CN108198635B - A kind of thorium base molten-salt breeder reactor (MSBR) reactor core - Google Patents
A kind of thorium base molten-salt breeder reactor (MSBR) reactor core Download PDFInfo
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- ZSLUVFAKFWKJRC-IGMARMGPSA-N 232Th Chemical compound [232Th] ZSLUVFAKFWKJRC-IGMARMGPSA-N 0.000 title claims abstract description 22
- 229910052776 Thorium Inorganic materials 0.000 title claims abstract description 22
- 150000003839 salts Chemical class 0.000 claims abstract description 101
- 239000010439 graphite Substances 0.000 claims abstract description 79
- 229910002804 graphite Inorganic materials 0.000 claims abstract description 79
- OKTJSMMVPCPJKN-UHFFFAOYSA-N Carbon Chemical compound [C] OKTJSMMVPCPJKN-UHFFFAOYSA-N 0.000 claims abstract description 78
- 239000000446 fuel Substances 0.000 claims abstract description 73
- 238000009395 breeding Methods 0.000 claims abstract description 45
- 230000001488 breeding effect Effects 0.000 claims abstract description 45
- 150000003841 chloride salts Chemical group 0.000 claims description 2
- 238000001816 cooling Methods 0.000 claims 1
- 238000001228 spectrum Methods 0.000 abstract description 32
- 230000009257 reactivity Effects 0.000 abstract description 23
- 230000009286 beneficial effect Effects 0.000 abstract description 6
- 230000000694 effects Effects 0.000 abstract description 5
- 230000035755 proliferation Effects 0.000 description 11
- 238000010586 diagram Methods 0.000 description 10
- 230000004992 fission Effects 0.000 description 9
- 238000005094 computer simulation Methods 0.000 description 7
- 238000006243 chemical reaction Methods 0.000 description 4
- 230000000052 comparative effect Effects 0.000 description 4
- 238000013461 design Methods 0.000 description 4
- 238000002474 experimental method Methods 0.000 description 4
- 239000000463 material Substances 0.000 description 3
- 239000007770 graphite material Substances 0.000 description 2
- 238000002844 melting Methods 0.000 description 2
- 230000008018 melting Effects 0.000 description 2
- 238000012986 modification Methods 0.000 description 2
- 230000004048 modification Effects 0.000 description 2
- 239000003758 nuclear fuel Substances 0.000 description 2
- YPELFRMCRYSPKZ-UHFFFAOYSA-N 4-amino-5-chloro-2-ethoxy-N-({4-[(4-fluorophenyl)methyl]morpholin-2-yl}methyl)benzamide Chemical compound CCOC1=CC(N)=C(Cl)C=C1C(=O)NCC1OCCN(CC=2C=CC(F)=CC=2)C1 YPELFRMCRYSPKZ-UHFFFAOYSA-N 0.000 description 1
- 235000010724 Wisteria floribunda Nutrition 0.000 description 1
- 238000004364 calculation method Methods 0.000 description 1
- 230000008859 change Effects 0.000 description 1
- 239000002826 coolant Substances 0.000 description 1
- 230000007547 defect Effects 0.000 description 1
- 238000011161 development Methods 0.000 description 1
- 230000008034 disappearance Effects 0.000 description 1
- 125000001153 fluoro group Chemical class F* 0.000 description 1
- 230000006872 improvement Effects 0.000 description 1
- 239000007788 liquid Substances 0.000 description 1
- 238000000034 method Methods 0.000 description 1
- 239000000203 mixture Substances 0.000 description 1
- 238000009377 nuclear transmutation Methods 0.000 description 1
- 238000005457 optimization Methods 0.000 description 1
- 239000002574 poison Substances 0.000 description 1
- 231100000614 poison Toxicity 0.000 description 1
- 239000011148 porous material Substances 0.000 description 1
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- G—PHYSICS
- G21—NUCLEAR PHYSICS; NUCLEAR ENGINEERING
- G21C—NUCLEAR REACTORS
- G21C1/00—Reactor types
- G21C1/04—Thermal reactors ; Epithermal reactors
- G21C1/06—Heterogeneous reactors, i.e. in which fuel and moderator are separated
- G21C1/22—Heterogeneous reactors, i.e. in which fuel and moderator are separated using liquid or gaseous fuel
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Abstract
本发明公开了一种钍基熔盐增殖堆堆芯,包括活性区和反射层,所述反射层包覆所述活性区,所述活性区是由燃料熔盐和由石墨制成的慢化剂栅元阵列组成,所述活性区包括中子提供区、功率展平区和增殖区,所述功率展平区包围所述中子提供区,所述增殖区包围所述功率展平区。本发明的钍基熔盐增殖堆堆芯通过改变石墨慢化剂栅元的熔盐、石墨体积比,将堆芯活性区分为混合有热谱和快谱的若干区,提高堆的增殖性能;通过设置功率展平区,延长石墨的更换周期至10年,使得反应堆具有负的温度反应性系数;通过设置轴向增殖区,可进一步提高堆的增殖性能,同时有利于堆的热工水力特性。
The invention discloses a thorium-based molten salt breeder core, comprising an active area and a reflective layer, the reflective layer wraps the active area, and the active area is a moderator made of fuel molten salt and graphite The active area includes a neutron supply area, a power flattening area and a multiplying area, the power flattening area surrounds the neutron providing area, and the multiplying area surrounds the power flattening area. The thorium-based molten salt breeder reactor core of the present invention divides the activity of the core into several areas mixed with thermal spectrum and fast spectrum by changing the volume ratio of molten salt and graphite in the graphite moderator cell, thereby improving the breeding performance of the reactor; By setting the power flattening zone, the graphite replacement cycle can be extended to 10 years, so that the reactor has a negative temperature reactivity coefficient; by setting the axial breeder zone, the breeder performance of the reactor can be further improved, and at the same time, it is beneficial to the thermal-hydraulic characteristics of the reactor. .
