CN106873025A - A kind of radon harvester and method - Google Patents

A kind of radon harvester and method Download PDF

Info

Publication number
CN106873025A
CN106873025A CN201710229067.6A CN201710229067A CN106873025A CN 106873025 A CN106873025 A CN 106873025A CN 201710229067 A CN201710229067 A CN 201710229067A CN 106873025 A CN106873025 A CN 106873025A
Authority
CN
China
Prior art keywords
collecting cassette
radon
harvester
seal box
activated carbon
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Pending
Application number
CN201710229067.6A
Other languages
Chinese (zh)
Inventor
李承文
乐仁昌
何志杰
陈林
孟祥贺
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
Fujian Normal University
Original Assignee
Fujian Normal University
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Fujian Normal University filed Critical Fujian Normal University
Priority to CN201710229067.6A priority Critical patent/CN106873025A/en
Publication of CN106873025A publication Critical patent/CN106873025A/en
Pending legal-status Critical Current

Links

Classifications

    • GPHYSICS
    • G01MEASURING; TESTING
    • G01TMEASUREMENT OF NUCLEAR OR X-RADIATION
    • G01T7/00Details of radiation-measuring instruments
    • G01T7/02Collecting means for receiving or storing samples to be investigated and possibly directly transporting the samples to the measuring arrangement; particularly for investigating radioactive fluids
    • GPHYSICS
    • G01MEASURING; TESTING
    • G01TMEASUREMENT OF NUCLEAR OR X-RADIATION
    • G01T1/00Measuring X-radiation, gamma radiation, corpuscular radiation, or cosmic radiation
    • G01T1/36Measuring spectral distribution of X-rays or of nuclear radiation spectrometry

Landscapes

  • Physics & Mathematics (AREA)
  • Spectroscopy & Molecular Physics (AREA)
  • Health & Medical Sciences (AREA)
  • Life Sciences & Earth Sciences (AREA)
  • General Physics & Mathematics (AREA)
  • High Energy & Nuclear Physics (AREA)
  • Molecular Biology (AREA)
  • Chemical & Material Sciences (AREA)
  • Analytical Chemistry (AREA)
  • Measurement Of Radiation (AREA)
  • Sampling And Sample Adjustment (AREA)

Abstract

The invention discloses a kind of radon harvester and method, described device includes collecting cassette, collection frame and seal box, the collecting cassette is cylindric collecting cassette, two axial ends of cylindric collecting cassette are molded by filter screen, activated carbon is filled with cylindric collecting cassette, the mesh aperture of the filter screen is less than activated carbon particle size, the collection frame includes trapezoidal base, the short side of trapezoidal base is connected with for the collecting cassette to be embedded in into interior accepting rack, the seal box is interior for the collecting cassette in non-sampled state to be sealed in, seal box includes box body and lid, box body and lid form confined space after being connected through a screw thread.Harvester of the present invention can realize that collecting cassette carries out two-sided collection, collecting cassette thickness is suitable, outer layer activated carbon can be ignored to the screen effect of internal layer active carbon adsorption radon ability, enable to whole activated carbon layer equably to adsorb radon, improve the degree of accuracy of measurement result.

