HRP20170278T1 - Samogaseći polimerni pripravak - Google Patents
Samogaseći polimerni pripravak Download PDFInfo
- Publication number
- HRP20170278T1 HRP20170278T1 HRP20170278TT HRP20170278T HRP20170278T1 HR P20170278 T1 HRP20170278 T1 HR P20170278T1 HR P20170278T T HRP20170278T T HR P20170278TT HR P20170278 T HRP20170278 T HR P20170278T HR P20170278 T1 HRP20170278 T1 HR P20170278T1
- Authority
- HR
- Croatia
- Prior art keywords
- weight
- phr
- self
- composition according
- polymer composition
- Prior art date
Links
- 239000000203 mixture Substances 0.000 title claims 13
- 229920000642 polymer Polymers 0.000 claims 15
- RTZKZFJDLAIYFH-UHFFFAOYSA-N Diethyl ether Chemical compound CCOCC RTZKZFJDLAIYFH-UHFFFAOYSA-N 0.000 claims 4
- 239000000654 additive Substances 0.000 claims 4
- 230000000996 additive effect Effects 0.000 claims 4
- 239000003795 chemical substances by application Substances 0.000 claims 2
- 229920001577 copolymer Polymers 0.000 claims 2
- 239000012747 synergistic agent Substances 0.000 claims 2
- QVGXLLKOCUKJST-UHFFFAOYSA-N atomic oxygen Chemical compound [O] QVGXLLKOCUKJST-UHFFFAOYSA-N 0.000 claims 1
- 239000011324 bead Substances 0.000 claims 1
- 229920001400 block copolymer Polymers 0.000 claims 1
- 239000000571 coke Substances 0.000 claims 1
- 125000003700 epoxy group Chemical group 0.000 claims 1
- 239000006260 foam Substances 0.000 claims 1
- 239000000463 material Substances 0.000 claims 1
- 229910052760 oxygen Inorganic materials 0.000 claims 1
- 239000001301 oxygen Substances 0.000 claims 1
- 230000005855 radiation Effects 0.000 claims 1
- 230000000087 stabilizing effect Effects 0.000 claims 1
- 229920006163 vinyl copolymer Polymers 0.000 claims 1
Classifications
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08J—WORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
- C08J9/00—Working-up of macromolecular substances to porous or cellular articles or materials; After-treatment thereof
- C08J9/0061—Working-up of macromolecular substances to porous or cellular articles or materials; After-treatment thereof characterized by the use of several polymeric components
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08F—MACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
- C08F212/00—Copolymers of compounds having one or more unsaturated aliphatic radicals, each having only one carbon-to-carbon double bond, and at least one being terminated by an aromatic carbocyclic ring
- C08F212/02—Monomers containing only one unsaturated aliphatic radical
- C08F212/04—Monomers containing only one unsaturated aliphatic radical containing one ring
- C08F212/06—Hydrocarbons
- C08F212/08—Styrene
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08F—MACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
- C08F293/00—Macromolecular compounds obtained by polymerisation on to a macromolecule having groups capable of inducing the formation of new polymer chains bound exclusively at one or both ends of the starting macromolecule
- C08F293/005—Macromolecular compounds obtained by polymerisation on to a macromolecule having groups capable of inducing the formation of new polymer chains bound exclusively at one or both ends of the starting macromolecule using free radical "living" or "controlled" polymerisation, e.g. using a complexing agent
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08F—MACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
- C08F8/00—Chemical modification by after-treatment
- C08F8/06—Oxidation
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08K—Use of inorganic or non-macromolecular organic substances as compounding ingredients
- C08K3/00—Use of inorganic substances as compounding ingredients
- C08K3/02—Elements
- C08K3/04—Carbon
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08K—Use of inorganic or non-macromolecular organic substances as compounding ingredients
- C08K5/00—Use of organic ingredients
- C08K5/0008—Organic ingredients according to more than one of the "one dot" groups of C08K5/01 - C08K5/59
- C08K5/0066—Flame-proofing or flame-retarding additives
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
- C08L25/00—Compositions of, homopolymers or copolymers of compounds having one or more unsaturated aliphatic radicals, each having only one carbon-to-carbon double bond, and at least one being terminated by an aromatic carbocyclic ring; Compositions of derivatives of such polymers
- C08L25/02—Homopolymers or copolymers of hydrocarbons
- C08L25/04—Homopolymers or copolymers of styrene
- C08L25/06—Polystyrene
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
