US3295938A - Method of polishing hygroscopic materials - Google Patents

Method of polishing hygroscopic materials Download PDF

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Publication number
US3295938A
US3295938A US283115A US28311563A US3295938A US 3295938 A US3295938 A US 3295938A US 283115 A US283115 A US 283115A US 28311563 A US28311563 A US 28311563A US 3295938 A US3295938 A US 3295938A
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polishing
hygroscopic
hygroscopic materials
polished
ethylene glycol
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US283115A
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Joseph C Jerome
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    • CCHEMISTRY; METALLURGY
    • C09DYES; PAINTS; POLISHES; NATURAL RESINS; ADHESIVES; COMPOSITIONS NOT OTHERWISE PROVIDED FOR; APPLICATIONS OF MATERIALS NOT OTHERWISE PROVIDED FOR
    • C09GPOLISHING COMPOSITIONS; SKI WAXES
    • C09G1/00Polishing compositions
    • C09G1/02Polishing compositions containing abrasives or grinding agents

Definitions

  • This invention relates to the use of polishing compounds and the prevention of surface oxidation of semiconductor films, and more particularly to surface oxidation preventatives and polishing compounds'for aluminum antimonide thin films and similar hygroscopic materials.
  • Aluminum antimonide and other similar hygroscopic materials used in the field of optics such as prisms and lenses, which are made of soft crystals such as potassium bromide or sodium chloride are difficult to grind and polish since anhydrous solutions must be used as the hydraulic vehicle for the grinding and polishing grit and powders. Water can not be used in the hydraulic vehicle because it will cause dissolving, deformation, pitting or softening of the hygroscopic materials. Further, many anhydrous solvents which could be used to polish aluminum antimonide and the like have a characteristic of quickly deteriorating the wax lapping tools used for polishing.
  • the present invention overcomes the disadvantages of other anhydrous solvents which could be used as hydraulic vehicles for the polishing grit or powder and at the same time provides a preservative coating which prevents surface oxidation on hygroscopic ferrous metals such as aluminum antimonide, and prevents excessive dissolving, deformation of surfaces and pitting and softening of highly hygroscopic materials such as potassium bromide, sodium chloride and other salt compounds which have a natural chemical affinity for absorbing moisture from the air.
  • the present invention also forms a protective antimoisture film over the polished surfaces and can easily be removed with 200 proof alcohol.
  • Still another object of the invention is to provide a protective anti-moisture coating for polished surfaces of hygroscopic materials.
  • a still further object of the invention is to provide a novel polishing compound for hygroscopic materials that will not attack the wax lapping tools used for polishing.
  • Anhydrous solutions of ethylene glycol with grinding and polishing grit and powders permit an easy method of polishing hygroscopic materials that are used almost exclusively in the field of optics.
  • potassium bromide, sodium chloride and other salt compounds can be ground and polished without dissolving, deforming, pitting or softening of the materials and without harm to the wax lapping tools. 7
  • ethylene glycol was the only hydraulic vehicle for the grinding and polishing powders that was compatible to both the hygroscopic materials being polished and the associated wax lapping tools used in the polishing process.
  • a composition comprising a mixture of powdered dehydrated abrasive material and ethylene glycol, in varying proportions depending on the type and nature of the surface to be polished can successfully be used to polish hygroscopic semiconductor materials and the like as mentioned above.
  • the abrasive material may be any of a variety of dry polishing, buffing or lapping abrasives suitable for grinding or polishing hygroscopic ferrous metals such as aluminum antimonide and other hygroscopic materials such as potassium bromide, sodium chloride and other salt compounds.
  • a few typical well known, inert abrasive powders used for polishing semiconductors are disclosed in Transistor Technology, vol. I, by H. E. Bridgers et al., D.
  • a method for polishing hygroscopic ferrous metals and forming a protective surface coating thereon consisting:
  • said hydraulic vehicle consisting entirely of ethylene glycol which will not soften and deform hygroscopic materials
  • said abrasive powder mixed with said ethylene glycol being any of a variety of polishing, bufiing :and lapping abrasives suitable for grinding and polishing hygroscopic materials and entirely free of water,
  • said abrasive powder being any of a variety of well known polishing, buffing, and lapping abrasives suitable for polishing'soft hygroscopic crystals and entirely free of water,

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  • Chemical & Material Sciences (AREA)
  • Organic Chemistry (AREA)
  • Finish Polishing, Edge Sharpening, And Grinding By Specific Grinding Devices (AREA)

