DE112014002888A5 - Bifunctional catalysts for the electrocatalytic reduction of oxygen and the oxidation of water - Google Patents

Bifunctional catalysts for the electrocatalytic reduction of oxygen and the oxidation of water Download PDF

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Publication number
DE112014002888A5
DE112014002888A5 DE112014002888.6T DE112014002888T DE112014002888A5 DE 112014002888 A5 DE112014002888 A5 DE 112014002888A5 DE 112014002888 T DE112014002888 T DE 112014002888T DE 112014002888 A5 DE112014002888 A5 DE 112014002888A5
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DE
Germany
Prior art keywords
oxidation
oxygen
water
bifunctional catalysts
electrocatalytic reduction
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Application number
DE112014002888.6T
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German (de)
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DE112014002888B4 (en
Inventor
Justus Masa
Wei Xia
Martin Muhler
Wolfgang Schumann
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Ruhr Universitaet Bochum
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Ruhr Universitaet Bochum
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Publication of DE112014002888A5 publication Critical patent/DE112014002888A5/en
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Classifications

    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/90—Selection of catalytic material
    • H01M4/9075—Catalytic material supported on carriers, e.g. powder carriers
    • H01M4/9083—Catalytic material supported on carriers, e.g. powder carriers on carbon or graphite
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J31/00—Catalysts comprising hydrides, coordination complexes or organic compounds
    • B01J31/16—Catalysts comprising hydrides, coordination complexes or organic compounds containing coordination complexes
    • B01J31/1616—Coordination complexes, e.g. organometallic complexes, immobilised on an inorganic support, e.g. ship-in-a-bottle type catalysts
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J31/00—Catalysts comprising hydrides, coordination complexes or organic compounds
    • B01J31/16—Catalysts comprising hydrides, coordination complexes or organic compounds containing coordination complexes
    • B01J31/18—Catalysts comprising hydrides, coordination complexes or organic compounds containing coordination complexes containing nitrogen, phosphorus, arsenic or antimony as complexing atoms, e.g. in pyridine ligands, or in resonance therewith, e.g. in isocyanide ligands C=N-R or as complexed central atoms
    • B01J31/1805—Catalysts comprising hydrides, coordination complexes or organic compounds containing coordination complexes containing nitrogen, phosphorus, arsenic or antimony as complexing atoms, e.g. in pyridine ligands, or in resonance therewith, e.g. in isocyanide ligands C=N-R or as complexed central atoms the ligands containing nitrogen
    • B01J31/181—Cyclic ligands, including e.g. non-condensed polycyclic ligands, comprising at least one complexing nitrogen atom as ring member, e.g. pyridine
    • B01J31/1825—Ligands comprising condensed ring systems, e.g. acridine, carbazole
    • B01J31/183—Ligands comprising condensed ring systems, e.g. acridine, carbazole with more than one complexing nitrogen atom, e.g. phenanthroline
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J2231/00—Catalytic reactions performed with catalysts classified in B01J31/00
    • B01J2231/60—Reduction reactions, e.g. hydrogenation
    • B01J2231/62—Reductions in general of inorganic substrates, e.g. formal hydrogenation, e.g. of N2
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J2231/00—Catalytic reactions performed with catalysts classified in B01J31/00
    • B01J2231/70—Oxidation reactions, e.g. epoxidation, (di)hydroxylation, dehydrogenation and analogues
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J2531/00—Additional information regarding catalytic systems classified in B01J31/00
    • B01J2531/02—Compositional aspects of complexes used, e.g. polynuclearity
    • B01J2531/0238—Complexes comprising multidentate ligands, i.e. more than 2 ionic or coordinative bonds from the central metal to the ligand, the latter having at least two donor atoms, e.g. N, O, S, P
    • B01J2531/0241—Rigid ligands, e.g. extended sp2-carbon frameworks or geminal di- or trisubstitution
    • B01J2531/025—Ligands with a porphyrin ring system or analogues thereof, e.g. phthalocyanines, corroles
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J2531/00—Additional information regarding catalytic systems classified in B01J31/00
    • B01J2531/70—Complexes comprising metals of Group VII (VIIB) as the central metal
    • B01J2531/72—Manganese
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J2531/00—Additional information regarding catalytic systems classified in B01J31/00
    • B01J2531/80—Complexes comprising metals of Group VIII as the central metal
    • B01J2531/84—Metals of the iron group
    • B01J2531/845—Cobalt
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J2531/00—Additional information regarding catalytic systems classified in B01J31/00
    • B01J2531/80—Complexes comprising metals of Group VIII as the central metal
    • B01J2531/84—Metals of the iron group
    • B01J2531/847—Nickel
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J35/00—Catalysts, in general, characterised by their form or physical properties
    • B01J35/30—Catalysts, in general, characterised by their form or physical properties characterised by their physical properties
    • B01J35/33—Electric or magnetic properties
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J37/00—Processes, in general, for preparing catalysts; Processes, in general, for activation of catalysts
    • B01J37/08—Heat treatment
    • B01J37/082—Decomposition and pyrolysis
    • B01J37/086—Decomposition of an organometallic compound, a metal complex or a metal salt of a carboxylic acid
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B82—NANOTECHNOLOGY
    • B82Y—SPECIFIC USES OR APPLICATIONS OF NANOSTRUCTURES; MEASUREMENT OR ANALYSIS OF NANOSTRUCTURES; MANUFACTURE OR TREATMENT OF NANOSTRUCTURES
    • B82Y30/00—Nanotechnology for materials or surface science, e.g. nanocomposites
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E60/00—Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
    • Y02E60/30—Hydrogen technology
    • Y02E60/50—Fuel cells