Description

A kind of radon harvester and method
Technical field
Radon technical field is surveyed the invention belongs to air, and in particular to a kind of radon harvester and method.
Background technology
Radon gas is a kind of tracer, and it can indicate subterranean deposit, geological structure, earthquake etc., therefore radon survey is wide It is general to be applied to the aspects such as mineral product geology, hydrogeology, engineering geology, disaster geology, environmental geology.The radioactivity of radon gas is to human body Health be harmful, before the more than ten years, EPA(EPA)《NATURE》It is open on magazine to point out:Radon is to be related to public affairs The popular problem of common health;Radon gas is present in the main construction and decoration such as soil, brick, cement, granite as natural radiation thing In material, it is considered to be only second to the second largest carcinogenic factor of smoking, be classified as radon make one carcinogenic 19 by the World Health Organization Plant one of topmost material.
Activated carbon is a kind of porous carbonaceous material, its flourishing microporous structure and huge specific surface area, makes it to being permitted Many kinds of substance has stronger adsorption capacity, and is used widely in many fields such as purification of air, waste water treatment.Due to work Property charcoal there is very strong adsorption capacity to radon, the activated carbon to having adsorbed radon gas carries out γ measurements, where can calculating activated carbon The radon consistence of environment, at present, activated carbon gamma spectrum survey radon method because its is cheap, measurement sensitivity is high, it is simple to operate the features such as Main flow surveys one of radon method in having become current environment air.
Traditional survey radon activated charcoal only has one side and air contact, and collecting efficiency is not high and thick to spend up to 3~5cm, top layer Activated carbon the shielded effect of bottom active carbon adsorption radon can not be ignored, when the sampling period is shorter, top layer activated carbon inhale Attached radon amount adsorbs radon amount more than bottom, and whole the uneven of active carbon layer radon absorption can make active carbon adsorption radon amount and Radon Deviation of concentration linear relationship, makes measurement result there is larger error.And during detector measurement, the less bottom of absorption radon amount close to Probe causes that detection efficient is relatively low.
The content of the invention
It is high it is an object of the invention to provide a kind of adsorption efficiency, the accurate radon harvester of measurement result and method.
To achieve these goals, the present invention uses following technical scheme:
A kind of radon harvester, it includes collecting cassette, collection frame and seal box, and the collecting cassette is cylindric collecting cassette, circle Two axial ends of column collecting cassette are molded by filter screen, and activated carbon, the mesh hole of the filter screen are filled with cylindric collecting cassette Footpath is less than activated carbon particle size, and the collection frame includes trapezoidal base, and the short side of trapezoidal base is connected with for by the collecting cassette Interior accepting rack is embedded in, the seal box is interior for the collecting cassette in non-sampled state to be sealed in, and seal box includes box Body and lid, box body and lid form confined space after being connected through a screw thread.
Further, it is described collection frame by toughness material be molded, the toughness material can for plastics or other.
The trapezoidal base and accepting rack of the collection frame are integrally formed.
The accepting rack is the circular frame matched with collection box shaped, size.
Further, the cylindric side of the collecting cassette is molded by aluminum material.
Further, two a diameter of 45~60mm of axial end of the collecting cassette, collecting cassette thickness is 7~9mm.
Preferably, the collecting cassette thickness is 7.5mm.
The seal box is molded by ferrous material, and the box body cross section and lid cross section of seal box are circle, its It is big neglect collecting cassette size depending on.
Method present invention also offers radon collection is carried out using the radon harvester, it is specific as follows:
1)Collecting cassette is taken out from seal box and is placed in baking oven, 5-6h is heated under the conditions of 120-130 DEG C, with except deactivation Radon gas and moisture in charcoal;
2)By in the accepting rack of collecting cassette insertion collection frame, then collection frame is put into the closed container equipped with uranium ore, most Closed container is put into during temperature has been set to 25 DEG C of baking boxs of constant temperature afterwards, starts the collection of radon, acquisition time is 2h;
3)After collection terminates, closed container is opened, collection frame is taken out, then collecting cassette is taken out and put back to close from accepting rack Jacket interior sealing;
4)Above-mentioned collecting cassette, up to after 3h, is put in BH1936 Low background multiple tracks gamma energy spectrometers by collecting cassette time of repose in the seal box Probe on, the either axial end face of the collecting cassette is carried out into activated carbon γ measurements close to probe, time of measuring is 300s, obtain Total γ is counted(Absorption is counted);
5)The total γ of background for measuring BH1936 Low background multiple tracks gamma energy spectrometers is counted, and time of measuring is 300s,;
6)By above-mentioned steps 4)The total γ for obtaining counts deduction step 5)The total γ of background of acquisition is counted, and obtains total γ net counts.
The present invention uses above technical scheme, during sampling, collecting cassette is embedded in the accepting rack of collection frame, the two of collecting cassette Individual axial end all with air contact, can realize two-sided collection, and traditional survey radon activated charcoal only has one side and air contact, The activated carbon of top layer has shielding action to bottom active carbon adsorption radon, especially when the sampling period is shorter, top layer activated carbon Absorption radon amount adsorbs radon amount more than bottom, and the uneven of whole active carbon layer radon absorption can make active carbon adsorption radon amount and air Radon consistence deviates linear relationship, measurement result is there is larger error.Radon harvester of the invention, its collection frame includes trapezoidal Base, the short side of trapezoidal base is connected with accepting rack, when carrying out radon collection, by the accepting rack of collecting cassette insertion collection frame, adopts Collect two axial ends of box all with air contact, the radon absorption of whole active carbon layer is more uniform, overcomes traditional survey radon collection Box active carbon layer adsorbs uneven defect so that measurement result is more accurate.Additionally, the present invention is also carried out to the thickness of collecting cassette Optimum choice, it is determined that optimal active carbon layer thickness, it is described to adopt when carrying out radon using radon harvester of the invention and gathering Collection box carries out two-sided collection, increased the contact area with air, and thickness is suitable, and outer layer activated carbon is to internal layer active carbon adsorption radon The screen effect of ability can be ignored, and enable to whole activated carbon layer equably to adsorb radon, and be placed in Low background γ radiation energies There is good gamma-ray detection efficiency on the probe of spectrometer, the sampling period more than 50% is shortened while improving accuracy of measurement.