- C08L51/00—Compositions of graft polymers in which the grafted component is obtained by reactions only involving carbon-to-carbon unsaturated bonds; Compositions of derivatives of such polymers
- C08L51/04—Compositions of graft polymers in which the grafted component is obtained by reactions only involving carbon-to-carbon unsaturated bonds; Compositions of derivatives of such polymers grafted on to rubbers
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
- C08L51/00—Compositions of graft polymers in which the grafted component is obtained by reactions only involving carbon-to-carbon unsaturated bonds; Compositions of derivatives of such polymers
- C08L51/06—Compositions of graft polymers in which the grafted component is obtained by reactions only involving carbon-to-carbon unsaturated bonds; Compositions of derivatives of such polymers grafted on to homopolymers or copolymers of aliphatic hydrocarbons containing only one carbon-to-carbon double bond
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08F—MACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
- C08F2438/00—Living radical polymerisation
- C08F2438/02—Stable Free Radical Polymerisation [SFRP]; Nitroxide Mediated Polymerisation [NMP] for, e.g. using 2,2,6,6-tetramethylpiperidine-1-oxyl [TEMPO]
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08F—MACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
- C08F293/00—Macromolecular compounds obtained by polymerisation on to a macromolecule having groups capable of inducing the formation of new polymer chains bound exclusively at one or both ends of the starting macromolecule
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08J—WORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
- C08J2325/00—Characterised by the use of homopolymers or copolymers of compounds having one or more unsaturated aliphatic radicals, each having only one carbon-to-carbon double bond, and at least one being terminated by an aromatic carbocyclic ring; Derivatives of such polymers
- C08J2325/02—Homopolymers or copolymers of hydrocarbons
- C08J2325/04—Homopolymers or copolymers of styrene
- C08J2325/06—Polystyrene
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08J—WORKING-UP; GENERAL PROCESSES OF COMPOUNDING; AFTER-TREATMENT NOT COVERED BY SUBCLASSES C08B, C08C, C08F, C08G or C08H
- C08J2325/00—Characterised by the use of homopolymers or copolymers of compounds having one or more unsaturated aliphatic radicals, each having only one carbon-to-carbon double bond, and at least one being terminated by an aromatic carbocyclic ring; Derivatives of such polymers
- C08J2325/02—Homopolymers or copolymers of hydrocarbons
- C08J2325/04—Homopolymers or copolymers of styrene
- C08J2325/08—Copolymers of styrene
- C08J2325/14—Copolymers of styrene with unsaturated esters
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
- C08L25/00—Compositions of, homopolymers or copolymers of compounds having one or more unsaturated aliphatic radicals, each having only one carbon-to-carbon double bond, and at least one being terminated by an aromatic carbocyclic ring; Compositions of derivatives of such polymers
- C08L25/02—Homopolymers or copolymers of hydrocarbons
- C08L25/04—Homopolymers or copolymers of styrene
- C08L25/08—Copolymers of styrene
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
- C08L53/00—Compositions of block copolymers containing at least one sequence of a polymer obtained by reactions only involving carbon-to-carbon unsaturated bonds; Compositions of derivatives of such polymers
Landscapes
- Chemical & Material Sciences (AREA)
- Health & Medical Sciences (AREA)
- Chemical Kinetics & Catalysis (AREA)
- Medicinal Chemistry (AREA)
- Polymers & Plastics (AREA)
- Organic Chemistry (AREA)
- General Chemical & Material Sciences (AREA)
- Engineering & Computer Science (AREA)
- Materials Engineering (AREA)
- Compositions Of Macromolecular Compounds (AREA)
- Fire-Extinguishing Compositions (AREA)
- Manufacture Of Porous Articles, And Recovery And Treatment Of Waste Products (AREA)
- Inorganic Chemistry (AREA)
Claims (12)
1. Samogaseći polimerni pripravak koji obuhvaća:
a) stabilizirajući polimerni pripravak koji sadrži
i) od 80% do 99,5% težine jednog ili više vinilaromatskih polimera međusobno kompatibilnih; i
ii) od 0,5% do 20% težine barem bloka kopolimera koji obuhvaća:
1) barem vinilaromatski polimerni blok kompatibilan s (i) i da po težini čini količinu jednaku ili veću od 15% težine s obzirom na cijeli blok kopolimer, i
2) barem vinilni kopolimerni blok koji sadrži epoksi skupine tako da ima od 0,7% do 19% težine oksiran kisika računato prema ukupnom bloku kopolimera; i
b) barem halogenirani teško zapaljivi materijal (retardant) od 0,03 phr težine do 10 phr težine, računato na bazi komponente (a).
