CN117264554A - Multifunctional flame-retardant heat-insulation aerogel composite material and preparation method thereof - Google Patents

Multifunctional flame-retardant heat-insulation aerogel composite material and preparation method thereof Download PDF

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Publication number
CN117264554A
CN117264554A CN202311158743.7A CN202311158743A CN117264554A CN 117264554 A CN117264554 A CN 117264554A CN 202311158743 A CN202311158743 A CN 202311158743A CN 117264554 A CN117264554 A CN 117264554A
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flame
retardant
layer
heat
adhesive layer
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王兆雄
蒋奇西
张弜
王鹏臻
王劲
陈昭圻
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Guangdong Qixiong New Material Technology Co ltd
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Guangdong Qixiong New Material Technology Co ltd
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    • C09DYES; PAINTS; POLISHES; NATURAL RESINS; ADHESIVES; COMPOSITIONS NOT OTHERWISE PROVIDED FOR; APPLICATIONS OF MATERIALS NOT OTHERWISE PROVIDED FOR
    • C09JADHESIVES; NON-MECHANICAL ASPECTS OF ADHESIVE PROCESSES IN GENERAL; ADHESIVE PROCESSES NOT PROVIDED FOR ELSEWHERE; USE OF MATERIALS AS ADHESIVES
    • C09J7/00Adhesives in the form of films or foils
    • C09J7/20Adhesives in the form of films or foils characterised by their carriers
    • C09J7/29Laminated material
    • CCHEMISTRY; METALLURGY
    • C09DYES; PAINTS; POLISHES; NATURAL RESINS; ADHESIVES; COMPOSITIONS NOT OTHERWISE PROVIDED FOR; APPLICATIONS OF MATERIALS NOT OTHERWISE PROVIDED FOR
    • C09JADHESIVES; NON-MECHANICAL ASPECTS OF ADHESIVE PROCESSES IN GENERAL; ADHESIVE PROCESSES NOT PROVIDED FOR ELSEWHERE; USE OF MATERIALS AS ADHESIVES
    • C09J11/00Features of adhesives not provided for in group C09J9/00, e.g. additives
    • C09J11/02Non-macromolecular additives
    • C09J11/04Non-macromolecular additives inorganic
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    • C09DYES; PAINTS; POLISHES; NATURAL RESINS; ADHESIVES; COMPOSITIONS NOT OTHERWISE PROVIDED FOR; APPLICATIONS OF MATERIALS NOT OTHERWISE PROVIDED FOR
    • C09JADHESIVES; NON-MECHANICAL ASPECTS OF ADHESIVE PROCESSES IN GENERAL; ADHESIVE PROCESSES NOT PROVIDED FOR ELSEWHERE; USE OF MATERIALS AS ADHESIVES
    • C09J197/00Adhesives based on lignin-containing materials
    • C09J197/02Lignocellulosic material, e.g. wood, straw or bagasse
    • CCHEMISTRY; METALLURGY
    • C09DYES; PAINTS; POLISHES; NATURAL RESINS; ADHESIVES; COMPOSITIONS NOT OTHERWISE PROVIDED FOR; APPLICATIONS OF MATERIALS NOT OTHERWISE PROVIDED FOR
    • C09JADHESIVES; NON-MECHANICAL ASPECTS OF ADHESIVE PROCESSES IN GENERAL; ADHESIVE PROCESSES NOT PROVIDED FOR ELSEWHERE; USE OF MATERIALS AS ADHESIVES
    • C09J7/00Adhesives in the form of films or foils
    • C09J7/30Adhesives in the form of films or foils characterised by the adhesive composition
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08KUse of inorganic or non-macromolecular organic substances as compounding ingredients
    • C08K3/00Use of inorganic substances as compounding ingredients
    • C08K3/32Phosphorus-containing compounds
    • C08K2003/321Phosphates
    • C08K2003/322Ammonium phosphate
    • C08K2003/323Ammonium polyphosphate
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08LCOMPOSITIONS OF MACROMOLECULAR COMPOUNDS
    • C08L2201/00Properties
    • C08L2201/02Flame or fire retardant/resistant
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    • C09DYES; PAINTS; POLISHES; NATURAL RESINS; ADHESIVES; COMPOSITIONS NOT OTHERWISE PROVIDED FOR; APPLICATIONS OF MATERIALS NOT OTHERWISE PROVIDED FOR
