JP2013040854A - Method of decontaminating radioactively contaminated water and radioactively contaminated soil - Google Patents

Abstract

PROBLEM TO BE SOLVED: To provide a method of decontaminating radioactively contaminated water for eliminating or reducing radioactive substances in water.SOLUTION: Radioactive substances in water are eliminated or reduced using an apparatus for activating liquid with molecular resonance effect technology.

Description

The present invention relates to a method for decontaminating radioactively contaminated water and soil.

A large amount of radioactive material was discharged from the Fukushima Daiichi Nuclear Power Station on March 11, 2011, polluting the surrounding tap water and natural water. Along with this, cesium 137 having a long half-life of 30 years among the radioactive materials mixed in the tap water and natural water is still detected in an amount of several tens of becquerels / kilogram depending on the location.

The provisional regulatory value of radioactive cesium (cesium 134 and cesium 137) applied to drinking water, milk and dairy products in Japan is 200 becquerels / kilogram after the earthquake. Vegetables, grains, meats, seafood, etc. Was 500 becquerels / kilogram. However, the standard value set by the World Health Organization (WHO, hereinafter referred to as “WHO”) for tap water is 10 becquerels / liter, and in Japan before March 17, 2011, the above WHO standard value for drinking water As for food, foods exceeding 10 becquerels / kilogram were not allowed to be imported.

In fact, it takes 100 to 200 days for radioactive cesium taken into the body to be released outside the body, and even if the amount is below the government standard value, the corresponding internal exposure occurs due to continuous intake. Cannot be denied, and there is no concern about the health of the public, especially infants.

For decontamination of contaminated water contaminated with radioactive substances, methods such as adsorption to minerals such as zeolite or filtration by filters are used, but radioactive cesium of about several tens of becquerels / kilogram is less than 10 becquerels / kilogram. In addition, it is difficult for individuals to process radioactive cesium adsorbed on stones and filters. In addition, when the above-mentioned processing is performed by a local government or the like, a large-scale facility is required, and a considerable cost is required for processing the generated waste. For food other than water, there is currently no way other than the state to buy and dispose of it.

Contamination of soil is even more serious, and contamination of arable land and pastures induces contamination of agricultural products and meat produced there. In addition, effective measures have not yet been found in the school yard, etc., after the earth and sand have moved to another place and the moved earth and sand has become a new problem for residents near the destination.

US Pat. No. 6,022,479 US Pat. No. 6,369,399

The objects of the present invention are as follows: (1) At home or at work, individuals lose or reduce radioactive cesium from tap water or natural water containing radioactive cesium that exceeds the WHO standard value, and use radioactively contaminated water as the WHO standard value. Providing a safe way to make the drinking water below, and (2) decontaminating the soil and soil contaminated with radioactive cesium without moving or digging back and making it usable again It is to provide.

In order to achieve the object (1), the present invention uses molecular resonance effect technology (US Pat. Nos. 6,022,479 and 6,369,399).

The molecular resonance effect means that when a polymer such as epoxy resin or urethane containing substances such as fine metal particles, metal salts, natural minerals, etc. is exposed to electromagnetic waves of a certain intensity, resonance vibration accompanied by corona discharge occurs. This is the effect of self-oscillating a low-frequency vibration wave that resonates with the nearby liquid or living tissue.

The technique using the molecular resonance effect is a growth of a plant that can be obtained as an effect of removing harmful effects on living cells due to electromagnetic waves (US Pat. No. 6,369,399) and supplying / ingesting active water produced by the technique. Applied to promotion and maintenance / recovery of the health condition of human living cells (US Pat. No. 6,022,479), and related products are manufactured and sold by US companies.

The method for decontaminating radioactively contaminated water according to the present invention is a process of using an apparatus for producing active water using the molecular resonance effect technique, and a method for decontaminating contaminated earth and sand is based on the apparatus. It was newly confirmed by spraying the produced active water on the earth and sand.

That is, in the process of activating radioactive polluted water having a certain value of radioactive cesium using the method and apparatus for producing active water described in US Pat. No. 6,022,479, radioactive cesium in water is not detected at all. I found a surprising effect.

Furthermore, when the active water produced by the apparatus was sprayed on the earth and sand where a certain amount of radiation dose was detected and the submerged state was maintained for a certain time, the radiation dose of the earth and sand was significantly reduced.

As described above, the decontamination method for radioactively contaminated water according to the present invention uses the “method for producing active water” described in US Pat. No. 6,022,479 as it is for radioactively contaminated water. Is. Hereinafter, a method for producing active water by the method and apparatus described in the aforementioned US Pat. No. 6,022,479 and decontaminating radioactively contaminated water will be described.

