CN105467424A - Plutonium-doped fiber and neutron measuring method thereof - Google Patents

Plutonium-doped fiber and neutron measuring method thereof Download PDF

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Publication number
CN105467424A
CN105467424A CN201410459792.9A CN201410459792A CN105467424A CN 105467424 A CN105467424 A CN 105467424A CN 201410459792 A CN201410459792 A CN 201410459792A CN 105467424 A CN105467424 A CN 105467424A
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China
Prior art keywords
plutonium
neutron
optical fiber
photomultiplier
mix
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Pending
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CN201410459792.9A
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Chinese (zh)
Inventor
刘建忠
王勇
任俊
宋嘉涛
杨明明
李建伟
于潜
赵迎喜
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China Institute for Radiation Protection
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China Institute for Radiation Protection
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Priority to CN201410459792.9A priority Critical patent/CN105467424A/en
Publication of CN105467424A publication Critical patent/CN105467424A/en
Pending legal-status Critical Current

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Abstract

The invention relates to a plutonium-doped fiber and neutron measuring method thereof, and belongs to the field of radiation measurement. The plutonium-doped fiber is placed in the measurement environment, and connected with a photomultiplier, and the photomultiplier is connected with a signal amplification circuit; and incoming neutrons react with plutonium in the fiber, the reaction energy is transmitted to a fiber material and excites the fiber material, photons are released during de-excitation, the photons are transmitted to the photomultiplier via the fiber and converted into electric signals, the electric signals are amplified and recorded by the signal amplification circuit, and the amount of the incoming neutrons is measured according to the principle that the photon amount is proportional to the neutron amount.