    • C09JADHESIVES; NON-MECHANICAL ASPECTS OF ADHESIVE PROCESSES IN GENERAL; ADHESIVE PROCESSES NOT PROVIDED FOR ELSEWHERE; USE OF MATERIALS AS ADHESIVES
    • C09J2301/00Additional features of adhesives in the form of films or foils
    • C09J2301/10Additional features of adhesives in the form of films or foils characterized by the structural features of the adhesive tape or sheet
    • C09J2301/12Additional features of adhesives in the form of films or foils characterized by the structural features of the adhesive tape or sheet by the arrangement of layers
    • C09J2301/122Additional features of adhesives in the form of films or foils characterized by the structural features of the adhesive tape or sheet by the arrangement of layers the adhesive layer being present only on one side of the carrier, e.g. single-sided adhesive tape
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    • C09JADHESIVES; NON-MECHANICAL ASPECTS OF ADHESIVE PROCESSES IN GENERAL; ADHESIVE PROCESSES NOT PROVIDED FOR ELSEWHERE; USE OF MATERIALS AS ADHESIVES
    • C09J2301/00Additional features of adhesives in the form of films or foils
    • C09J2301/10Additional features of adhesives in the form of films or foils characterized by the structural features of the adhesive tape or sheet
    • C09J2301/16Additional features of adhesives in the form of films or foils characterized by the structural features of the adhesive tape or sheet by the structure of the carrier layer
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    • C09DYES; PAINTS; POLISHES; NATURAL RESINS; ADHESIVES; COMPOSITIONS NOT OTHERWISE PROVIDED FOR; APPLICATIONS OF MATERIALS NOT OTHERWISE PROVIDED FOR
    • C09JADHESIVES; NON-MECHANICAL ASPECTS OF ADHESIVE PROCESSES IN GENERAL; ADHESIVE PROCESSES NOT PROVIDED FOR ELSEWHERE; USE OF MATERIALS AS ADHESIVES
    • C09J2301/00Additional features of adhesives in the form of films or foils
    • C09J2301/40Additional features of adhesives in the form of films or foils characterized by the presence of essential components
    • C09J2301/408Additional features of adhesives in the form of films or foils characterized by the presence of essential components additives as essential feature of the adhesive layer
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    • C09J2400/10Presence of inorganic materials
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    • C09J2400/00Presence of inorganic and organic materials
    • C09J2400/10Presence of inorganic materials
    • C09J2400/14Glass
    • C09J2400/143Glass in the substrate
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    • C09J2400/00Presence of inorganic and organic materials
    • C09J2400/10Presence of inorganic materials
    • C09J2400/16Metal
    • C09J2400/163Metal in the substrate
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    • C09JADHESIVES; NON-MECHANICAL ASPECTS OF ADHESIVE PROCESSES IN GENERAL; ADHESIVE PROCESSES NOT PROVIDED FOR ELSEWHERE; USE OF MATERIALS AS ADHESIVES
    • C09J2400/00Presence of inorganic and organic materials
    • C09J2400/20Presence of organic materials
    • C09J2400/26Presence of textile or fabric
    • C09J2400/263Presence of textile or fabric in the substrate
    • YGENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02BCLIMATE CHANGE MITIGATION TECHNOLOGIES RELATED TO BUILDINGS, e.g. HOUSING, HOUSE APPLIANCES OR RELATED END-USER APPLICATIONS
    • Y02B80/00Architectural or constructional elements improving the thermal performance of buildings
    • Y02B80/10Insulation, e.g. vacuum or aerogel insulation