2. Samogaseći polimerni pripravak prema zahtjevu 1 koji dalje obuhvaća sinergijsko sredstvo od 1 phr do 4 phr težine, računato na bazi komponente (a).
3. Samogaseći polimerni pripravak prema zahtjevu 2 koji dalje obuhvaća sinergijsko sredstvo od 0,1 phr do 1 phr težine, računato na bazi komponente (a).
4. Samogaseći polimerni pripravak prema bilo kojem od zahtjeva 1 do 3 koji dalje sadrži ekspandirajuće sredstvo od 0,2 phr težine do 10 phr težine, računato na bazi komponente (a).
5. Samogaseći polimerni pripravak prema zahtjevu 4 koji dalje sadrži ekspandirajuće sredstvo od 1 phr težine do 10 phr težine, računato na bazi komponente (a).
6. Samogaseći polimerni pripravak prema bilo kojem od zahtjeva 1 do 5 koji dalje sadrži atermani aditiv (nepropustan za toplinsko zračenje) od 0 phr težine do 25 phr težine, računato na bazi komponente (a).
7. Samogaseći polimerni pripravak prema zahtjevu 6 koji dalje sadrži atermani aditiv od 0,2 phr težine do 25 phr težine, računato na bazi komponente (a).
8. Samogaseći polimerni pripravak prema zahtjevu 7 koji dalje sadrži atermani aditiv od 1 phr težine do 20 phr težine, računato na bazi komponente (a).
9. Samogaseći polimerni pripravak prema bilo kojem od zahtjeva 6 do 8 gdje je atermani aditiv koks.
10. Ekspandirajuća zrnca koja sadrže samogaseći polimerni pripravak prema bilo kojem od zahtjeva 4 do 9.
11. Oblikovani predmeti koji sadrže samogaseći polimerni pripravak prema bilo kojem od zahtjeva 1 do 3.
12. Polimerne pjene koje sadrže samogaseći polimerni pripravak prema bilo kojem od zahtjeva 2 do 9.
Applications Claiming Priority (3)
Application Number | Priority Date | Filing Date | Title |
---|---|---|---|
IT001973A ITMI20121973A1 (it) | 2012-11-20 | 2012-11-20 | Composizione polimerica autoestinguente |
EP13805588.4A EP2922917B1 (en) | 2012-11-20 | 2013-11-15 | Self-extinguishing polymeric composition |
PCT/IB2013/060157 WO2014080326A1 (en) | 2012-11-20 | 2013-11-15 | Self-extinguishing polymeric composition |
Publications (1)
Publication Number | Publication Date |
---|---|
HRP20170278T1 true HRP20170278T1 (hr) | 2017-06-16 |
Family
ID=47631657
Family Applications (1)
Application Number | Title | Priority Date | Filing Date |
---|---|---|---|
HRP20170278TT HRP20170278T1 (hr) | 2012-11-20 | 2017-02-21 | Samogaseći polimerni pripravak |
Country Status (15)
Country | Link |
---|---|
US (1) | US10087297B2 (hr) |
EP (1) | EP2922917B1 (hr) |
JP (1) | JP2015535029A (hr) |
CN (1) | CN104781338B (hr) |
BR (1) | BR112015004249B1 (hr) |
ES (1) | ES2619415T3 (hr) |
HR (1) | HRP20170278T1 (hr) |
HU (1) | HUE032417T2 (hr) |
IT (1) | ITMI20121973A1 (hr) |
MX (1) | MX367146B (hr) |
MY (1) | MY169236A (hr) |
PL (1) | PL2922917T3 (hr) |
PT (1) | PT2922917T (hr) |
RU (1) | RU2645485C2 (hr) |