Description
技术领域technical field
本发明涉及熔盐堆堆芯设计领域,具体涉及一种钍基熔盐增殖堆堆芯。The invention relates to the field of molten salt reactor core design, in particular to a thorium-based molten salt breeder reactor core.
背景技术Background technique
熔盐堆是六种第四代反应堆候选堆型中唯一使用液态燃料的反应堆,在固有安全性、经济性、防核扩散和核燃料可持续发展等方面具有其独特优势。熔盐堆的燃料一方面无需像传统反应堆那样进行制造,另一方面还兼顾冷却剂的功能,当含有裂变材料的燃料熔盐以以高于自身熔点的入口温度进入堆芯并临界时,燃料发生裂变产生热量,同时又将热量带至二回路。The molten salt reactor is the only reactor using liquid fuel among the six candidate types of fourth-generation reactors, and has its unique advantages in terms of inherent safety, economy, non-proliferation and sustainable development of nuclear fuel. On the one hand, the fuel of molten salt reactor does not need to be manufactured like traditional reactors, and on the other hand, it also takes into account the function of coolant. When the molten salt of fuel containing fissile material enters the core at an inlet temperature higher than its own melting point and becomes critical, the fuel Fission occurs to generate heat, and at the same time, the heat is brought to the secondary circuit.
自熔盐堆概念诞生以来,世界上主要的熔盐增殖堆概念设计研究主要为:美国橡树岭国家实验室的熔盐增殖堆MSBR(Molten Salt Breeder Reactor),法国国家科学研究院的无慢化熔盐快堆MSFR(Molten Salt Fueled Reactor),熔盐堆实验MSRE(Molten SaltReactor Experiment),日本的FUJI系列熔盐堆以及俄国的熔盐嬗变堆MOSART。Since the birth of the molten salt reactor concept, the world's main molten salt breeder conceptual design research is mainly: Molten Salt Breeder Reactor MSBR (Molten Salt Breeder Reactor) of the Oak Ridge National Laboratory in the United States, non-moderation of the French National Academy of Sciences Molten Salt Fueled Reactor MSFR (Molten Salt Fueled Reactor), Molten Salt Reactor Experiment MSRE (Molten Salt Reactor Experiment), Japan's FUJI series molten salt reactor and Russia's molten salt transmutation reactor MOSART.
熔盐堆实验MSRE(Molten Salt Reactor Experiment)是唯一建成并运行的采用石墨为慢化剂的熔盐堆。慢化剂栅元为侧面开凹槽,横截面近似为正方形的四棱柱。相邻慢化剂的凹槽拼合在一起形成熔盐流道,供燃料盐流动带出热量。慢化剂栅元下端插入打孔的栅格板中固定其位置,排布成近似圆形的堆芯。Molten Salt Reactor Experiment MSRE (Molten Salt Reactor Experiment) is the only molten salt reactor built and running that uses graphite as moderator. The moderator cells are quadrangular prisms with side grooves and approximately square cross-sections. The grooves of the adjacent moderators are assembled together to form a molten salt flow channel for the fuel salt to flow and bring out the heat. The lower end of the moderator cell is inserted into the perforated grid plate to fix its position, and is arranged into an approximately circular core.
热堆的典型堆型为MSBR,采用FLiBe熔盐作为载体盐,石墨作为慢化剂和反射层,堆芯入口温度约560℃,出口温度约700℃,热功率为2250MW。据评估,MSBR具有正的温度反应性系数,对反应堆的安全性有严重影响,且其堆芯石墨需以四年为周期进行更换,这使得反应堆的成本也较高,其增殖比在1.06左右。The typical type of thermal reactor is MSBR, which uses FLiBe molten salt as carrier salt and graphite as moderator and reflector. It is estimated that MSBR has a positive temperature reactivity coefficient, which has a serious impact on the safety of the reactor, and its core graphite needs to be replaced every four years, which makes the cost of the reactor relatively high, and its breeding ratio is about 1.06 .
快堆的典型代表MSFR是法国国家科学研究院CNRS提出的无石墨慢化的熔盐堆快堆概念。MSFR能谱由热谱向快谱的转变可以获得较大的负温度反应性系数和空泡系数、较大的增殖比和无石墨寿命限制等独特优点。但氟盐的慢化性能较好,使得MSFR具有较大的燃料装载量,成本高,堆的倍增时间长(大于30年),且快堆技术难度也较大。The typical representative of fast reactor MSFR is the fast reactor concept of molten salt reactor without graphite moderation proposed by CNRS of the French National Academy of Sciences. The transformation of MSFR energy spectrum from thermal spectrum to fast spectrum can obtain unique advantages such as larger negative temperature reactivity coefficient and cavitation coefficient, larger reproduction ratio and no graphite lifetime limitation. However, the better moderation performance of fluorine salts makes MSFR have a large fuel loading, high cost, long doubling time of the reactor (more than 30 years), and the technical difficulty of fast reactors is also relatively large.
发明内容SUMMARY OF THE INVENTION
本发明要解决的技术问题是为了克服现有技术中堆芯增殖比不超过1.06,石墨更换周期不超过4年,温度反应性系数为正的缺陷,提供一种高功率混合能谱钍基熔盐增殖堆堆芯,其堆芯的增殖比可达1.08以上,其石墨更换周期达10年,提高了100%以上,其温度反应性系数为负。The technical problem to be solved by the present invention is to provide a high-power hybrid energy-spectrum thorium-based melting pot in order to overcome the defects in the prior art that the core breeding ratio does not exceed 1.06, the graphite replacement cycle does not exceed 4 years, and the temperature reactivity coefficient is positive. For the salt breeder reactor core, the breeder ratio of the core can reach more than 1.08, the graphite replacement cycle can reach 10 years, an increase of more than 100%, and the temperature reactivity coefficient is negative.