The said active water manufacturing apparatus used for the method which concerns on this invention is comprised with the member installed in the form fitted into the water inlet of this water tank perpendicularly | vertically from the top.

The member is composed of a chamber storing an electric circuit or the like located in the upper part and a housing storing a polymer main body or the like located in the lower part.

A cylindrical case for supporting the polymer main body so as to wrap the polymer main body is stored inside the housing, and the cylindrical case has an annular wall (side surface) having a certain thickness, and the annular wall The inner peripheral surface of the polymer body surrounds and supports the polymer main body so as to be in close contact with the outer peripheral surface of the polymer main body. The lower bottom surface of the cylindrical case is disposed so as to protrude into the tank, and faces the water surface of the water in the tank while maintaining a certain distance.

At least one set of magnets is embedded in the annular wall of the cylindrical case, and the two magnets constituting the set of magnets are arranged facing each other across the polymer body inside the case. The magnetic field in the range of 2500-25000 oersteds is created by the at least one set of magnets.

The polymer matrix constituting the polymer main body inside the cylindrical case contains substances such as metal salts and minerals that are easily reacted when receiving a certain amount of electromagnetic radiation in the form of ultrafine particles. The proportion of material to the total weight of the polymer body is in the range of 0.04-30 weight percent.

As a decontamination mechanism, first, the semiconductor diode that has obtained power from the electric circuit connected to a battery or a household power source is directed toward the polymer body containing the substance at a frequency of 7.2. Emits visible electromagnetic wave at 7.8Hz, wavelength 400-800nm (nanometer)

Next, the substance mixed in the polymer body is exposed to a magnetic field in the range of 2500-25000 oersted created by the at least one set of magnets installed on the wall of the cylinder. The substance that has received the visible electromagnetic wave resonates with the electromagnetic wave and vibrates with the surrounding polymer matrix.

Furthermore, vibration waves are emitted from the lower bottom surface of the cylindrical case toward the water surface in the tank due to the vibration of the substance and the polymer matrix.

The water that has received the vibration wave is activated by a resonance effect. When the water is radioactively contaminated water, the radioactive substance is decontaminated simultaneously with the activation.

In order to achieve the object (2), the present invention uses active water produced by the molecular resonance effect technique.

That is, the water activated by the apparatus for activating water using the molecular resonance effect technique is sufficiently sprayed on the earth and sand contaminated with radioactive cesium, thereby eliminating the radioactive cesium contained in the earth or sand. It is to reduce.

Safe decontamination of radioactive contaminated water Use of this method allows decontamination of radioactive contaminated water to be easily and safely performed at home and at work. In particular, problems such as difficulty in processing radioactive materials after decontamination, which are seen in conventional decontamination methods, are solved.

The degree of contamination of radioactively contaminated water that can be decontaminated by the method according to the present invention is not clear at present, but natural water containing 11 becquerels / kg of cesium 137 collected in Iidate Village, Fukushima Prefecture by the applicant. As a result of using this method, the value of the cesium 137 decreased to an undetectable range.

Safe decontamination of radioactively contaminated earth and sand The use of this method allows decontamination of radioactively contaminated earth and sand. In particular, the contaminated schoolyard can be used again without the need to move or dig up the soil, and the production activities on the contaminated arable land and pasture can be resumed early. Become.

The experimental results relating to the safe decontamination of the soil contaminated with radioactivity include the following.

Divide the sediment with an equivalent dose of 0.14 microsieverts / hour into three dishes, A, B, and C. A does nothing, and B is submerged with inactive water (natural water) over the soil. , C was submerged with the active water produced by the apparatus. When the equivalent doses of the three were measured after 30 minutes, the following results were obtained. The results of the experiment show the fact that application of active water is effective for decontamination of contaminated soil.

Expected effects in the future As described above, the active water produced by the above technology is applied to soil and sand, in addition to the decontamination effect of contaminated water when the molecular resonance effect technology is applied directly to radioactively contaminated water. The decontamination effect that can be obtained by spraying is widely applied. This is because the decontamination effect of active water, which is effective against sediment, can be expected to be effective against things other than sediment (for example, feed such as straw and human food), and already incorporates radioactive substances into the body. If the active water is treated for humans and animals exposed to the risk of exposure, the radioactive substances accumulated in the body can be reduced, and the effects of internal exposure can be reduced to a minimum. It is.

At the time of filing this application, the applicant has continued experiments from various directions, and the results will be added to the present application as necessary through correction and the like.

