や配管内部に金属粉が堆積することが少なくなり、溶
解槽自体や溶解槽以降の機器構造や運転方法を簡潔にす
ることができるため、運転コストや保守コストを低減さ
せることが可能となる。
As can be seen from the above detailed description, according to the present invention, when a spent fuel rod is sheared together with a cladding tube and pretreated in a nitric acid dissolving tank or a molten salt electrolytic cell, a conventional sheared material is used. After crushing into finer granules or powder and magnetically collecting and removing the crushed product of the cladding tube in the crushed product, only the spent fuel crushed product was pretreated in the nitric acid dissolving tank or molten salt electrolytic tank Therefore, it is possible to significantly reduce the amount of the coated tube pulverized product transferred to the dissolution tank as compared with the conventional case. As a result, metal powder is less likely to be deposited inside the melting tank and piping, and the melting tank itself and the device structure and operation method after the melting tank can be simplified, thus reducing operating costs and maintenance costs. Is possible.

【0039】また、使用済燃料粉砕物を細かい粉状また
は粒状に粉砕したため、溶媒との接触面積が増大した結
果、溶解時間を大幅に短縮化できる。これにより、溶解
槽や電解槽の大きさを大幅に小型化することが可能にな
り、機器製作コストを大幅に低減できる。
Further, since the spent fuel pulverized product is pulverized into fine powdery or granular form, the contact area with the solvent is increased, and as a result, the dissolution time can be greatly shortened. As a result, the size of the melting tank and the electrolytic tank can be significantly reduced, and the device manufacturing cost can be significantly reduced.

【0040】さらに、最終的に放射性固体廃棄物として
回収される被覆管粉砕物についても、従来のせん断物に
比較して細かく粉砕されているため、ハル缶に充填する
場合に、ハル缶1個当たりの充填量を増加させることが
できる。その結果、ハル缶の数を減らすことができ、放
射性廃棄物を地中処分する際の処分コストを低減できる
という効果をもたらす。
Further, the crushed product of the coated tube which is finally recovered as radioactive solid waste is also finely crushed as compared with the conventional sheared product, so when filling the hull can, one hull can is filled. The filling amount per hit can be increased. As a result, the number of hull cans can be reduced, and the disposal cost for underground disposal of radioactive waste can be reduced.

【0041】さらに本発明の前処理装置によれば、使用
済燃料棒を縦方向に取り扱えるため、従来の横置きタイ
プのせん断処理装置に比べて、装置全体のコンパクト化
を図ることができ、装置製作コストの削減および設置ス
ペースの縮小も可能になる。
Further, according to the pretreatment apparatus of the present invention, since the spent fuel rods can be handled in the vertical direction, the apparatus as a whole can be made compact as compared with the conventional horizontal type shear treatment apparatus. It is possible to reduce the manufacturing cost and the installation space.

【0042】さらにまた、本発明の前処理装置は、その
構造が比較的簡単であるため、マニピュレータやロボッ
ト等の遠隔操作機器を用いて構成部材ごとの個別保守、
点検ならびに部品交換が可能となる。
Furthermore, since the pretreatment device of the present invention has a relatively simple structure, it is possible to perform individual maintenance for each component by using a remote control device such as a manipulator or a robot.
Inspection and parts replacement are possible.

【図面の簡単な説明】[Brief description of drawings]

【図1】本発明の前処理装置の実施例を示す説明図であ
る。
FIG. 1 is an explanatory diagram showing an embodiment of a pretreatment device of the present invention.

【図2】本発明の前処理装置の別な実施例を示す説明図
である。
FIG. 2 is an explanatory view showing another embodiment of the pretreatment apparatus of the present invention.

【図3】本発明の前処理装置で使用できる粉砕用の回転
ロータの別な実施例を示す説明図である。
FIG. 3 is an explanatory view showing another embodiment of a rotary rotor for pulverization that can be used in the pretreatment device of the present invention.

【符号の説明】[Explanation of symbols]

A:挿入部 15:配管 B:粉砕部 16:棒状磁石 C:フィルター部 17:切替バルブ D:磁気分離部 22:ハンマー 1:使用済燃料棒 23:回転ロータ 2:せん断刃 3:回転ロータ 4:フィルター 7:固定磁石 8:回転ドラム 9:使用済燃料粉砕物 10:移送管 11:被覆管粉砕物 12:排出管 13:圧縮空気 14:圧縮空気吹き付け管 A: Insertion part 15: Piping B: Grinding unit 16: Bar magnet C: Filter 17: Switching valve D: Magnetic separation part 22: Hammer 1: Spent fuel rod 23: Rotating rotor 2: Shear blade 3: Rotating rotor 4: Filter 7: Fixed magnet 8: rotating drum 9: Crushed spent fuel 10: Transfer tube 11: Crushed tube 12: Discharge pipe 13: Compressed air 14: Compressed air blowing tube

