IT202100015005A1 - Processo per il recupero e la valorizzazione di poliesteri e poliammidi provenienti da manufatti polimerici di scarto - Google Patents

Processo per il recupero e la valorizzazione di poliesteri e poliammidi provenienti da manufatti polimerici di scarto Download PDF

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Publication number
IT202100015005A1
IT202100015005A1 IT102021000015005A IT202100015005A IT202100015005A1 IT 202100015005 A1 IT202100015005 A1 IT 202100015005A1 IT 102021000015005 A IT102021000015005 A IT 102021000015005A IT 202100015005 A IT202100015005 A IT 202100015005A IT 202100015005 A1 IT202100015005 A1 IT 202100015005A1
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IT
Italy
Prior art keywords
solvent
process according
polymer
temperature
stage
Prior art date
Application number
IT102021000015005A
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English (en)
Italian (it)
Inventor
Flavio Tollini
Massimo Morbidelli
Giuseppe Storti
Original Assignee
Milano Politecnico
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Milano Politecnico filed Critical Milano Politecnico
Priority to IT102021000015005A priority Critical patent/IT202100015005A1/it
Priority to US18/567,307 priority patent/US20240262975A1/en
Priority to PCT/IB2022/055289 priority patent/WO2022259142A1/en
Priority to MX2023014727A priority patent/MX2023014727A/es
Priority to EP22735228.3A priority patent/EP4352128A1/en
Priority to JP2023575996A priority patent/JP2024523242A/ja
Publication of IT202100015005A1 publication Critical patent/IT202100015005A1/it

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    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08JWORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
    • C08J11/00Recovery or working-up of waste materials
    • C08J11/04Recovery or working-up of waste materials of polymers
    • C08J11/10Recovery or working-up of waste materials of polymers by chemically breaking down the molecular chains of polymers or breaking of crosslinks, e.g. devulcanisation
    • C08J11/18Recovery or working-up of waste materials of polymers by chemically breaking down the molecular chains of polymers or breaking of crosslinks, e.g. devulcanisation by treatment with organic material
    • C08J11/22Recovery or working-up of waste materials of polymers by chemically breaking down the molecular chains of polymers or breaking of crosslinks, e.g. devulcanisation by treatment with organic material by treatment with organic oxygen-containing compounds
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08GMACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G63/00Macromolecular compounds obtained by reactions forming a carboxylic ester link in the main chain of the macromolecule
    • C08G63/02Polyesters derived from hydroxycarboxylic acids or from polycarboxylic acids and polyhydroxy compounds
    • C08G63/12Polyesters derived from hydroxycarboxylic acids or from polycarboxylic acids and polyhydroxy compounds derived from polycarboxylic acids and polyhydroxy compounds
    • C08G63/16Dicarboxylic acids and dihydroxy compounds
    • C08G63/18Dicarboxylic acids and dihydroxy compounds the acids or hydroxy compounds containing carbocyclic rings
    • C08G63/181Acids containing aromatic rings
    • C08G63/183Terephthalic acids
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08GMACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G63/00Macromolecular compounds obtained by reactions forming a carboxylic ester link in the main chain of the macromolecule
    • C08G63/78Preparation processes
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08GMACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G63/00Macromolecular compounds obtained by reactions forming a carboxylic ester link in the main chain of the macromolecule
    • C08G63/78Preparation processes
    • C08G63/82Preparation processes characterised by the catalyst used
    • C08G63/85Germanium, tin, lead, arsenic, antimony, bismuth, titanium, zirconium, hafnium, vanadium, niobium, tantalum, or compounds thereof
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08GMACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G63/00Macromolecular compounds obtained by reactions forming a carboxylic ester link in the main chain of the macromolecule
    • C08G63/88Post-polymerisation treatment
    • C08G63/90Purification; Drying
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08GMACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G63/00Macromolecular compounds obtained by reactions forming a carboxylic ester link in the main chain of the macromolecule
    • C08G63/91Polymers modified by chemical after-treatment
    • C08G63/914Polymers modified by chemical after-treatment derived from polycarboxylic acids and polyhydroxy compounds
    • C08G63/916Dicarboxylic acids and dihydroxy compounds
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08JWORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
    • C08J2367/00Characterised by the use of polyesters obtained by reactions forming a carboxylic ester link in the main chain; Derivatives of such polymers
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08JWORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
    • C08J2367/00Characterised by the use of polyesters obtained by reactions forming a carboxylic ester link in the main chain; Derivatives of such polymers
    • C08J2367/02Polyesters derived from dicarboxylic acids and dihydroxy compounds
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08JWORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
    • C08J2377/00Characterised by the use of polyamides obtained by reactions forming a carboxylic amide link in the main chain; Derivatives of such polymers
    • YGENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02WCLIMATE CHANGE MITIGATION TECHNOLOGIES RELATED TO WASTEWATER TREATMENT OR WASTE MANAGEMENT
    • Y02W30/00Technologies for solid waste management
    • Y02W30/50Reuse, recycling or recovery technologies
    • Y02W30/62Plastics recycling; Rubber recycling