It is a perspective view of the activated water manufacturing apparatus used for this invention. It is a top view of the said active water manufacturing apparatus. FIG. 3 is a cross-sectional view taken along line A-A ′ of FIG. 2. A part of the tank is omitted.

Method for decontamination of radioactively contaminated water A most preferred embodiment for carrying out the present invention will be described with reference to the drawings.
The apparatus 2 of the present invention includes a tank 4, a housing 8 that is vertically arranged by storing a cylindrical case 10 that encloses a polymer body 12 therein, and a screw thread on the tank 4 integrally with the housing 8. And a removable chamber 14 including a semiconductor diode 16 that emits electromagnetic waves adjacent to an upper portion of the housing 8 and an electric circuit 18 for operating the semiconductor diode 16. Has been.

A socket 20 for supplying electricity to the electric circuit 18 is installed on the top of the chamber 14. The socket 20 can be connected to a battery, and can also serve as an outlet for drawing DC external power (not shown).

As shown in FIG. 1, to use the device, the tank 4 is first almost filled with water or radioactively contaminated water 22. In order to prevent contaminants from being present in the contaminated water and adversely affecting the decontamination or reducing the speed, it is desirable to use water that has been completely purified as the water injected into the tank 4.

The bottom bottom surface portion 24 of the cylindrical case 10 has a hole 26 through which the main body 12 radiates a low-frequency vibration wave toward the water 22. The height of the water surface is adjusted so that the distance between the lower bottom surface portion 24 of the housing 8 and the water surface 21 is at least 2.5 cm.

The lid 6 is detachably mounted on the neck 30 at the top of the tank 4 by means of a corresponding thread 28 for water access. Similarly, the chamber 14 is also attached to the top of the housing 8 by corresponding threads 32 so that the cylindrical case 10 can be inserted into and removed from the housing 8. Further, since the chamber 14 can be removed, the semiconductor diode 16 and the circuit 18 can be maintained and replaced.

On the side wall of the cylindrical case 10, cylindrical storage portions for arranging the magnets 34 are installed so as to face each other, and the magnets 34 are stored in the storage portions. In this embodiment, three sets of magnets 34 are shown, but any number of sets may be used as long as the total magnetic field to be created is in the range of 2500-25000 oersted. In place of the magnet, an electromagnet can be used.

As shown by + and-in FIG. 2, the magnets 34 arranged in a row vertically have the same pole, and the other one row of magnets 34 facing each other have all the opposite poles. Has been.

A hole 26 is provided in the lower bottom surface portion 24 of the cylindrical case 10 so that the polymer body 12 can radiate low-frequency vibration waves toward the contaminated water 22.

  The electric circuit 18 housed in the chamber 14 is supplied with power through the socket 20, and the semiconductor diode 16 has a visible wavelength of 400-800 nm (nanometer) lambda and a visible electromagnetic wave having a frequency of 7.2-8.2 Hz. It is designed to create enough power to generate

  The frequency and wavelength range of the visible electromagnetic wave emitted from the semiconductor diode 16 and the strength of the magnetic field governing the polymer body 12 and the material at that time are very important for the practice of the present invention. The polymer body 12 and the particulate matter contained therein react only to electromagnetic waves of the frequency and wavelength in a magnetic field in the range of 2500-25000 oersteds, and as a result resonate and are active against water 22 This is because the energy for conversion or decontamination is emitted.

  Next, the polymer and the particulate material constituting the polymer body 12 that resonates upon receiving electromagnetic radiation will be described.

  The polymer body 12 is a polymer of a polymer matrix in which polymers having a length in which at least 38 monomer units are linearly chain-polymerized are assembled. Although a thermosetting polymer or a thermoplastic polymer may be used, it is preferable to use a polymer having a relatively high relative dielectric constant. This is because, when the relative dielectric constant is high, substitution of bonded electrons and non-bonded electrons in the polymer when affected by a magnetic field is facilitated, and the reaction of the substance inside with respect to the electromagnetic wave continues.

The polymer must be capable of absorbing visible electromagnetic waves with a wavelength of 400-800 nm. Examples of the polymer having a high relative dielectric constant and the ability to absorb visible electromagnetic waves include urethane, epoxy, and furan. In this embodiment, urethane is used.

  The polymer matrix incorporates the material described below, which is a flash of light (visible electromagnetic wave) with a frequency of 7.2-8.2 Hz and a wavelength of 400-800 nm when the polymer body is subject to a 2500-25000 oersted magnetic field. Resonates in response to). The substance emits a low-frequency vibration wave along with the resonance, and the electromagnetic wave promotes and enhances corona discharge of itself or another substance. The resulting vibration wave is usually in the range of 0.5-5.0 Hz.