Brief description of the drawings
Fig. 1 is the schematic diagram of radon harvester sample states of the present invention;
Fig. 2 is the collecting cassette schematic diagram of radon harvester of the present invention;
Fig. 3 is the seal box schematic diagram of radon harvester of the present invention;
Fig. 4 is the collecting cassette thickness and total net relation curve of γ net counts of radon harvester of the present invention.
Specific embodiment
Below in conjunction with the accompanying drawings and embodiment the present invention will be further described.
Embodiment 1
As shown in one of Fig. 1-3, radon harvester of the invention, it includes collecting cassette 1, collection frame 2 and seal box 3, described Collecting cassette 1 is cylindric collecting cassette, and two axial ends of cylindric collecting cassette are molded by filter screen 11, filling in cylindric collecting cassette Active charcoal 4, the mesh aperture of the filter screen 11 is less than activated carbon particle size 4, and the collection frame 2 includes trapezoidal base 21, trapezoidal The short side of base 21 is connected with for the collecting cassette 1 to be embedded in into interior accepting rack 22, and the seal box 3 is used for will be in non- In the collecting cassette 1 of sample states is sealed in, seal box 3 includes box body 32 and lid 31, and box body 32 and lid 31 are connected by screw thread Confined space is formed after connecing.
The collection frame 2 is molded by the good material of plastics or other toughness, gathers the trapezoidal base 21 and accepting rack of frame 2 22 are integrally formed, and the accepting rack 22 is the circular frame matched with the shape of collecting cassette 1, size.
The cylindric side 12 of the collecting cassette 1 is molded by aluminum material.Two axial ends of the collecting cassette 1 are a diameter of 45~60mm, the thickness of collecting cassette 1 is 7~9mm, and optimum thickness is 7.5mm.
The seal box 3 is molded by ferrous material, and the cross section of box body 32 and the cross section of lid 31 of seal box 3 are circle Shape, it is neglected greatly depending on collecting cassette size.
Embodiment 2
The thickness selection of collecting cassette
Axial end diameter is consistent, and the different collecting cassette sample of thickness is keeping carrying out radon simultaneously in the case that other conditions are consistent Collection experiment, step is as follows:
1)Collecting cassette is taken out from seal box and is placed in baking oven, 5-6h is heated under the conditions of 120-130 DEG C, with except deactivation Radon gas and moisture in charcoal;
2)By in the accepting rack of collecting cassette insertion collection frame, then collection frame is put into the closed container equipped with uranium ore, most Closed container is put into during temperature has been set to 25 DEG C of baking boxs of constant temperature afterwards, starts the collection of radon, acquisition time is 2h;
3)After collection terminates, closed container is opened, collection frame is taken out, then collecting cassette is taken out and put back to close from accepting rack Jacket interior sealing;
4)Above-mentioned collecting cassette, up to after 3h, is put in BH1936 Low background multiple tracks gamma energy spectrometers by collecting cassette time of repose in the seal box Probe on, the either axial end face of the collecting cassette is carried out into activated carbon γ measurements close to probe, time of measuring is 300s, obtain Total γ is counted(Absorption is counted);
5)The total γ of background for measuring BH1936 Low background multiple tracks gamma energy spectrometers is counted, and time of measuring is 300s,;
6)By above-mentioned steps 4)The total γ for obtaining counts deduction step 5)The total γ of background of acquisition is counted, and obtains total γ net counts.
Experimental result is as shown in table 1:
Total γ of the collecting cassette of table 1 absorption radon experiment is counted
Thickness(mm) 5 7.5 10 12.5 15 17.5 20 25 30 35
The total γ of background is counted 1265 1307 1362 1284 1360 1329 1309 1338 1347 1434
Absorption is counted 9508 10271 9787 9577 9616 8883 8904 8500 7716 8060
Total γ net counts 8243 8964 8425 8293 8256 7554 7595 7162 6369 6626
With collecting cassette thickness(mm)It is transverse axis, total γ net counts are the longitudinal axis, the relation curve for obtaining therebetween is as shown in Figure 4. As seen from Figure 4, when collecting cassette thickness is less than 7.5mm, total γ net counts increase with the increase of thickness;When collecting cassette is thick More than after 7.5mm, total γ net counts are reduced degree with the increase of thickness.The above results are illustrated, when collecting cassette thickness is smaller, are increased Plus collecting cassette thickness can effectively increase the adsorbance of radon and then increase total γ net counts;When collecting cassette thickness reach it is a certain Value, being now further added by the thickness of collecting cassette can not effectively increase the adsorbance of radon, because outer layer activated carbon is to internal layer activity The screen effect of charcoal absorption radon can not be ignored so that activated carbon can not sufficiently uniformly adsorb radon;Further, since collecting cassette thickness Increase, gamma-ray detection efficiency reduction of the probe to another axial end of collecting cassette so that total γ net counts are shown as with adopting Collect the increase of box thickness and reduce.In sum, the final thickness for determining collecting cassette of the present invention is 7~9mm, and optimum thickness is 7.5mm。
When carrying out radon collection using radon harvester of the invention, by the accepting rack of collecting cassette insertion collection frame, gather Two axial ends of box all carry out two-sided collection with air contact, the i.e. collecting cassette, increased the contact area with air, whole The radon absorption of individual active carbon layer is more uniform, and collecting cassette thickness is suitable in addition, and outer layer activated carbon is to internal layer active carbon adsorption radon ability Screen effect can ignore, enable to whole activated carbon layer equably to adsorb radon, and be placed in Low background γ radiation spectrometers Probe on have good gamma-ray detection efficiency, it is possible to increase the degree of accuracy of measurement result.