Landscapes

  • Chemical & Material Sciences (AREA)
  • Engineering & Computer Science (AREA)
  • Materials Engineering (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Organic Chemistry (AREA)
  • Inorganic Chemistry (AREA)
  • Electrochemistry (AREA)
  • General Chemical & Material Sciences (AREA)
  • Catalysts (AREA)
  • Inert Electrodes (AREA)
DE112014002888.6T 2013-06-18 2014-06-17 Bifunctional catalysts for the electrocatalytic reduction of oxygen and the oxidation of water Active DE112014002888B4 (en)

Applications Claiming Priority (3)

Application Number Priority Date Filing Date Title
DE102013211356.0 2013-06-18
DE102013211356.0A DE102013211356A1 (en) 2013-06-18 2013-06-18 BIFUNCTIONAL CATALYSTS FOR THE ELECTROCATALYTIC REDUCTION OF OXYGEN AND THE OXIDATION OF WATER
PCT/EP2014/062750 WO2014202628A2 (en) 2013-06-18 2014-06-17 Bifunctional catalysts for the electro-catalytic reduction of oxygen and the oxidation of water

Publications (2)

Publication Number Publication Date
DE112014002888A5 true DE112014002888A5 (en) 2016-03-10
DE112014002888B4 DE112014002888B4 (en) 2019-10-31

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Family Applications (2)

Application Number Title Priority Date Filing Date
DE102013211356.0A Withdrawn DE102013211356A1 (en) 2013-06-18 2013-06-18 BIFUNCTIONAL CATALYSTS FOR THE ELECTROCATALYTIC REDUCTION OF OXYGEN AND THE OXIDATION OF WATER
DE112014002888.6T Active DE112014002888B4 (en) 2013-06-18 2014-06-17 Bifunctional catalysts for the electrocatalytic reduction of oxygen and the oxidation of water

Family Applications Before (1)

Application Number Title Priority Date Filing Date
DE102013211356.0A Withdrawn DE102013211356A1 (en) 2013-06-18 2013-06-18 BIFUNCTIONAL CATALYSTS FOR THE ELECTROCATALYTIC REDUCTION OF OXYGEN AND THE OXIDATION OF WATER

Country Status (2)

Country Link
DE (2) DE102013211356A1 (en)
WO (1) WO2014202628A2 (en)

Families Citing this family (4)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
CN110544774B (en) * 2019-09-09 2020-11-10 长春理工大学 Transition metal nanocrystalline-nitrogen-doped carbon nanotube composite bifunctional catalyst and preparation method and application thereof
CN111408375A (en) * 2020-04-18 2020-07-14 台州学院 Preparation method of CoFe/C electrocatalyst
CN112331869A (en) * 2020-11-06 2021-02-05 五邑大学 Cobalt-nitrogen double-doped hybrid carbon material and preparation method thereof
CN113381031B (en) * 2021-06-11 2022-08-19 郑州大学 Forest derived air electrode material and preparation method and application thereof

Family Cites Families (5)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US7618915B2 (en) 2006-05-08 2009-11-17 University Of South Carolina Composite catalysts supported on modified carbon substrates and methods of making the same
US20100048380A1 (en) 2008-08-21 2010-02-25 Board Of Trustees Of Michigan State University Novel catalyst for oxygen reduction reaction in fuel cells
US8709295B2 (en) * 2010-04-26 2014-04-29 Los Alamos National Security, Llc Nitrogen-doped carbon-supported cobalt-iron oxygen reduction catalyst
KR101239966B1 (en) * 2010-11-04 2013-03-06 삼성전자주식회사 Positive electrode for lithium air battery, method of preparing the same, and lithium air battery employing the same
US9305716B2 (en) * 2010-12-03 2016-04-05 Imra America, Inc. Rechargeable electrochemical energy storage device

Also Published As

Publication number Publication date
DE112014002888B4 (en) 2019-10-31
DE102013211356A1 (en) 2014-12-18
WO2014202628A2 (en) 2014-12-24
WO2014202628A3 (en) 2015-02-19

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