In this example, the following substances selected from the viewpoint of maximizing the reaction to electromagnetic waves are made into ultra-particles and dispersed in a polymer matrix. The unit of numerical values representing the amount of each substance is weight percent. Antimony potassium tartrate 1.3 Chromium potassium sulfate 1.6 Lead oxide 0.4 Boric acid 4.2 Aluminum sulfate 1.2
Nickel nitrate 1.6 Iron oxide 6.2 Calcite [CaCO.sub.3] 0.3 Peacock stone [Cu.sub.2 Co.sub.3 (OH) sub.2] 0.3 Quartz [SiO.
sub.2] 1.3 Agate [SiO. sub.2] 0.3 Carnelian [
SiO.sub.2] 3.2 Amethyst [SiO.sub.2] 0.2 Citrulline [SiO.sub.2] 1.3 Soft ball or jade [Ca.sub.2 Mg.sub.5 (Si.sub. 8O.sub.8O.sub.22) (OH) .sub.2
2.2 Opal [SiO.sub.2
.multidot. nH.sub.2O] 0.4 Total 26.0

By using this method for contaminated water containing 11 becquerels / kg cesium 137, the cesium 137 will not be detected at all at the time of filing. Although it cannot be shown, the following considerations are possible.

That is, it has been reported that the exchange and transfer of electrons within and between atoms occurs in the molecule due to the molecular resonance effect. Changes in the number and position of electrons in the radioactive cesium atoms in the water that received the vibrational wave radiation from the polymer body promoted the change in the number of neutrons and promoted the decay of the radioactive cesium. Conceivable.

In addition, vibrational waves are radiated from water molecules activated by the molecular resonance effect, causing other water molecules to resonate, and the molecular resonance and vibrational wave radiation expand in a chained manner, causing the decay of the radioactive cesium. It is thought that this is further promoted.

Decontamination of earth and sand related to radioactive contamination using activated water The method for producing activated water is the same as the decontamination method of radioactively contaminated water described above.

By dewatering the activated water produced by the above method to the soil contaminated with radioactive cesium, decontamination of the earth and sand constituting the soil is performed.

About the method of spraying the active water, depending on the size of the soil to be decontaminated, it can be from manual operation using rain dew or bucket, etc., but by a machine such as a pump or sprinkler, but in any case However, it is necessary to ensure that the active water is distributed evenly over the entire contaminated soil. Moreover, about the depth of inundation, it is desirable to sprinkle so that active water may spread at least from the ground surface to the depth of 10 centimeters.

The process for producing the decontamination effect on the earth and sand is not clear at the time of filing, but the following consideration is possible. That is, as described in the discussion on the decontamination of contaminated water, the water molecules activated by the above method constantly emit vibration waves to the surroundings due to molecular resonance. As in the case of decontamination of the radioactively contaminated water, it is considered that this vibration wave affects the structure of electrons and neutrons in the cesium atoms contained in the earth and sand, and promotes the decay of the cesium. Currently, further experiments are being conducted to elucidate the mechanism of decontamination.

However, even if a definite chemical or physical process of change cannot be shown, it does not affect the surprising effects and values that the present invention has. Various embodiments of the present invention relating to a method for decontaminating radioactive pollutants using molecular resonance effect technology can be made by modifying the apparatus for generating resonance and selecting materials. It is clear that it belongs to the category and technical scope of thought.

2
Device 3
Tank 4
Lid 5
Housing 6
Cylindrical case 7
Polymer body 8
Semiconductor diode 9
Electrical circuit 10
Socket 11
Chamber 12
Water surface 13
Water 14
Lower bottom 15
Hole 16
Thread (bottom)
17
Thread (top)
18
magnet

Claims (4)

A method for decontaminating radioactive water, wherein molecular resonance effect technology is used for the radioactive water.   2. A method of decontaminating radioactively contaminated water according to claim 1, wherein the device for activating liquid using the molecular resonance effect technique is used to eliminate or reduce radioactive cesium in water. .   A method for decontamination of radioactively contaminated soil, characterized by using molecular resonance effect technology on radioactively contaminated sediment   The active water produced using the apparatus for activating a liquid using the molecular resonance effect technique is sprayed on the earth and sand constituting the soil contaminated with radioactive cesium. A method for decontaminating earth and sand composing soil contaminated by the radioactive cesium.

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