Claims (10)

1. a kind of radon harvester, it is characterised in that:It includes collecting cassette, collection frame and seal box, and the collecting cassette is circle Column collecting cassette, two axial ends of cylindric collecting cassette are molded by filter screen, and activated carbon is filled with cylindric collecting cassette, described The mesh aperture of filter screen is less than activated carbon particle size, and the collection frame includes trapezoidal base, the short side of trapezoidal base be connected with for The collecting cassette is embedded in interior accepting rack, the seal box is interior for the collecting cassette in non-sampled state to be sealed in, Seal box includes that box body and lid, box body and lid form confined space after being connected through a screw thread.
2. a kind of radon harvester according to claim 1, it is characterised in that:The collection frame is molded by toughness material.
3. a kind of radon harvester according to claim 2, it is characterised in that:The toughness material is plastics.
4. a kind of radon harvester according to claim 1, it is characterised in that:The trapezoidal base of the collection frame and storage Frame is integrally formed.
5. a kind of radon harvester according to claim 1, it is characterised in that:The accepting rack be with collection box shaped, The circular frame of size matching.
6. a kind of radon harvester according to claim 1, it is characterised in that:The cylindric side of the collecting cassette is by aluminium Material is molded.
7. according to a kind of radon harvester described in claim 1, it is characterised in that:Two axial ends of the collecting cassette are a diameter of 45~60mm, collecting cassette thickness is 7~9mm.
8. a kind of radon harvester according to claim 7, it is characterised in that:The collecting cassette thickness is 7.5mm.
9. a kind of radon harvester according to claim 1, it is characterised in that:The seal box is molded by ferrous material, The box body cross section and lid cross section of seal box are circle.
10. a kind of radon acquisition method, the method is using one of claim 1-9 described radon harvester, it is characterised in that:Institute State method specific as follows:
1)Collecting cassette is taken out from seal box and is placed in baking oven, 5-6h is heated under the conditions of 120-130 DEG C;
2)By in the accepting rack of collecting cassette insertion collection frame, then collection frame is put into the closed container equipped with uranium ore, most Closed container is put into during temperature has been set to 25 DEG C of baking boxs of constant temperature afterwards, starts the collection of radon, acquisition time is 2h;
3)After collection terminates, closed container is opened, collection frame is taken out, then collecting cassette is taken out and put back to close from accepting rack Jacket interior sealing;
4)Above-mentioned collecting cassette, up to after 3h, is put in BH1936 Low background multiple tracks gamma energy spectrometers by collecting cassette time of repose in the seal box Probe on, the either axial end face of the collecting cassette is carried out into activated carbon γ measurements close to probe, time of measuring is 300s, obtain Total γ is counted;
5)The total γ of background for measuring BH1936 Low background multiple tracks gamma energy spectrometers is counted, and time of measuring is 300s,;
6)By above-mentioned steps 4)The total γ for obtaining counts deduction step 5)The total γ of background of acquisition is counted, and obtains total γ net counts.
CN201710229067.6A 2017-04-10 2017-04-10 A kind of radon harvester and method Pending CN106873025A (en)