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  • Chemical & Material Sciences (AREA)
  • Health & Medical Sciences (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Medicinal Chemistry (AREA)
  • Polymers & Plastics (AREA)
  • Organic Chemistry (AREA)
  • Life Sciences & Earth Sciences (AREA)
  • Sustainable Development (AREA)
  • General Chemical & Material Sciences (AREA)
  • Separation, Recovery Or Treatment Of Waste Materials Containing Plastics (AREA)
  • Polyesters Or Polycarbonates (AREA)
  • Manufacture Of Porous Articles, And Recovery And Treatment Of Waste Products (AREA)
IT102021000015005A 2021-06-09 2021-06-09 Processo per il recupero e la valorizzazione di poliesteri e poliammidi provenienti da manufatti polimerici di scarto IT202100015005A1 (it)

Priority Applications (6)

Application Number Priority Date Filing Date Title
IT102021000015005A IT202100015005A1 (it) 2021-06-09 2021-06-09 Processo per il recupero e la valorizzazione di poliesteri e poliammidi provenienti da manufatti polimerici di scarto
US18/567,307 US20240262975A1 (en) 2021-06-09 2022-06-07 Process for recovery and exploitation of polyesters and polyamides from waste polymeric artifacts
PCT/IB2022/055289 WO2022259142A1 (en) 2021-06-09 2022-06-07 Process for recovery and exploitation of polyesters and polyamides from waste polymeric artifacts
MX2023014727A MX2023014727A (es) 2021-06-09 2022-06-07 Procedimiento de recuperacion y aprovechamiento de poliesteres y poliamidas a partir de residuos de artefactos polimericos.
EP22735228.3A EP4352128A1 (en) 2021-06-09 2022-06-07 Process for recovery and exploitation of polyesters and polyamides from waste polymeric artifacts
JP2023575996A JP2024523242A (ja) 2021-06-09 2022-06-07 廃棄ポリマー加工品からのポリエステルおよびポリアミドの回収および利用のためのプロセス

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
IT102021000015005A IT202100015005A1 (it) 2021-06-09 2021-06-09 Processo per il recupero e la valorizzazione di poliesteri e poliammidi provenienti da manufatti polimerici di scarto

Publications (1)

Publication Number Publication Date
IT202100015005A1 true IT202100015005A1 (it) 2022-12-09

Family

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IT102021000015005A IT202100015005A1 (it) 2021-06-09 2021-06-09 Processo per il recupero e la valorizzazione di poliesteri e poliammidi provenienti da manufatti polimerici di scarto

Country Status (6)

Country Link
US (1) US20240262975A1 (https=)
EP (1) EP4352128A1 (https=)
JP (1) JP2024523242A (https=)
IT (1) IT202100015005A1 (https=)
MX (1) MX2023014727A (https=)
WO (1) WO2022259142A1 (https=)

Cited By (1)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
ES3052849A1 (es) * 2025-08-07 2026-01-15 Univ Valencia Politecnica Procedimiento de reciclaje químico de succinato de polibutileno y biopoliéster obtenido por dicho procedimiento

Families Citing this family (3)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
KR20260006939A (ko) * 2024-07-05 2026-01-13 에스케이케미칼 주식회사 폐 폴리에스테르 텍스타일의 처리 방법
KR20260006940A (ko) * 2024-07-05 2026-01-13 에스케이케미칼 주식회사 폐 폴리에스테르 텍스타일의 해중합 방법
CN118812841B (zh) * 2024-07-08 2026-04-10 东华大学 一种可多次水解回收pa6及其制备方法和闭环回收方法

Citations (2)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
EP3606980A1 (en) * 2017-04-21 2020-02-12 Sulzer Management AG A process to prepare a cyclic oligomer and a cyclic oligomer obtainable thereby and a process to polymerize it
EP3778744A1 (en) * 2020-03-03 2021-02-17 UAB Neo Group Processes for recycling polyethylene terephthalate

Patent Citations (2)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
EP3606980A1 (en) * 2017-04-21 2020-02-12 Sulzer Management AG A process to prepare a cyclic oligomer and a cyclic oligomer obtainable thereby and a process to polymerize it
EP3778744A1 (en) * 2020-03-03 2021-02-17 UAB Neo Group Processes for recycling polyethylene terephthalate

Non-Patent Citations (2)

* Cited by examiner, † Cited by third party
Title
HODGE PHILIP ED - LIOU GUEY-SHENG ET AL: "Cyclodepolymerization as a method for the synthesis of macrocyclic oligomers", REACTIVE AND FUNCTIONAL POLYMERS, vol. 80, 31 December 2013 (2013-12-31), pages 21 - 32, XP028655060, ISSN: 1381-5148, DOI: 10.1016/J.REACTFUNCTPOLYM.2013.12.008 *
KAMAU S D ET AL: "CYCLO-DEPOLYMERIZATION OF POLY(PROPYLENE TEREPHTHALATE): SOME RING-OPENING POLYMERIZATIONS OF THE CYCLIC OLIGOMERS PRODUCED", POLYMERS FOR ADVANCED TECHNOLOGIES, WILEY & SONS , BOGNOR REGIS, GB, vol. 14, no. 7, 1 July 2003 (2003-07-01), pages 492 - 501, XP001177207, ISSN: 1042-7147, DOI: 10.1002/PAT.360 *

Cited By (1)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
ES3052849A1 (es) * 2025-08-07 2026-01-15 Univ Valencia Politecnica Procedimiento de reciclaje químico de succinato de polibutileno y biopoliéster obtenido por dicho procedimiento

Also Published As

Publication number Publication date
US20240262975A1 (en) 2024-08-08
JP2024523242A (ja) 2024-06-28
EP4352128A1 (en) 2024-04-17
MX2023014727A (es) 2024-01-16
WO2022259142A1 (en) 2022-12-15

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