Description

United States Patent the Navy No Drawing. Filed May 24, 1963, Ser. No. 283,115 2 Claims. '(Cl. 51-293) The invention herein described may be manufactured and used by or for the Government of the United States of America for governmental purposes Without the payment of any royalties thereon or therefor.
This invention relates to the use of polishing compounds and the prevention of surface oxidation of semiconductor films, and more particularly to surface oxidation preventatives and polishing compounds'for aluminum antimonide thin films and similar hygroscopic materials.
Previous to the present invention there was no known method of polishing aluminum antimonide and preserving it in a state free of surface contamination caused by oxidation. The present invention now greatly extends the use ful life of such semiconductor films.
Aluminum antimonide and other similar hygroscopic materials used in the field of optics such as prisms and lenses, which are made of soft crystals such as potassium bromide or sodium chloride are difficult to grind and polish since anhydrous solutions must be used as the hydraulic vehicle for the grinding and polishing grit and powders. Water can not be used in the hydraulic vehicle because it will cause dissolving, deformation, pitting or softening of the hygroscopic materials. Further, many anhydrous solvents which could be used to polish aluminum antimonide and the like have a characteristic of quickly deteriorating the wax lapping tools used for polishing. The present invention overcomes the disadvantages of other anhydrous solvents which could be used as hydraulic vehicles for the polishing grit or powder and at the same time provides a preservative coating which prevents surface oxidation on hygroscopic ferrous metals such as aluminum antimonide, and prevents excessive dissolving, deformation of surfaces and pitting and softening of highly hygroscopic materials such as potassium bromide, sodium chloride and other salt compounds which have a natural chemical affinity for absorbing moisture from the air.
The present invention also forms a protective antimoisture film over the polished surfaces and can easily be removed with 200 proof alcohol.
It is an object of the invention, therefore, to provide a novel method for polishing hygroscopic materials and preventing the rapid surface oxidation thereof.
It is another object of the invention to provide the hydraulic vehicle for polishing grit and powders which will prevent the rapid oxidation formations on polished surfaces of hygroscopic ferrous metals.
It is a further object of the invention to provide a new polishing compound for polishing hygroscopic materials which will prevent rapid oxidation of the polished surfaces, prevent excessive dissolving, deformation, pitting and softening of the hygroscopic materials which have a natural chemical affinity for absorbing moisture from the am Still another object of the invention is to provide a protective anti-moisture coating for polished surfaces of hygroscopic materials.
A still further object of the invention is to provide a novel polishing compound for hygroscopic materials that will not attack the wax lapping tools used for polishing.
Other objects and many of the attendant advantages of this invention will become readily appreciated as the same becomes better understood by reference to the following detailed description:
In the polishing of semiconductor films, such as aluminum autimonide, which quickly oxidize when exposed to the air because of the natural aflinity for absorbing moisture from the air, it is necessary to use an anhydrous hydraulic vehicle for the grinding and polishing abrasive powders. Semiconductors such as aluminum antimonide quickly oxidize when exposed to the air; therefore, the polished surface of such semiconductors must be protected in order to prevent surface contamination caused by oxidation. While almost every type of water-free compound can be used as a hydraulic agent, all, except ethylene glycol will attack beeswax, crystalline wax, burgundy wax, and micro-pitch wax used on the lapping tools for polishing these materials. Ethylene glycol when used as the hydraulic vehicle for the polishing grit and powders will form a protective anti-moisture film over the polished surfaces and thus extend the useful life of the semi-conductor films.
Anhydrous solutions of ethylene glycol with grinding and polishing grit and powders permit an easy method of polishing hygroscopic materials that are used almost exclusively in the field of optics. Using the polishing compound of the present invention, potassium bromide, sodium chloride and other salt compounds can be ground and polished without dissolving, deforming, pitting or softening of the materials and without harm to the wax lapping tools. 7
It was determined by experimentation that ethylene glycol was the only hydraulic vehicle for the grinding and polishing powders that was compatible to both the hygroscopic materials being polished and the associated wax lapping tools used in the polishing process.
There are a number of known polishing compounds which use ethylene glycol as an ingredient, however, every one of these known compounds would have a very corrosive efiect upon the hygroscopic materials being polished since these prior compounds either contain water, soaps, oils, fatty acids or other corrosive ingredients, or a combination thereof.
Therefore a composition comprising a mixture of powdered dehydrated abrasive material and ethylene glycol, in varying proportions depending on the type and nature of the surface to be polished can successfully be used to polish hygroscopic semiconductor materials and the like as mentioned above. The abrasive material may be any of a variety of dry polishing, buffing or lapping abrasives suitable for grinding or polishing hygroscopic ferrous metals such as aluminum antimonide and other hygroscopic materials such as potassium bromide, sodium chloride and other salt compounds. A few typical well known, inert abrasive powders used for polishing semiconductors are disclosed in Transistor Technology, vol. I, by H. E. Bridgers et al., D. Van Nostrand Co., Inc., Princeton, N.J., 1958 (page 317). With the aforementioned type polishing composition using ethylene glycol as a hydraulic vehicle aluminum antimonide has been surface polished to a thickness of 0.013 of an inch with mirror-like polished surfaces remaining in that state even after a long period of time without any visible discolora tion caused by surface oxidation.
Obviously many modifications and variations of the present invention are possible in the light of the above teachings. It is therefore to be understood that within the scope of the appended claims the invention may be practiced otherwise than as specifically described.
What is claimed is:
1. A method for polishing hygroscopic ferrous metals and forming a protective surface coating thereon consisting:
sisting of a mixture ofan anhydrous hydraulic vehicle and a dehydrated abrasive powder in proportions depending on the type and nature of the hygroscopic surface to be polished, said hydraulic vehicle also being unharmful to said wax lapping tool,
(b) said hydraulic vehicle consisting entirely of ethylene glycol which will not soften and deform hygroscopic materials,
(0) said abrasive powder mixed with said ethylene glycol being any of a variety of polishing, bufiing :and lapping abrasives suitable for grinding and polishing hygroscopic materials and entirely free of water,
(d) contacting the lapping tool with polishing composition thereon to the surface of a hygroscopic ferrous metal until polished to a mirror-like surface,
(e) washing said surface with ethylene glycol to re move excess abrasive,
' (f) forming an anti-moisture film over the polished surface of the hygroscopic ferrous metal with said ethylene glycol during and by the polishing and washing of said surface for preventing contamination of said surface by oxidation thereof. 2. A method for polishing hygroscopic materials such as, aluminum antimonide and other hygroscopic metals, potassium bromide, sodium chloride and other salt compounds which have a natural chemical afiinity for absorbing moisture from the atmosphere, thin semiconductor films and hygroscopic materials used in the field of optics and forming a protective surface coating thereon consisting:
(a) applying to a polishing tool a water-free composition compatible with said lapping tool and consisting of a mixture of an anhydrous hydraulic vehicle and a suitable dehydrated abrasive powder in proportions depending on the type andnature of thehygroscopic material to be polished said hydraulic vehicle also being unharmful to said lapping tool,
(b) said hydraulic vehicle consisting entirely of ethylene glycol which will not soften and deform hygroscopic materials, v
(c) said abrasive powder being any of a variety of well known polishing, buffing, and lapping abrasives suitable for polishing'soft hygroscopic crystals and entirely free of water,
(d) contacting the polishing tool with said polishing composition thereon to the surface of the hygroscopic material until polished to a-bright surface,
(e) washing said surface with ethylene glycol to remove excess abrasive,
(f) forming aprotective film over the polished surfaces of the hygroscopic material with said ethylene glycol during and by the polishing and washing of said surface for preventing oxidation, excessive dissolving, deformation, pittingand softening of the hygroscopic materials.
References Cited by the Examiner UNITED STATES PATENTS 2,006,162 6/ 1935 Fuchs 51,3 04 2,200,726 5/ 1940 Seeley 5 l300 2,980,524 4/1961 Morton 5l304 ALEXANDER H. BRODMERKEL, Primary Examiner.
MORRIS LIEBMAN, Examiner.
D. I. ARNOLD, Assistant Examiner.
US283115A 1963-05-24 1963-05-24 Method of polishing hygroscopic materials Expired - Lifetime US3295938A (en)