WO (1) | WO2014080326A1 (hr) |
Families Citing this family (3)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
ITMI20121808A1 (it) * | 2012-10-24 | 2014-04-25 | Versalis Spa | Composizioni polimeriche concentrate di polimeri e/o copolimeri vinilaromatici |
DE102021104714A1 (de) | 2021-02-26 | 2022-09-01 | Sunpor Kunststoff Gmbh | Reaktive Flammschutzzusammensetzung |
CN114516935B (zh) * | 2021-12-07 | 2024-04-05 | 徐州耐威斯新材料有限公司 | 一种反应型阻燃剂改性聚苯乙烯泡沫材料和制备方法 |
Family Cites Families (25)
Publication number | Priority date | Publication date | Assignee | Title |
---|---|---|---|---|
US4032481A (en) | 1976-01-30 | 1977-06-28 | Arco Polymers, Inc. | Heat stabilizers for expandable styrene polymers |
US4051199A (en) | 1976-03-04 | 1977-09-27 | Phillips Petroleum Company | Epoxidized copolymers of styrene, butadiene and isoprene |
US4131725A (en) | 1977-08-08 | 1978-12-26 | Phillips Petroleum Company | Polymer epoxidation process |
DE3122341A1 (de) | 1981-06-05 | 1982-12-23 | Chemische Werke Hüls AG, 4370 Marl | Feinteilige expandierbare styrolpolymerisate |
DE3402539C2 (de) | 1983-02-02 | 1985-07-18 | Chemische Fabrik Kalk GmbH, 5000 Köln | Verfahren zur Stabilisierung von Tetrabrombisphenol A-bis-(dibrompropyl)-äther oder Hexabromcyclododecan |
JPH0841351A (ja) * | 1994-08-03 | 1996-02-13 | Sumitomo Bakelite Co Ltd | 熱可塑性樹脂組成物 |
US6576692B1 (en) | 1994-10-06 | 2003-06-10 | Daicel Chemical Industries, Ltd. | Epoxidized block copolymer, its production, and its composition |
IT1275915B1 (it) * | 1995-03-16 | 1997-10-24 | Enichem Spa | Composizioni polimeriche autoestinguenti |
WO1997009374A1 (en) | 1995-09-07 | 1997-03-13 | Bromine Compounds Ltd. | Thermally stable hexabromocyclododecane fire retardants |
JPH09194739A (ja) * | 1996-01-17 | 1997-07-29 | Daicel Chem Ind Ltd | 難燃性樹脂組成物 |
JPH10168273A (ja) * | 1996-12-13 | 1998-06-23 | Daicel Chem Ind Ltd | 難燃性樹脂組成物 |
ITMI981156A1 (it) | 1998-05-26 | 1999-11-26 | Enichem Spa | Composizioni polimeriche |
JPH11343381A (ja) * | 1998-06-01 | 1999-12-14 | Daicel Chem Ind Ltd | 熱可塑性樹脂組成物 |
JP3983388B2 (ja) * | 1998-09-29 | 2007-09-26 | 出光興産株式会社 | 熱可塑性樹脂組成物および射出成形品 |
US6903164B2 (en) | 2000-11-13 | 2005-06-07 | Daicel Chemical Industries, Ltd. | Epoxidized thermoplastic polymers and processes for their production |
ITMI20012708A1 (it) | 2001-12-20 | 2003-06-20 | Enichem Spa | Dispositivo per la granulazione a caldo di polimeri termolastici |
ITMI20021495A1 (it) | 2002-07-09 | 2002-10-08 | Polimeri Europa Spa | Procedimento per la preparazione di copolimeri a blocchi. |
JP2006083282A (ja) * | 2004-09-16 | 2006-03-30 | Wintech Polymer Ltd | 難燃性ポリブチレンテレフタレート樹脂組成物 |
US7468415B2 (en) | 2007-01-04 | 2008-12-23 | E. I. Du Pont De Nemours And Company | Method for preparing glycidyloxystyrene monomers and polymers thereof |