本发明是通过下述技术方案来解决上述技术问题:The present invention solves the above-mentioned technical problems through the following technical solutions:
一种钍基熔盐增殖堆堆芯,包括活性区和反射层,所述反射层包覆所述活性区,所述活性区包括燃料熔盐和由石墨制成的慢化剂栅元的阵列,所述活性区包括中子提供区和增殖区,所述中子提供区和所述增殖区的体积比为2.0:1~2.5:1,所述中子提供区的燃料熔盐和石墨的体积比为1:7.2~1:3.2,所述增殖区的燃料熔盐和石墨的体积比为1:3.2~1:1.8。通过大量的不同燃料熔盐和石墨体积比的堆芯计算,并综合考虑有效增殖系数、温度反应性系数和增殖比进行优化选择,将所述中子提供区的燃料熔盐和石墨的体积比设置为1:7.2~1:3.2,将所述增殖区的燃料熔盐和石墨的体积比设置为1:3.2~1:1.8。燃料熔盐和石墨的体积比等于在堆芯横截面中燃料熔盐和石墨的面积比。如此能够实现综合热谱反应堆和快谱反应堆的优点,达到较高的增殖比,使得增殖比从现有技术的1.06提高到本发明的1.08以上。由于在核燃料裂变中,可裂变核子数以增殖比为底数呈指数增长,因此即便很小的提高,经过指数运算,都会使结果产生巨大的增加,从而显著提高反应堆的效率。A thorium-based molten salt breeder core includes an active region and a reflective layer, the reflective layer wrapping the active region, the active region including a fuel molten salt and an array of moderator cells made of graphite , the active area includes a neutron supply area and a breeder area, the volume ratio of the neutron supply area and the breeder area is 2.0:1 to 2.5:1, and the fuel molten salt and graphite in the neutron supply area are mixed The volume ratio is 1:7.2-1:3.2, and the volume ratio of the fuel molten salt and graphite in the breeding zone is 1:3.2-1:1.8. Through the calculation of a large number of cores with different volume ratios of fuel molten salt and graphite, and comprehensively considering the effective breeding coefficient, temperature reactivity coefficient and breeding ratio to optimize the selection, the volume ratio of fuel molten salt and graphite in the neutron supply zone is calculated. It is set to 1:7.2-1:3.2, and the volume ratio of the fuel molten salt and graphite in the breeding zone is set to be 1:3.2-1:1.8. The volume ratio of the fuel molten salt and the graphite is equal to the area ratio of the fuel molten salt and the graphite in the cross section of the core. In this way, the advantages of the thermal spectrum reactor and the fast spectrum reactor can be integrated, and a higher breeding ratio can be achieved, so that the breeding ratio is increased from 1.06 in the prior art to more than 1.08 in the present invention. Since in nuclear fuel fission, the number of fissionable nucleons increases exponentially with the breeding ratio as the base, so even a small increase will result in a huge increase after exponential operation, thereby significantly improving the efficiency of the reactor.
优选地,所述活性区还包括第一功率展平区,所述第一功率展平区包围所述中子提供区,所述增殖区包围所述第一功率展平区,所述中子提供区和所述第一功率展平区的体积比为1:1~2.0:1,所述第一功率展平区的燃料熔盐和石墨的体积比为1:1.8~1:0.01。通过设置第一功率展平区,展平了堆芯功率分布,通过将第一功率展平区的燃料熔盐和石墨的体积比设置为1:1.8~1:0.01,优化了温度反应性系数,延长石墨更换周期。Preferably, the active region further includes a first power flattening region, the first power flattening region surrounds the neutron supply region, the breeding region surrounds the first power flattening region, and the neutron The volume ratio of the supply area and the first power flattening area is 1:1-2.0:1, and the volume ratio of the fuel molten salt and graphite in the first power flattening area is 1:1.8-1:0.01. By setting the first power flattening zone, the core power distribution is flattened. By setting the volume ratio of the fuel molten salt and graphite in the first power flattening zone to 1:1.8~1:0.01, the temperature reactivity coefficient is optimized. , to extend the graphite replacement cycle.
优选地,所述活性区还包括第一功率展平区和第二功率展平区,所述中子提供区和所述第二功率展平区的体积比为1:1~2.0:1,所述第一功率展平区的燃料熔盐和石墨的体积比为1:1.8~1:0.01,所述第二功率展平区为燃料熔盐,所述增殖区临接并围绕所述第一功率展平区,所述第一功率展平区临接并围绕所述中子提供区,所述中子提供区临接并围绕所述第二功率展平区,所述第二功率展平区位于所述活性区的中央。通过第一功率展平区和第二功率展平区的配合作用,进一步优化了温度反应性系数,使得温度反应性系数为负,保证了反应堆的安全,延长石墨更换周期。Preferably, the active region further includes a first power flattening region and a second power flattening region, and the volume ratio of the neutron providing region and the second power flattening region is 1:1˜2.0:1, The volume ratio of fuel molten salt and graphite in the first power flattening zone is 1:1.8-1:0.01, the second power flattening zone is fuel molten salt, and the breeding zone is adjacent to and surrounds the first power flattening zone. a power flattening region, the first power flattening region adjoins and surrounds the neutron providing region, the neutron providing region adjoins and surrounds the second power flattening region, the second power flattening region The flat area is located in the center of the active area. Through the cooperation of the first power flattening zone and the second power flattening zone, the temperature reactivity coefficient is further optimized, so that the temperature reactivity coefficient is negative, which ensures the safety of the reactor and prolongs the graphite replacement cycle.