Priority Applications (1)

Application Number Priority Date Filing Date Title
CN201710229067.6A CN106873025A (en) 2017-04-10 2017-04-10 A kind of radon harvester and method

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
CN201710229067.6A CN106873025A (en) 2017-04-10 2017-04-10 A kind of radon harvester and method

Publications (1)

Publication Number Publication Date
CN106873025A true CN106873025A (en) 2017-06-20

Family

ID=59161945

Family Applications (1)

Application Number Title Priority Date Filing Date
CN201710229067.6A Pending CN106873025A (en) 2017-04-10 2017-04-10 A kind of radon harvester and method

Country Status (1)

Country Link
CN (1) CN106873025A (en)

Cited By (3)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
CN108519255A (en) * 2018-04-12 2018-09-11 福建拓普检测技术有限公司 A kind of detection method for acquiring radon consistence in soil
CN113539542A (en) * 2021-07-19 2021-10-22 中国人民解放军火箭军工程大学 Radon gas enrichment type alpha-ray nuclear battery
CN107807380B (en) * 2017-12-14 2023-08-11 福建师范大学 Instrument coefficient scale device and method for radon measurement by activated carbon box

Citations (7)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
JPH10258272A (en) * 1997-03-05 1998-09-29 Fuji Denki Ii I C Kk Deodorizing and bacteria removing filter apparatus for hot water of bathtub
CN102043162A (en) * 2010-10-20 2011-05-04 中国人民解放军海军医学研究所 High-efficiency radon-measuring activated carbon box
CN201849227U (en) * 2010-11-10 2011-06-01 佟灿 Multi-purpose combination pen container
CN201935837U (en) * 2010-12-23 2011-08-17 核工业北京地质研究院 Activated carbon absorber for collecting radon gas in soil
CN203920829U (en) * 2014-06-24 2014-11-05 兴化市联发食品有限公司 A kind of with vegetables treatment hole and the dual-purpose conveying device of automanual discharging
CN204126642U (en) * 2014-09-07 2015-01-28 河南理工大学 A kind of colliery radon survey device based on activated carbon box method
CN204770636U (en) * 2015-07-01 2015-11-18 马鞍山市润启新材料科技有限公司 Water a packet shallow