フロントページの続き (56)参考文献 特開 平8−224498(JP,A) 特開 平11−14797(JP,A) 特開 昭59−59807(JP,A) 特開 昭60−4890(JP,A) 鈴木義明、鷲谷忠博、小山智造,I29 前処理工程における大粒径スラッジ分 離技術の開発について、日本原子力学会 「2000年秋の大会」予稿集,日本,日本 原子力学会,2000年 8月10日,第3分 冊,P555 鈴木義明、鷲谷忠博、小山智造,N12 せん断金属粉のマルテンサイト変態量 について,日本原子力学会「2001年春の 年会」要旨集,日本,日本原子力学会, 2001年 3月 5日,P718 山田誠也、小泉務、小山智造、原輝 夫、大和矢秀成り,N2 高速炉燃料再 処理用機械式脱被覆法の開発(1) − 多軸せん断破砕方式による脱被覆予備試 験−,日本原子力学会「2001年秋の大 会」予稿集,日本,日本原子力学会, 2001年 8月10日,P801 山田誠也、竹内正行、小泉務、小山智 造、高見和男、原輝夫、B58 高速炉燃 料再処理用機械式脱被覆法の開発(2) −二軸せん断破砕方式による脱被覆要 素試験−,日本原子力学会「2002年秋の 大会」予稿集,日本,日本原子力学会, 2002年 8月 5日,P524 竹内正行、山田誠也、小泉務、小山智 造、高見和男、原輝夫、B59 高速炉燃 料再処理用機械式脱被覆法の開発(3) −磁気分離法による燃料分離基礎試験 −,日本原子力学会「2002年秋の大会」 予稿集,日本,日本原子力学会,2002年 8月 5日,P525 (58)調査した分野(Int.Cl.7,DB名) G21C 19/36 G21C 19/44 Continuation of the front page (56) Reference JP-A-8-224498 (JP, A) JP-A-11-14797 (JP, A) JP-A-59-59807 (JP, A) JP-A-60-4890 (JP , A) Suzuki, A., Washiya, T., Koyama, S. I29 Development of large particle size sludge separation technology in pretreatment process, Atomic Energy Society of Japan, "Autumn of 2000" Proceedings, Japan, Atomic Energy Society of Japan, 2000 8 10th, 3rd volume, P555 Yoshiaki Suzuki, Tadahiro Washiya, Tomozo Koyama, Martensitic transformation of N12 shear metal powder, Atomic Energy Society of Japan, "Annual Meeting of Spring 2001", Japan, Atomic Energy Society of Japan, March 5, 2001, P718 Seiya Yamada, Tsutomu Koizumi, Tomozo Koyama, Teruo Hara, Hidenori Yamato, Development of mechanical decoating method for N2 fast reactor fuel reprocessing (1) -Multiaxial shear fracture method Decoating Preliminary Test by Atomic Energy-, Atomic Energy Society of Japan "Autumn Meeting of 2001", Japan, This Atomic Energy Society, August 10, 2001, P801 Seiya Yamada, Masayuki Takeuchi, Tsutomu Koizumi, Tomozo Koyama, Kazuo Takami, Teruo Hara, B58 Development of mechanical decoating method for fast reactor fuel reprocessing (2) − De-coating element test by biaxial shear crushing method, Proceedings of Atomic Energy Society of Japan "Autumn 2002 Conference", Japan, Japan Atomic Energy Society, August 5, 2002, P524 Masayuki Takeuchi, Seiya Yamada, Tsutomu Koizumi, Satoshi Koyama Zouzo, Kazuo Takami, Teruo Hara, B59 Development of mechanical decoating method for fast reactor fuel reprocessing (3) -Fuel separation basic test by magnetic separation method-, Atomic Energy Society of Japan "Autumn 2002 Fall" Proceedings, Japan , Japan Atomic Energy Society, August 5, 2002, P525 (58) Fields investigated (Int.Cl. 7 , DB name) G21C 19/36 G21C 19/44

Claims (10)