优选地,所述活性区还包括第一功率展平区和第二功率展平区,所述中子提供区和所述第二功率展平区的体积比为1:1~2.0:1,所述第一功率展平区的燃料熔盐和石墨的体积比为1:1.8~1:0.01,所述第二功率展平区为燃料熔盐,所述增殖区临接并围绕所述第一功率展平区,所述第一功率展平区临接并围绕所述第二功率展平区,所述第二功率展平区临接并围绕所述中子提供区,所述中子提供区位于所述活性区的中央。通过将第一功率展平区和第二功率展平区层叠设置,进一步优化了温度反应性系数,使得温度反应性系数为负,保证了反应堆的安全,延长石墨更换周期。Preferably, the active region further includes a first power flattening region and a second power flattening region, and the volume ratio of the neutron providing region and the second power flattening region is 1:1˜2.0:1, The volume ratio of fuel molten salt and graphite in the first power flattening zone is 1:1.8-1:0.01, the second power flattening zone is fuel molten salt, and the breeding zone is adjacent to and surrounds the first power flattening zone. a power flattening region, the first power flattening region adjoining and surrounding the second power flattening region, the second power flattening region adjoining and surrounding the neutron providing region, the neutron supplying region The supply area is located in the center of the active area. By stacking the first power flattening area and the second power flattening area, the temperature reactivity coefficient is further optimized, so that the temperature reactivity coefficient is negative, which ensures the safety of the reactor and prolongs the graphite replacement cycle.
优选地,所述燃料熔盐为FLiBe熔盐。Preferably, the fuel molten salt is FLiBe molten salt.
优选地,所述燃料熔盐为LiF-BeF2-(Th+U)F4熔盐。Preferably, the fuel molten salt is LiF-BeF 2 -(Th+U)F 4 molten salt.
优选地,所述燃料熔盐为氯盐。Preferably, the fuel molten salt is a chloride salt.
优选地,所述增殖区包括径向增殖区和轴向增殖区,所述径向增殖区和所述轴向增殖区将所述中子提供区包裹在内。这样的结构能够提供中子经济性。Preferably, the proliferation region includes a radial proliferation region and an axial proliferation region, and the radial proliferation region and the axial proliferation region enclose the neutron supply region. Such a structure can provide neutron economy.
优选地,所述反射层包括径向反射层和轴向反射层,所述径向反射层围绕在活性区外围,所述轴向反射层位于所述径向反射层的两侧。Preferably, the reflection layer includes a radial reflection layer and an axial reflection layer, the radial reflection layer surrounds the periphery of the active region, and the axial reflection layer is located on both sides of the radial reflection layer.
优选地,所述轴向反射层包括上反射层和下反射层,所述上反射层位于所述活性区的正上方,并呈圆台状,所述下反射层位于所述活性区的正下方,并呈圆台状。Preferably, the axial reflection layer includes an upper reflection layer and a lower reflection layer, the upper reflection layer is located directly above the active region and is in the shape of a truncated cone, and the lower reflection layer is located directly under the active region , and in the shape of a cone.
优选地,所述慢化剂栅元的中间设置有燃料孔道,用于使燃料熔盐流经并冷却石墨慢化剂。通过改变燃料孔道的直径,能够改变燃料熔盐和石墨的体积比。Preferably, a fuel channel is provided in the middle of the moderator cell for allowing the molten fuel salt to flow through and cool the graphite moderator. By changing the diameter of the fuel pores, the volume ratio of the fuel molten salt and graphite can be changed.
优选地,所述慢化剂栅元的侧面设置有鳍,用于形成栅元之间的缝隙供燃料熔盐流通并冷却石墨慢化剂。通过改变鳍的大小,能够改变栅元之间的缝隙的大小,进而能够改变燃料熔盐和石墨的体积比。Preferably, the side surfaces of the moderator cells are provided with fins, which are used to form gaps between the cells for fuel molten salt to flow and to cool the graphite moderator. By changing the size of the fins, the size of the gap between the cells can be changed, thereby changing the volume ratio of the molten fuel salt and the graphite.
在不影响中子经济性的前提下节约石墨用料,并减轻了石墨反射层的正温度反应性效应。The graphite material is saved without affecting the neutron economy, and the positive temperature reactivity effect of the graphite reflective layer is alleviated.
在符合本领域常识的基础上,上述各优选条件,可任意组合,即得本发明各较佳实例。On the basis of conforming to common knowledge in the art, the above preferred conditions can be combined arbitrarily to obtain preferred examples of the present invention.
本发明的积极进步效果在于:本发明的钍基熔盐增殖堆堆芯通过改变石墨慢化剂栅元的熔盐、石墨体积比,将堆芯活性区分为混合有热谱和快谱的若干区,将堆芯的增殖比提高到1.08以上;通过设置功率展平区,延长石墨的更换周期至10年,使得反应堆具有负的温度反应性系数;通过设置轴向增殖区,可进一步提高堆的增殖性能,同时有利于堆的热工水力特性。The positive improvement effect of the present invention is that: the thorium-based molten salt breeder reactor core of the present invention divides the core activity into several types of mixed thermal spectrum and fast spectrum by changing the volume ratio of molten salt and graphite in the graphite moderator cells. By setting the power flattening zone, the graphite replacement cycle can be extended to 10 years, so that the reactor has a negative temperature reactivity coefficient; by setting the axial breeding zone, the reactor can be further improved The breeding performance is beneficial to the thermal-hydraulic properties of the reactor.
附图说明Description of drawings
图1为本发明的实施例1的堆芯的截面结构示意图。FIG. 1 is a schematic cross-sectional structure diagram of a core according to Embodiment 1 of the present invention.