JP2008189823A (ja) * | 2007-02-06 | 2008-08-21 | Yokohama Rubber Co Ltd:The | 熱硬化性接着剤組成物 |
ITMI20080823A1 (it) * | 2008-05-07 | 2009-11-08 | Polimeri Europa Spa | Composizioni di polimeri vinilaromatici espansibili a migliorata capacita' di isolamento termico, procedimento per la loro preparazione ed articoli espansi da esse ottenuti |
KR100975024B1 (ko) * | 2008-08-14 | 2010-08-11 | 제일모직주식회사 | 내충격성 및 내화학성이 향상된 난연성 열가소성 수지 조성물 |
IT1392391B1 (it) * | 2008-12-19 | 2012-03-02 | Polimeri Europa Spa | Composizioni di polimeri vinilaromatici espansibili a migliorata capacita' di isolamento termico, procedimento per la loro preparazione ed articoli espansi da loro ottenuti |
IT1393962B1 (it) * | 2009-05-05 | 2012-05-17 | Polimeri Europa Spa | Articoli espansi con ottima resistenza allo irraggiamento solare e ottime proprieta' termoisolanti e meccaniche |
CN102471397B (zh) | 2009-06-30 | 2013-11-06 | 陶氏环球技术有限责任公司 | 溴化并环氧化的阻燃剂 |
-
2012
- 2012-11-20 IT IT001973A patent/ITMI20121973A1/it unknown
-
2013
- 2013-11-15 EP EP13805588.4A patent/EP2922917B1/en active Active
- 2013-11-15 HU HUE13805588A patent/HUE032417T2/en unknown
- 2013-11-15 US US14/441,673 patent/US10087297B2/en not_active Expired - Fee Related
- 2013-11-15 WO PCT/IB2013/060157 patent/WO2014080326A1/en active Application Filing
- 2013-11-15 PT PT138055884T patent/PT2922917T/pt unknown
- 2013-11-15 BR BR112015004249-0A patent/BR112015004249B1/pt not_active IP Right Cessation
- 2013-11-15 CN CN201380059106.2A patent/CN104781338B/zh active Active
- 2013-11-15 MX MX2015001920A patent/MX367146B/es active IP Right Grant
- 2013-11-15 PL PL13805588T patent/PL2922917T3/pl unknown
- 2013-11-15 MY MYPI2015000364A patent/MY169236A/en unknown
- 2013-11-15 RU RU2015105039A patent/RU2645485C2/ru active
- 2013-11-15 JP JP2015542402A patent/JP2015535029A/ja active Pending
- 2013-11-15 ES ES13805588.4T patent/ES2619415T3/es active Active
-
2017
- 2017-02-21 HR HRP20170278TT patent/HRP20170278T1/hr unknown
Also Published As
Publication number | Publication date |
---|---|
RU2645485C2 (ru) | 2018-02-21 |
US10087297B2 (en) | 2018-10-02 |
CN104781338A (zh) | 2015-07-15 |
MY169236A (en) | 2019-03-19 |
MX367146B (es) | 2019-08-07 |
BR112015004249A2 (pt) | 2017-07-04 |
ES2619415T3 (es) | 2017-06-26 |
RU2015105039A (ru) | 2017-01-10 |
PT2922917T (pt) | 2017-03-21 |
BR112015004249B1 (pt) | 2021-02-02 |
ITMI20121973A1 (it) | 2014-05-21 |
EP2922917A1 (en) | 2015-09-30 |
EP2922917B1 (en) | 2017-01-04 |
PL2922917T3 (pl) | 2017-07-31 |
WO2014080326A1 (en) | 2014-05-30 |
CN104781338B (zh) | 2017-07-25 |
HUE032417T2 (en) | 2017-10-30 |
US20150299410A1 (en) | 2015-10-22 |
JP2015535029A (ja) | 2015-12-07 |
MX2015001920A (es) | 2015-06-22 |
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