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Cited By (3)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US4613345A (en) * 1985-08-12 1986-09-23 International Business Machines Corporation Fixed abrasive polishing media
FR2590844A1 (en) * 1985-07-31 1987-06-05 Inst Fiz An Bssr PROCESS FOR ABRASION MACHINING OF ISLAND SPATH
WO2024173948A1 (en) * 2023-02-17 2024-08-22 University Of Rochester Surfactant-modified abrasives and method of use for polishing water-soluble optical crystals

Citations (3)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US2006162A (en) * 1934-07-25 1935-06-25 Permatex Company Inc Grinding composition
US2200726A (en) * 1939-05-20 1940-05-14 Eldridge E Seeley Buffing compound
US2980524A (en) * 1957-04-29 1961-04-18 Engis Equipment Company Abrasive compositions

Patent Citations (3)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US2006162A (en) * 1934-07-25 1935-06-25 Permatex Company Inc Grinding composition
US2200726A (en) * 1939-05-20 1940-05-14 Eldridge E Seeley Buffing compound
US2980524A (en) * 1957-04-29 1961-04-18 Engis Equipment Company Abrasive compositions

Cited By (3)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
FR2590844A1 (en) * 1985-07-31 1987-06-05 Inst Fiz An Bssr PROCESS FOR ABRASION MACHINING OF ISLAND SPATH
US4613345A (en) * 1985-08-12 1986-09-23 International Business Machines Corporation Fixed abrasive polishing media
WO2024173948A1 (en) * 2023-02-17 2024-08-22 University Of Rochester Surfactant-modified abrasives and method of use for polishing water-soluble optical crystals

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