图2为本发明的实施例1的堆芯的侧视结构示意图。FIG. 2 is a schematic side view of the structure of the core according to Embodiment 1 of the present invention.
图3为本发明的实施例1的一种慢化剂栅元的截面结构示意图。3 is a schematic cross-sectional structure diagram of a moderator cell according to Embodiment 1 of the present invention.
图4为本发明的实施例1的另一种慢化剂栅元的截面结构示意图。4 is a schematic cross-sectional structure diagram of another moderator cell according to Embodiment 1 of the present invention.
图5为本发明的实施例1的慢化剂栅元组合后的立体结构示意图。FIG. 5 is a schematic three-dimensional structure diagram of the moderator cells combined according to Embodiment 1 of the present invention.
图6为本发明的实施例1的板型石墨棱柱的结构示意图。FIG. 6 is a schematic structural diagram of the plate-type graphite prism in Example 1 of the present invention.
图7为本发明的实施例1的堆芯的横截面与中子能量关系示意图。FIG. 7 is a schematic diagram showing the relationship between the cross section of the core and the neutron energy according to Embodiment 1 of the present invention.
图8为本发明的实施例1的慢化剂栅元的侧视结构示意图。FIG. 8 is a schematic side view of the structure of the moderator cell according to Embodiment 1 of the present invention.
图9为本发明的实施例2的堆芯的截面结构示意图。FIG. 9 is a schematic cross-sectional structure diagram of the core according to Embodiment 2 of the present invention.
图10为本发明的实施例3的堆芯的截面结构示意图。FIG. 10 is a schematic cross-sectional structure diagram of the core according to Embodiment 3 of the present invention.
图11为本发明的实施例4的堆芯的截面结构示意图。FIG. 11 is a schematic cross-sectional structure diagram of the core according to Embodiment 4 of the present invention.
图12为本发明的实施例1-8的反应堆系统的结构示意图。FIG. 12 is a schematic structural diagram of the reactor system of Embodiments 1-8 of the present invention.
附图标记说明:Description of reference numbers:
活性区 1Active Zone 1
增殖区 11Proliferation Zone 11
第一功率展平区 12First Power Flattening Zone 12
第二功率展平区 13Second Power Flattening Zone 13
中子提供区 14Neutron supply area 14
反射层 2Reflector 2
径向反射层 21Radial Reflector 21
轴向反射层 22Axial Reflector 22
上反射层 23upper reflective layer 23
下反射层 24lower reflective layer 24
燃料孔道 3fuel port 3
鳍 4Fin 4
慢化剂栅元头 51Moderator Cell Head 51
慢化剂栅元末端 52Moderator Cell End 52
反应堆 61Reactor 61
主泵 62main pump 62
主换热器 63Main Heat Exchanger 63
后处理系统 64Aftertreatment System 64
具体实施方式Detailed ways
下面通过实施例的方式进一步说明本发明,但并不因此将本发明限制在的实施例范围之中。The present invention is further described below by means of examples, but the present invention is not limited to the scope of the examples.
实施例1Example 1
本实施例的高功率混合能谱钍基熔盐增殖堆堆芯,如图1所示,包括活性区1和反射层2,反射层2包覆活性区1,活性区1包括中子提供区14和增殖区11,中子提供区14的中子能谱峰值为小于10-6MeV,增殖区11的中子能谱峰值为10-6MeV~10-3MeV。The high-power hybrid energy spectrum thorium-based molten salt breeder reactor core of this embodiment, as shown in FIG. 1 , includes an active region 1 and a reflective layer 2 , the reflective layer 2 coats the active region 1, and the active region 1 includes a neutron supply region 14 and the breeding area 11, the neutron energy spectrum peak of the neutron providing area 14 is less than 10 -6 MeV, and the neutron energy spectrum peak of the breeding area 11 is 10 -6 MeV~10 -3 MeV.
如图2所示,反射层2在活性区1外围和上、下两端。反射层2也可分为径向反射层21和轴向反射层22。径向反射层21围绕在活性区1外围。轴向反射层22分为上反射层23和下反射层24,上反射层23位于活性区1正上方,呈圆台状,下反射层24位于活性区1正下方,也呈圆台状。反射层2在不影响中子经济性的前提下节约石墨用料,并减轻了石墨反射层的正温度反应性效应。As shown in FIG. 2 , the reflective layer 2 is at the periphery of the active region 1 and at the upper and lower ends. The reflection layer 2 can also be divided into a radial reflection layer 21 and an axial reflection layer 22 . The radial reflection layer 21 surrounds the periphery of the active region 1 . The axial reflection layer 22 is divided into an upper reflection layer 23 and a lower reflection layer 24. The upper reflection layer 23 is located directly above the active area 1 and is in the shape of a truncated cone. The reflective layer 2 saves graphite materials on the premise of not affecting the neutron economy, and reduces the positive temperature reactivity effect of the graphite reflective layer.
设计采用LiF-BeF2-(Th+U)F4熔盐作为裂变燃料和转换燃料的载体盐,采用石墨作为慢化剂和反射层。堆芯包括活性区1和反射层2,活性区1是由石墨慢化剂栅元和流经其中的燃料熔盐组成,石墨慢化剂栅元的设计可通过改变几个关键几何尺寸来灵活调节熔盐、石墨体积比,将堆芯分为具有热中子谱(能谱峰值位于能量小于10-6MeV的区域)的中子提供区14及具有超热中子谱(能谱峰值位于10-6MeV~10-3MeV能区)的增殖区11。The design uses LiF-BeF 2 -(Th+U)F 4 molten salt as the carrier salt for fission fuel and conversion fuel, and graphite as the moderator and reflector. The core includes an active area 1 and a reflective layer 2. The active area 1 is composed of a graphite moderator cell and a fuel molten salt flowing through it. The design of the graphite moderator cell can be flexibly changed by changing several key geometric dimensions. By adjusting the volume ratio of molten salt and graphite, the core is divided into a neutron providing region 14 with a thermal neutron spectrum (the peak of the energy spectrum is located in a region with energy less than 10 -6 MeV) and a neutron supply region 14 with an epithermal neutron spectrum (the peak of the energy spectrum is located at 10 -6 MeV ~ 10 -3 MeV energy region) proliferation zone 11.