Patent Citations (7)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
JPH10258272A (en) * 1997-03-05 1998-09-29 Fuji Denki Ii I C Kk Deodorizing and bacteria removing filter apparatus for hot water of bathtub
CN102043162A (en) * 2010-10-20 2011-05-04 中国人民解放军海军医学研究所 High-efficiency radon-measuring activated carbon box
CN201849227U (en) * 2010-11-10 2011-06-01 佟灿 Multi-purpose combination pen container
CN201935837U (en) * 2010-12-23 2011-08-17 核工业北京地质研究院 Activated carbon absorber for collecting radon gas in soil
CN203920829U (en) * 2014-06-24 2014-11-05 兴化市联发食品有限公司 A kind of with vegetables treatment hole and the dual-purpose conveying device of automanual discharging
CN204126642U (en) * 2014-09-07 2015-01-28 河南理工大学 A kind of colliery radon survey device based on activated carbon box method
CN204770636U (en) * 2015-07-01 2015-11-18 马鞍山市润启新材料科技有限公司 Water a packet shallow

Non-Patent Citations (2)

* Cited by examiner, † Cited by third party
Title
乐仁昌 等: "氡及其子体水平扩散系数测量研究", 《核技术》 *
江熊主编, 化学工业出版社 *

Cited By (4)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
CN107807380B (en) * 2017-12-14 2023-08-11 福建师范大学 Instrument coefficient scale device and method for radon measurement by activated carbon box
CN108519255A (en) * 2018-04-12 2018-09-11 福建拓普检测技术有限公司 A kind of detection method for acquiring radon consistence in soil
CN113539542A (en) * 2021-07-19 2021-10-22 中国人民解放军火箭军工程大学 Radon gas enrichment type alpha-ray nuclear battery
CN113539542B (en) * 2021-07-19 2024-01-30 中国人民解放军火箭军工程大学 Radon gas enrichment type alpha ray nuclear battery

Similar Documents

Publication Publication Date Title
CN106873025A (en) A kind of radon harvester and method
Hassan et al. Radon migration process and its influence factors; review
Forkapic et al. Correlations between soil characteristics and radioactivity content of Vojvodina soil
CN101609154A (en) Measure the method for precipitation rate of radon
CN102426379A (en) Method for measuring radon emanation rate by adopting two-stage method
Kaur et al. Study of radon/thoron exhalation rate, soil-gas radon concentration, and assessment of indoor radon/thoron concentration in Siwalik Himalayas of Jammu & Kashmir
Harb et al. Radioactivity levels and soil-to-plant transfer factor of natural radionuclides from protectorate area in Aswan, Egypt
CN103760068A (en) Method and device for determining diffusion and reduction processes of nitrous oxide in soil
Ye et al. Simultaneous determination of the radon diffusion coefficient and the free radon production rate from compact porous emanation media
Žunić et al. High natural radiation exposure in radon spa areas: a detailed field investigation in Niška Banja (Balkan region)
De Simone et al. Correcting for H2O interference using a RAD7 electrostatic collection-based silicon detector
CN107229080A (en) A kind of acquisition methods of geochemical well logging neutron absorption gamma spectra
Karadeniz et al. Dynamic equilibrium of radiocesium with stable cesium within the soil–mushroom system in Turkish pine forest
Pressyanov et al. Sorption and desorption of radioactive noble gases in polycarbonates
CN206757053U (en) A kind of radon harvester
Karadeniz et al. Estimation of vertical migration velocity of 137Cs in the Mount IDA/Kazdagi, Turkey
CN106873023B (en) A method of air radon consistence is measured using activated charcoal
Yanchao et al. Study on a new charcoal closed chamber method for measuring radon exhalation rate of building materials
Major Biochar Application to a colombian savanna oxisol: fate and effect on soil fertility, crop production, nutrient leaching and soil hydrology volume I
Al-Saadi et al. Measurement of radon and uranium concentrations in the dates and their seeds of different regions in Karbala governorate
De Simone et al. Using natural radon as a tracer of gasoline contamination
CN203350088U (en) Compact type radon collector
Canoba et al. Radon determination by activated charcoal adsorption and liquid scintillation measurement
Abdalla et al. Radon gas build up using alpha scintillation cell: Experimentally and theoretically
CN102043162B (en) High-efficiency radon-measuring activated carbon box

Legal Events

Date Code Title Description
PB01 Publication
PB01 Publication
SE01 Entry into force of request for substantive examination
SE01 Entry into force of request for substantive examination
RJ01 Rejection of invention patent application after publication

Application publication date: 20170620

RJ01 Rejection of invention patent application after publication