Description

A kind of method of mixing plutonium optical fiber and measuring neutron
Technical field
The invention belongs to actinometry field, be specifically related to a kind of method of mixing plutonium optical fiber and measuring neutron.
Background technology
Light transmitting fiber is called for short optical fiber, and to conduct, distance, signal attenuation are little, message capacity is widely used in the communications industry greatly.Optical fiber can not only light conducting signal, under specific condition, also can launch photon, have that structure is simple, volume is little simultaneously, lightweight, lay convenient, with low cost advantage, the therefore attention of also extremely actinometry industry.
Along with the continuous popularization of Application of Nuclear Technology, the place of neutron monitoring is needed to get more and more, when needing the regional compare of monitoring unevenness that is large or radiation field more serious, during as used traditional neutron probe formula area monitoring technology, then need the probe quantity of laying more, will the cost of whole system be made very high, use neutron optical fiber technology to complete same work and then want much cheap, meanwhile, middle sub-optical fibre can also measure the neutron irradiation in narrow region.
The primary structure of optical fiber generally can be divided into fibre core, covering, coat, jacket layer, what wherein play the effect of transmission photon is sandwich layer, its constituent material has quartz, fluoride glass, chalcogenide glass, polymethylmethacrylate (PMMA), polystyrene (PSt), fluorine-containing transparent resin or deuterate PMMA etc., the reaction cross-section of these materials and neutron is all smaller, and therefore general optical fiber can not be directly used in measurement neutron.
Summary of the invention
The object of the invention is to for problems of the prior art, provide a kind of can be used for neutron measurement mix plutonium optical fiber, and use the method for this optical fiber measurement neutron.
Technical scheme of the present invention is as follows: one mixes plutonium optical fiber, comprises fibre core, covering, coat, jacket layer, and wherein, mix the raw material containing plutonium-239 in the material of described fibre core, the incorporation of the raw material containing plutonium-239 accounts for the 10%-15% of fibre core gross mass.
Further, mix plutonium optical fiber as above, wherein, the described raw material containing plutonium-239 can select plutonium dioxide, tri-chlorination plutonium, PuF3 or plutonium hexafluoride, raw material containing plutonium-239 is mixed in core material by corresponding proportion, fully mixes under molten condition.
Above-mentioned method of mixing plutonium optical fiber measurement neutron, plutonium optical fiber will be mixed and be placed in measurement environment, mix plutonium optical fiber to be connected with photomultiplier, photomultiplier connection signal amplifying circuit and pulse recording circuit, plutonium in incident neutron and optical fiber reacts, reaction can pass to fiber optic materials makes it excite, photon is released during de excitation, photon through Optical Fiber Transmission to photomultiplier, to be amplified by signal amplification circuit after converting electric impulse signal to and by pulse recording circuit record, the quantity of electric pulse is the number of times being proportional to neutron and plutonium generation nuclear reaction, also incident neutron quantity is just proportional to, the electric impulse signal amount of record unit time can calculate the fluence of neutron, realize the measurement of neutron fluence.
Beneficial effect of the present invention is as follows: neutron sensitive material plutonium-239 mixes in the core material of optical fiber by the present invention, and the material containing plutonium effectively can measure neutron.The method of this employing optical fiber measurement neutron is cheap, and applied range can measure the neutron irradiation of narrow zone easily.
Accompanying drawing explanation
Fig. 1 is the principle schematic of mixing plutonium optical fiber measurement neutron.
Embodiment
Below in conjunction with drawings and Examples, the present invention is described in detail.
Neutron can with a lot of material generation nuclear reaction, after mixing a certain proportion of neutron sensitive material in optical fiber, incident neutron and its reaction, reaction can pass to fiber optic materials makes it excite, photon is released during de excitation, photon through Optical Fiber Transmission to photomultiplier, convert to electric signal and amplify after by subsequent conditioning circuit record.The energy that photon numbers absorbs to material is directly proportional, and the reaction of nuclear reaction can be certain, and photon numbers is also just proportional to number of neutrons.
239pu fissions under the bombardment of neutron, release the energy of about 170Mev, mainly distribute to two fission fragments, the material therefore containing plutonium effectively can measure neutron, method mixes a certain proportion of plutonium material, and concrete mixed ratio can be determined by experiment.Contain 239the raw material of Pu can select any one of plutonium dioxide, tri-chlorination plutonium, PuF3 or plutonium hexafluoride, or also can consider to adopt two or more composite materials.
The present invention mixes in the fibre core of optical fiber 239pu, utilizes the material containing plutonium effectively can measure neutron.The fission fragment that above-mentioned fission reaction generates can by energy loss in fiber optic materials, core material is made to be in excited state, photon will inevitably be released during de excitation, photon numbers is proportional to the energy of loss, the i.e. quantity of fission reaction, also incident neutron number is just proportional to, thus the measurement of the neutron fluence realized, be multiplied by fluence-dose conversion coefficient and can obtain the Radiation Protection Quantities such as neutron DE.
The number of pulses that neutron is finally formed with mix the ratio of plutonium, photomultiplier model is relevant with photomultiplier duty, when mixing plutonium ratio-dependent, photomultiplier model is when determining to complete with photomultiplier circuit design, can with the method analog computation of Monte Carlo and the method verified by experiment obtain.
Plutonium is mixed in core material, weakening of core light transmissibility will inevitably be caused, but the object of the invention is neutron measurement, general application scenario can not be greater than the length of tens of meters, less demanding to the light transmissibility of optical fiber, as long as therefore the ratio of plutonium is controlled just can meet request for utilization in the reasonable scope.
The incorporation of the raw material containing plutonium-239 accounts for the 10%-15% of fibre core gross mass, and this concentration range both can ensure that in optical fiber measurement, the period of the day from 11 p.m. to 1 a.m had good detection efficiency, and optical fiber also can be made to also have certain light conductive performance.First mixed the optical fiber of plutonium ratio by small-scale production difference, as in core material 239puO 2content is 10%, 11% ..., 15%, through experiment choose the highest plutonium ratio of mixing of detection efficiency as the optimal proportion produced from now on.
Embodiment
Mix plutonium optical fiber and comprise fibre core, covering, coat, jacket layer, concrete preparation method is will 239puO 2raw material (the mainly SiO producing preform is incorporated into by corresponding proportion 2) in, be heated to molten condition, fully make preform after mixing, the production technologies such as follow-up polishing, wire drawing, coating are identical with the production technology of general optical fiber with flow process.
As shown in Figure 1, above-mentioned method of mixing plutonium optical fiber measurement neutron, plutonium optical fiber will be mixed and be placed in measurement environment, mix plutonium optical fiber to be connected with photomultiplier, photomultiplier connection signal amplifying circuit and pulse recording circuit, plutonium in incident neutron and optical fiber reacts, reaction can pass to fiber optic materials makes it excite, photon is released during de excitation, photon through Optical Fiber Transmission to photomultiplier, amplified and record by signal amplification circuit after converting electric impulse signal to, and the quantity of this electric pulse is the number of times being proportional to neutron and plutonium generation nuclear reaction, also incident neutron quantity is just proportional to, the electric impulse signal amount of record unit time can calculate the fluence of neutron, realize the measurement of neutron fluence.The number of pulses that neutron is finally formed with mix the ratio of plutonium, photomultiplier model is relevant with photomultiplier duty, when mixing plutonium ratio-dependent, photomultiplier model is when determining to complete with photomultiplier circuit design, can with the method analog computation of Monte Carlo and the method verified by experiment obtain.
Obviously, those skilled in the art can carry out various change and modification to the present invention and not depart from the spirit and scope of the present invention.Like this, if these amendments of the present invention and modification belong within the scope of the claims in the present invention and equivalent technology thereof, then the present invention is also intended to comprise these change and modification.

Claims (3)

1. mix a plutonium optical fiber, comprise fibre core, covering, coat, jacket layer, it is characterized in that: in the material of described fibre core, mix the raw material containing plutonium-239, the incorporation of the raw material containing plutonium-239 accounts for the 10%-15% of fibre core gross mass.
2. mix plutonium optical fiber as claimed in claim 1, it is characterized in that: the described raw material containing plutonium-239 can select plutonium dioxide, tri-chlorination plutonium, PuF3 or plutonium hexafluoride, raw material containing plutonium-239 is mixed in core material by corresponding proportion, fully mixes under molten condition.
3. adopt the method for mixing plutonium optical fiber measurement neutron described in claim 1 or 2, it is characterized in that: plutonium optical fiber will be mixed and be placed in measurement environment, mix plutonium optical fiber to be connected with photomultiplier, photomultiplier connection signal amplifying circuit and pulse recording circuit, plutonium in incident neutron and optical fiber reacts, reaction can pass to fiber optic materials makes it excite, photon is released during de excitation, photon through Optical Fiber Transmission to photomultiplier, to be amplified by signal amplification circuit after converting electric impulse signal to and by pulse recording circuit record, the quantity of electric pulse is the number of times being proportional to neutron and plutonium generation nuclear reaction, also incident neutron quantity is just proportional to, the electric impulse signal amount of record unit time can calculate the fluence of neutron, realize the measurement of neutron fluence.
CN201410459792.9A 2014-09-10 2014-09-10 Plutonium-doped fiber and neutron measuring method thereof Pending CN105467424A (en)

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Application publication date: 20160406