如图3所示,慢化剂栅元可以是石墨六棱柱,中间具有燃料孔道3供燃料熔盐流经并冷却石墨慢化剂,其不相邻的三个侧面上有鳍4,用以形成栅元之间的缝隙供燃料熔盐流通并冷却石墨慢化剂。栅元呈正三角形状排布。如图4所示,慢化剂栅元也可以是正四边形石墨棱柱,中间具有燃料孔道3供燃料熔盐流经并冷却石墨慢化剂,其四个侧边为鳍4,用以形成栅元之间的缝隙供燃料熔盐流通并冷却石墨慢化剂,其中栅元呈正四边形排布。如图5和图6所示,慢化剂栅元也可以是板型石墨棱柱,板上有鳍4,用以形成栅元之间的缝隙供燃料熔盐流通并冷却石墨慢化剂。栅元可呈正六边形状或四边形状排布。As shown in FIG. 3 , the moderator cell can be a graphite hexagonal prism, with a fuel channel 3 in the middle for the molten salt of fuel to flow through and cool the graphite moderator, and fins 4 are arranged on three non-adjacent sides thereof for the purpose of The gaps between the cells are formed for the fuel molten salt to flow and to cool the graphite moderator. The cells are arranged in an equilateral triangle shape. As shown in FIG. 4 , the moderator cell can also be a regular quadrilateral graphite prism, with a fuel channel 3 in the middle for the molten salt to flow through and cool the graphite moderator, and its four sides are fins 4 to form the cell The gaps between are for the fuel molten salt to circulate and cool the graphite moderator, and the cells are arranged in a regular quadrilateral. As shown in FIGS. 5 and 6 , the moderator cells can also be plate-type graphite prisms with fins 4 on the plate to form gaps between the cells for the fuel molten salt to flow and cool the graphite moderator. The cells can be arranged in a regular hexagonal shape or a quadrilateral shape.
如图7所示,根据U233裂变截面以及Th232俘获截面对比显示,有益于增殖的中子能谱(能谱峰值位于10-5MeV~10-3MeV能区,即共振区)要较有益于裂变的中子能谱(能谱峰值位于能量小于10-6MeV的区域,即热能区)硬,所以增殖区11的燃料和石墨的体积比(1:3.2~1:1.8)大于中子提供区14的燃料和石墨的体积比(1:7.2~1:3.2),并且,为有效利用中子提供区14产生的中子,将中子提供区14置于活性区1内部,增殖区11置于活性区1外围。在本实施例中,增殖区11的燃料和石墨的体积比为1:2.8,中子提供区14的燃料和石墨的体积比为1:6。As shown in Figure 7, according to the comparison of U233 fission cross section and Th232 capture cross section, the neutron energy spectrum that is beneficial to proliferation (the energy spectrum peak is located in the energy region of 10 -5 MeV ~ 10 -3 MeV, that is, the resonance region) is more beneficial to The neutron energy spectrum of fission (the energy spectrum peak is located in the region with energy less than 10 -6 MeV, that is, the thermal energy region) is hard, so the volume ratio (1:3.2~1:1.8) of fuel and graphite in the breeding region 11 is greater than that provided by neutrons The volume ratio of fuel and graphite in the zone 14 (1:7.2 to 1:3.2), and, in order to effectively utilize the neutrons generated by the neutron-providing zone 14, the neutron-providing zone 14 is placed inside the active zone 1, and the breeding zone 11 Placed on the periphery of active area 1. In this embodiment, the volume ratio of fuel and graphite in the breeding zone 11 is 1:2.8, and the volume ratio of fuel and graphite in the neutron providing zone 14 is 1:6.
增殖区11还可进一步分为径向增殖区(图中未示出)和轴向增殖区(图中未示出),将中子提供区14包裹在内,以提供中子经济性。径向增殖区具有石墨六棱柱栅元的燃料孔径和侧面鳍4。轴向增殖区是由石墨慢化剂栅元的轴向几何结构形成,如图8所示,石墨慢化剂栅元包括慢化剂栅元头51和慢化剂栅元末端52,栅元两端棒头横截面明显较中段横截面小,燃料石墨体积比大,有益于增殖。The breeding zone 11 can be further divided into a radial breeding zone (not shown in the figure) and an axial breeding zone (not shown in the figure), which wraps the neutron supplying zone 14 in order to provide neutron economy. The radial breeder region has fuel apertures and side fins 4 of graphite hexagonal cells. The axial breeder zone is formed by the axial geometry of the graphite moderator cell. As shown in FIG. 8, the graphite moderator cell includes a moderator cell head 51 and a moderator cell end 52. The cross section of the rod head at both ends is obviously smaller than that of the middle section, and the fuel-to-graphite volume ratio is large, which is beneficial to proliferation.