(57)【特許請求の範囲】(57) [Claims] 【請求項1】 高速炉または高速増殖炉における使用済
核燃料棒をオーステナイト系ステンレス鋼製の被覆管ご
と粒状または粉状に粉砕する工程、粉砕物から被覆管粉
砕物を磁気的に捕集除去して使用済核燃料粉砕物を分離
する工程、分離された使用済核燃料粉砕物を硝酸溶解槽
または溶融塩電解槽に移送して処理する工程からなるこ
とを特徴とする使用済核燃料の前処理方法。
1. A step of pulverizing spent nuclear fuel rods in a fast reactor or a fast breeder reactor together with an austenitic stainless steel cladding tube into a granular or powder form, and magnetically collecting and removing the pulverized cladding material from the pulverized material. And a process for separating the separated spent nuclear fuel pulverized product into a nitric acid dissolving tank or a molten salt electrolytic bath for processing.
【請求項2】 前記使用済核燃料粉砕物の分離工程の後
に、磁気的に捕集されている状態の被覆管粉砕物に圧縮
空気を吹き付けあるいは軽い衝撃を与えることによっ
て、被覆管粉砕物に付着している使用済核燃料粉砕物を
払い落として回収する工程をさらに含むことを特徴とす
る請求項1に記載の使用済核燃料の前処理方法。
2. After the spent nuclear fuel pulverized product is separated, it is adhered to the pulverized product of the cladding tube by blowing compressed air or applying a light impact to the pulverized product of the cladding tube in a magnetically collected state. The pretreatment method for spent nuclear fuel according to claim 1, further comprising a step of scraping off and recovering the spent nuclear fuel pulverized product.
【請求項3】 高速炉または高速増殖炉における使用済
核燃料棒を被覆管ごと粒状または粉状に粉砕する工程、
粉砕された粉砕物を硝酸溶解槽または溶融塩電解槽に移
送して使用済核燃料粉砕物を硝酸溶解処理または溶融塩
電解処理する工程、処理液から被覆管粉砕物を磁気的に
捕集除去する工程からなることを特徴とする使用済核燃
料の前処理方法。
3. A process of pulverizing a spent nuclear fuel rod in a fast reactor or a fast breeder reactor together with a cladding tube into a granular or powder form,
A step of transferring the crushed pulverized product to a nitric acid dissolving tank or a molten salt electrolysis tank to perform a nitric acid dissolving treatment or a molten salt electrolytic treatment of the spent nuclear fuel pulverized product, and magnetically collecting and removing the pulverized clad tube from the treatment liquid. A pretreatment method for spent nuclear fuel, comprising a process.
【請求項4】 高速炉または高速増殖炉における使用済
核燃料棒をオーステナイト系ステンレス鋼製の被覆管ご
と縦方向に挿入する挿入部と、挿入された使用済核燃料
を被覆管ごと下端から順次粉砕する粉砕部と、所定寸法
に粉砕された粉砕物のみを通過させるフィルター部と、
前記フィルター部を通過した粉砕物中の被覆管粉砕物を
磁気的に捕集除去して使用済核燃料粉砕物のみを硝酸溶
解槽または溶融塩電解槽へ移送する磁気分離部とからな
ることを特徴とする使用済核燃料の前処理装置。
4. An insertion part for vertically inserting a spent nuclear fuel rod in a fast reactor or a fast breeder reactor together with an austenitic stainless steel cladding tube, and the inserted spent nuclear fuel together with the cladding tube is crushed sequentially from the lower end. A crushing unit and a filter unit that allows only a crushed product crushed to a predetermined size to pass through,
It is characterized by comprising a magnetic separation part for magnetically collecting and removing the crushed product of the cladding tube in the crushed product that has passed through the filter part and transferring only the spent nuclear fuel crushed product to the nitric acid dissolving tank or the molten salt electrolytic tank. Pretreatment equipment for spent nuclear fuel.
【請求項5】 前記粉砕部は、外周に複数のせん断刃を
取り付けた回転ロータを有する構造としたことを特徴と
する請求項4に記載の使用済核燃料の前処理装置。
5. The spent nuclear fuel pretreatment device according to claim 4, wherein the crushing unit has a structure having a rotating rotor having a plurality of shear blades attached to the outer periphery thereof.
【請求項6】 前記粉砕部は、外周に複数のハンマーを
揺動可能に取り付けた回転ロータを有する構造としたこ
とを特徴とする請求項4に記載の使用済核燃料の前処理
装置。
6. The spent nuclear fuel pretreatment device according to claim 4, wherein the crushing unit has a structure having a rotary rotor on the outer periphery of which a plurality of hammers are swingably mounted.
【請求項7】 前記磁気分離部は、回転ドラムの内部の
片側に、回転ドラムとともに回転せずかつ回転ドラムの
略半周分に相当する固定磁石を配設してなる磁気分離手
段を有し、固定磁石配設側の前記回転ドラム下方に使用
済核燃料粉砕物を硝酸溶解槽または溶融塩電解槽へ移送
するための移送管を設け、固定磁石を配設していない側
の前記回転ドラム下方に被覆管粉砕物を排出するための
排出管を設けた構造としたことを特徴とする請求項4〜
6のいずれか1項に記載の使用済核燃料の前処理装置。
7. The magnetic separation unit has a magnetic separation means, which is provided on one side inside the rotary drum, with a fixed magnet which does not rotate together with the rotary drum and which corresponds to approximately half a circumference of the rotary drum. A transfer pipe for transferring the spent nuclear fuel pulverized product to the nitric acid dissolving tank or the molten salt electrolysis tank is provided below the rotary drum on the side where the fixed magnet is provided, and below the rotary drum on the side where the fixed magnet is not provided. A structure provided with a discharge pipe for discharging the crushed product of the covering pipe is characterized in that
The spent fuel pretreatment device according to any one of 6 above.
【請求項8】 固定磁石配設側の前記回転ドラムに向け
て圧縮空気を吹き付けるための圧縮空気吹き付け管を配
設し、あるいは前記回転ドラムに軽い衝撃を与えるノッ
カを配設し、回転ドラム表面に磁気的に捕集されている
被覆管粉砕物に付着している使用済核燃料粉砕物を払い
落として回収するようにしたことを特徴とする請求項7
に記載の使用済核燃料の前処理装置。
8. The surface of the rotary drum, wherein a compressed air blowing pipe for blowing compressed air toward the fixed drum is provided, or a knocker for giving a light impact to the rotary drum is provided. The spent nuclear fuel pulverized material adhered to the pulverized material of the cladding tube that is magnetically collected in the above is scraped off and collected.
The pretreatment device for spent nuclear fuel according to 1.
【請求項9】 前記磁気分離部は、配管途中に、配管直
径を横切るように配管外部から抜き差し可能に複数の棒
状磁石を配設し、前記配管下流に使用済核燃料粉砕物を
硝酸溶解槽または溶融塩電解槽へ移送するための移送管
を連接し、前記配管から分岐させて被覆管粉砕物を排出
するための切替バルブ付排出管を設けた構造としたこと
を特徴とする請求項4〜6のいずれか1項に記載の使用
済核燃料の前処理装置。
9. The magnetic separation unit is provided with a plurality of rod-shaped magnets in the middle of the pipe so as to be able to be inserted and removed from the outside of the pipe so as to traverse the pipe diameter, and the spent nuclear fuel pulverized product is placed in a nitric acid dissolving tank or a downstream of the pipe. 5. A structure in which a transfer pipe for transferring to the molten salt electrolyzer is connected and a discharge pipe with a switching valve for branching from the pipe and discharging the crushed product of the coated pipe is provided. The spent fuel pretreatment device according to any one of 6 above.
【請求項10】 前記棒状磁石に向けて圧縮空気を吹き
付けるための圧縮空気吹き付け管を配設し、あるいは前
記棒状磁石に軽い衝撃を与えるノッカを配設し、棒状磁
石表面に磁気的に捕集されている被覆管粉砕物に付着し
ている使用済核燃料粉砕物を払い落として回収するよう
にしたことを特徴とする請求項9に記載の使用済核燃料
の前処理装置。
10. A compressed air blowing tube for blowing compressed air toward the rod-shaped magnet is arranged, or a knocker for giving a light impact to the rod-shaped magnet is arranged to magnetically collect on the surface of the rod-shaped magnet. The spent nuclear fuel pretreatment device according to claim 9, wherein the spent nuclear fuel pulverized material adhering to the clad tube pulverized material is scraped off and collected.
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Non-Patent Citations (5)