采用蒙卡软件MCNP进行反应堆建模,并选定其中可灵活改变的燃料孔径或栅元板厚度以及鳍4的横截面圆直径作为优化参数,通过改变慢化剂栅元的燃料孔径或栅元板的厚度,以及鳍4的横截面圆直径,可以调节燃料和石墨的体积比,使得活性区1局部区域的能谱有所不同。而根据Th的中子俘获截面以及U的裂变截面随中子能量变化的情况,优选出合适的燃料和石墨体积比,以分别得到有益于增殖和裂变的能谱,从而将活性区1进行中子提供区14和增殖区11的划分。中子提供区14和增殖区11均大体排列成圆形。根据计算得到的有效增殖系数、增殖比以及温度反应性系数进行优化,优选出合适的中子提供区14和增殖区11的等效直径。本实施例给出的堆芯热功率为2250MW。The MCNP is used to model the reactor, and the flexibly changeable fuel aperture or cell plate thickness and the cross-sectional circle diameter of the fin 4 are selected as optimization parameters. By changing the fuel aperture or cell of the moderator cell The thickness of the plate, as well as the cross-sectional circular diameter of the fins 4, can adjust the volume ratio of fuel and graphite, so that the energy spectrum of the local area of the active zone 1 is different. According to the change of the neutron capture cross section of Th and the fission cross section of U with neutron energy, an appropriate volume ratio of fuel and graphite is optimized to obtain energy spectra that are beneficial to breeding and fission, respectively. The sub-providing area 14 and the division of the proliferation area 11. Both the neutron supplying region 14 and the propagation region 11 are arranged in a substantially circular shape. According to the calculated effective reproduction coefficient, reproduction ratio and temperature reactivity coefficient, the appropriate diameters of the neutron supplying area 14 and the reproduction area 11 are optimized. The core thermal power given in this embodiment is 2250MW.
在本实施例中,模拟计算得到的堆芯的增殖比提高到1.085。In this embodiment, the breeding ratio of the core calculated by simulation is increased to 1.085.
实施例2Example 2
实施例2的结构与实施例1基本相同,不同之处在于,如图9所示,实施例2的活性区1中加入了第一功率展平区12。第一功率展平区12包围中子提供区14,增殖区11包围第一功率展平区12,第一功率展平区12的中子能谱峰值大于10-3MeV,具有快中子谱。第一功率展平区12能够展平堆芯功率分布和优化温度反应性系数,第一功率展平区12设置在堆芯中央或在中子提供区14和增殖区11之间,中子能谱为快谱(能谱峰值位于能量大于10-3MeV的区域、燃料石墨体积比1:1.8~1:0.01)。控制棒放置在功率展平区内。The structure of Embodiment 2 is basically the same as that of Embodiment 1, except that, as shown in FIG. 9 , a first power flattening area 12 is added to the active area 1 of Embodiment 2. The first power flattening region 12 surrounds the neutron providing region 14, the breeding region 11 surrounds the first power flattening region 12, and the neutron energy spectrum peak of the first power flattening region 12 is greater than 10-3 MeV and has a fast neutron spectrum . The first power flattening region 12 can flatten the core power distribution and optimize the temperature reactivity coefficient. The first power flattening region 12 is arranged in the center of the core or between the neutron providing region 14 and the breeding region 11. The neutron energy The spectrum is a fast spectrum (the peak of the energy spectrum is located in the region where the energy is greater than 10 -3 MeV, and the volume ratio of fuel to graphite is 1:1.8~1:0.01). The control rods are placed in the power flattening area.
在本实施例中,根据计算机模拟结果,增殖比提高到了1.09,石墨的更换周期延长到10年,使得反应堆具有负的温度反应性系数。In this embodiment, according to the computer simulation results, the breeding ratio is increased to 1.09, and the replacement period of graphite is extended to 10 years, so that the reactor has a negative temperature reactivity coefficient.
实施例3Example 3
实施例3的结构与实施例2基本相同,不同之处在于,如图10所示,活性区1还包括第一功率展平区12和第二功率展平区13,第一功率展平区12的燃料熔盐和石墨的体积比为1:1,第二功率展平区13为燃料熔盐,增殖区11临接并围绕第一功率展平区12,第一功率展平区12临接并围绕中子提供区14,中子提供区14临接并围绕第二功率展平区13,第二功率展平区13位于活性区1的中央。根据计算机模拟结果,通过第一功率展平区12和第二功率展平区13的配合作用,将增殖比提高到1.1,进一步优化了温度反应性系数,使得温度反应性系数为负,保证了反应堆的安全,延长石墨更换周期。The structure of Embodiment 3 is basically the same as that of Embodiment 2, except that, as shown in FIG. 10 , the active region 1 further includes a first power flattening region 12 and a second power flattening region 13 . The first power flattening region The volume ratio of fuel molten salt and graphite in 12 is 1:1, the second power flattening area 13 is fuel molten salt, the breeding area 11 is adjacent to and surrounds the first power flattening area 12, and the first power flattening area 12 is adjacent to the first power flattening area 12. The neutron providing region 14 is adjacent to and surrounds the neutron providing region 14 , which is adjacent to and surrounds the second power flattening region 13 , which is located in the center of the active region 1 . According to the computer simulation results, through the cooperation of the first power flattening region 12 and the second power flattening region 13, the breeding ratio is increased to 1.1, and the temperature reactivity coefficient is further optimized, so that the temperature reactivity coefficient is negative, ensuring that the temperature reactivity coefficient is negative. Reactor safety, extended graphite replacement cycle.