* Cited by examiner, † Cited by third party
Title
山田誠也、小泉務、小山智造、原輝夫、大和矢秀成り,N2 高速炉燃料再処理用機械式脱被覆法の開発(1) −多軸せん断破砕方式による脱被覆予備試験−,日本原子力学会「2001年秋の大会」予稿集,日本,日本原子力学会,2001年 8月10日,P801
山田誠也、竹内正行、小泉務、小山智造、高見和男、原輝夫、B58 高速炉燃料再処理用機械式脱被覆法の開発(2) −二軸せん断破砕方式による脱被覆要素試験−,日本原子力学会「2002年秋の大会」予稿集,日本,日本原子力学会,2002年 8月 5日,P524
竹内正行、山田誠也、小泉務、小山智造、高見和男、原輝夫、B59 高速炉燃料再処理用機械式脱被覆法の開発(3) −磁気分離法による燃料分離基礎試験−,日本原子力学会「2002年秋の大会」予稿集,日本,日本原子力学会,2002年 8月 5日,P525
鈴木義明、鷲谷忠博、小山智造,I29 前処理工程における大粒径スラッジ分離技術の開発について、日本原子力学会「2000年秋の大会」予稿集,日本,日本原子力学会,2000年 8月10日,第3分冊,P555
鈴木義明、鷲谷忠博、小山智造,N12 せん断金属粉のマルテンサイト変態量について,日本原子力学会「2001年春の年会」要旨集,日本,日本原子力学会,2001年 3月 5日,P718

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