实施例4Example 4
实施例4的结构与实施例2基本相同,不同之处在于,如图11所示,活性区1还包括第一功率展平区12和第二功率展平区13,第一功率展平区12的燃料熔盐和石墨的体积比为1:1,第二功率展平区13为燃料熔盐,增殖区11临接并围绕第一功率展平区12,第一功率展平区12临接并围绕第二功率展平区13,第二功率展平区13临接并围绕中子提供区14,中子提供区14位于活性区1的中央。根据计算机模拟结果,通过将第一功率展平区12和第二功率展平区13层叠设置,将增殖比提高到1.1,进一步优化了温度反应性系数,并使得温度反应性系数为负,保证了反应堆的安全,延长石墨更换周期。The structure of Embodiment 4 is basically the same as that of Embodiment 2, the difference is that, as shown in FIG. 11 , the active region 1 further includes a first power flattening region 12 and a second power flattening region 13 . The first power flattening region The volume ratio of fuel molten salt and graphite in 12 is 1:1, the second power flattening area 13 is fuel molten salt, the breeding area 11 is adjacent to and surrounds the first power flattening area 12, and the first power flattening area 12 is adjacent to the first power flattening area 12. The second power flattening region 13 is adjacent to and surrounds the neutron supplying region 14 , and the neutron supplying region 14 is located in the center of the active region 1 . According to the computer simulation results, by stacking the first power flattening region 12 and the second power flattening region 13 to increase the breeding ratio to 1.1, the temperature reactivity coefficient is further optimized, and the temperature reactivity coefficient is made negative, ensuring that the The safety of the reactor is improved and the graphite replacement cycle is extended.
实施例5-8Examples 5-8
实施例5-8与实施例1基本相同,不同之处在于,增殖区11的燃料和石墨的体积比,以及中子提供区14的燃料和石墨的体积比均有所不同。Examples 5-8 are basically the same as Example 1, except that the volume ratio of fuel and graphite in the breeding zone 11 and the volume ratio of fuel and graphite in the neutron providing zone 14 are different.
实施例5-8的计算机模拟结果如表1中所示:The computer simulation results of Examples 5-8 are shown in Table 1:
表1:实施例5-8的计算机模拟结果Table 1: Computer Simulation Results of Examples 5-8
对比例1-4Comparative Examples 1-4
对比例1-4与实施例1基本相同,不同之处在于,增殖区11的燃料和石墨的体积比,以及中子提供区14的燃料和石墨的体积比均有所不同。对比例1-4的计算机模拟结果如表2中所示:Comparative Examples 1-4 are basically the same as Example 1, except that the volume ratio of fuel and graphite in the breeding zone 11 and the volume ratio of fuel and graphite in the neutron providing zone 14 are different. The computer simulation results of Comparative Examples 1-4 are shown in Table 2:
表2:对比例1-4的计算机模拟结果Table 2: Computer Simulation Results of Comparative Examples 1-4
在表2中,转换比是指反应堆61内产生的易裂变材料量和消耗的易裂变材料量之比,当该比值大于1时,称为增殖比。不临界是指反应堆的中子的产生率和消失率之间不再平衡,使链式反应不能持续地进行下去的状态。In Table 2, the conversion ratio refers to the ratio between the amount of fissile material produced and the amount of fissile material consumed in the reactor 61, and when the ratio is greater than 1, it is called the breeding ratio. Non-criticality refers to the state in which the neutron generation rate and disappearance rate of the reactor are no longer balanced, so that the chain reaction cannot continue.
如图12所示,本发明的高功率混合能谱钍基熔盐增殖堆堆芯设置于反应堆61中,反应堆61中的裂变热通过熔盐-熔盐主换热器63带至三回路的热电转化系统(常规岛)。此外,通过一支熔盐旁路,对燃料盐进行在线后处理,主要为去除裂变产物中的中子毒物,提高堆芯的增殖比。受反应堆61加热的热水到达主泵62,由主泵62输送到主热换器,然后到达后处理系统64。As shown in FIG. 12 , the core of the high-power hybrid energy spectrum thorium-based molten salt breeder reactor of the present invention is arranged in the reactor 61 , and the fission heat in the reactor 61 is brought to the three-circuit heat exchanger 63 through the molten salt-molten salt main heat exchanger 63 . Thermoelectric conversion system (conventional island). In addition, the on-line post-processing of the fuel salt is carried out through a molten salt bypass, mainly to remove the neutron poison in the fission products and improve the breeding ratio of the core. The hot water heated by the reactor 61 reaches the main pump 62 , where it is delivered to the main heat exchanger, and then to the aftertreatment system 64 .
本实施例的高功率混合能谱钍基熔盐增殖堆堆芯通过改变石墨慢化剂栅元的熔盐、石墨体积比,将堆芯活性区分为混合有热谱和快谱的若干区,将堆芯的增殖比提高到1.08以上;通过设置功率展平区,延长石墨的更换周期至10年,使得反应堆具有负的温度反应性系数;通过设置轴向增殖区,可进一步提高堆的增殖性能,同时有利于堆的热工水力特性。In the high-power mixed-energy-spectrum thorium-based molten salt breeder reactor core of this embodiment, by changing the volume ratio of molten salt and graphite in the graphite moderator cells, the active zone of the core is divided into several zones with a mixture of thermal spectrum and fast spectrum, Increase the breeding ratio of the core to more than 1.08; extend the graphite replacement cycle to 10 years by setting the power flattening zone, so that the reactor has a negative temperature reactivity coefficient; by setting the axial breeding zone, the breeding of the reactor can be further improved. performance, while contributing to the thermal-hydraulic properties of the reactor.
虽然以上描述了本发明的具体实施方式,但是本领域的技术人员应当理解,这仅是举例说明,本发明的保护范围是由所附权利要求书限定的。本领域的技术人员在不背离本发明的原理和实质的前提下,可以对这些实施方式做出多种变更或修改,但这些变更和修改均落入本发明的保护范围。Although the specific embodiments of the present invention are described above, those skilled in the art should understand that this is only an illustration, and the protection scope of the present invention is defined by the appended claims. Those skilled in the art can make various changes or modifications to these embodiments without departing from the principle and essence of the present invention, but these changes and modifications all fall within the protection scope of the present invention.
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