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  • Chemical & Material Sciences (AREA)
  • Organic Chemistry (AREA)
  • Engineering & Computer Science (AREA)
  • Life Sciences & Earth Sciences (AREA)
  • Wood Science & Technology (AREA)
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  • Inorganic Chemistry (AREA)
  • Laminated Bodies (AREA)

Abstract

The invention discloses a multifunctional flame-retardant heat-insulating aerogel composite material and a preparation method thereof. The invention has the functions of flame retardance, heat preservation, convenient installation and the like, wherein the heat insulation performance of the aerogel heat insulation felt layer improves the heat insulation and heat preservation functions of the material, compared with the traditional material, the heat retardance and heat preservation performance are greatly enhanced, and the use and installation functions of the material are more convenient by adding the anti-solidification release film (paper).

Description

Multifunctional flame-retardant heat-insulation aerogel composite material and preparation method thereof
Technical Field
The invention belongs to the technical field of flame-retardant heat-insulating composite materials, and particularly relates to a multifunctional flame-retardant heat-insulating aerogel composite material and a preparation method thereof.
Background
The multifunctional flame-retardant heat-insulating material is a material with wide application fields and huge application prospects in engineering, and is permeated into various fields of national defense and military industry, aerospace, transportation, biomedicine, constructional engineering and the like. Meanwhile, the lighter and stronger material can greatly reduce the survival cost of human beings on the premise of not influencing the requirements of the human beings, and effectively relieve the requirements of the human beings on energy sources.
Aerogel is used as a first-choice material of a future heat-insulating flame-retardant material, and on the basis of solving the production, products capable of being optimized and even replacing the existing materials in multiple fields such as buildings, ships, rail transit and the like are developed. Especially in the field of ships, the problems of more dust, large construction pollution, large occupied space, influence on human health and the like of the existing materials are solved.
However, the aerogel materials with low density developed in recent years have a good heat-insulating effect, but have a low mechanical modulus. Compared with the traditional external wall heat insulation material, the aerogel is fragile, and the block material formed by aerogel particles is easy to crack and does not have good adhesion.
Disclosure of Invention
In order to solve the technical problems in the prior art, the invention provides a multifunctional flame-retardant heat-insulation aerogel composite material and a preparation method thereof. The material can greatly reduce dust hazard, reduce environmental pollution of a construction site, improve working efficiency of the construction site, and achieve the effect of construction requirements by using lighter and less space.
In order to achieve the above object, the present invention provides the following technical solutions:
the multifunctional flame-retardant heat-insulating aerogel composite material is of a multilayer structure and is characterized by comprising a fireproof material layer, a first flame-retardant adhesive layer, an aerogel heat-insulating felt layer, a second flame-retardant adhesive layer, a flame-retardant material fiber layer, a flame-retardant adhesive layer and a curing-preventing release paper layer which are sequentially stacked from top to bottom.
Further, the fireproof material layer is one or a combination of more of marine flame-retardant white cloth, glass fiber cloth, aluminum silicate cloth, high silica fiber cloth, aluminum foil fiber cloth or basalt fiber cloth.
Further, the first flame-retardant adhesive and the second flame-retardant adhesive layer are formed by mixing 3-5% of artificial seawater, 10 # engine oil, 3-10% of hydrochloric acid and 7-9% of sodium hydroxide.
Further, the aerogel insulation blanket is comprised of an aerogel composite.
Further, the flame retardant material fiber layer is one of glass fiber cloth or basalt fiber cloth.
Further, the flame-retardant adhesive layer is formed by mixing 30% of acrylic resin, 20% of ammonium polyphosphate and 50% of base paper.
The invention also provides a preparation method of the multifunctional flame-retardant heat-insulating aerogel composite material, which is characterized by comprising the following steps:
s1, coating a first flame-retardant adhesive on one side of a fireproof material layer to form a first flame-retardant adhesive layer, coating a second flame-retardant adhesive on one side of an aerogel heat insulation felt layer to form a second flame-retardant adhesive layer, coating the first flame-retardant adhesive layer with the fireproof material layer on the surface of the aerogel heat insulation felt layer far away from the second flame-retardant adhesive layer, coating a flame-retardant material fiber layer on the surface of the second flame-retardant adhesive layer, and carrying out composite shaping through a high-temperature rolling method to initially prepare the multifunctional flame-retardant heat insulation aerogel composite board;
s2, covering the surface of a flame-retardant material fiber layer of the preliminarily formed composite board with flame-retardant self-adhesive layer to form a flame-retardant self-adhesive layer, coating anti-curing release paper on the surface of the flame-retardant self-adhesive layer, and carrying out rolling composite shaping at normal temperature to finally form a multifunctional flame-retardant heat-insulation aerogel composite material finished product;
s3, cutting the composite board formed in the step S2 into different sizes according to actual needs.
Further, the hot pressing temperature in the step S1 is 675-700 ℃, the pressure is 5.76-10 MPa, and the time is 20-30 min.
Further, the first flame-retardant adhesive and the second flame-retardant adhesive in the S1 are formed by mixing 5% -10% of artificial seawater, 10 # engine oil, 6% -15% of hydrochloric acid and 5% -10% of sodium hydroxide.
Further, the pressure of the normal temperature rolling composite shaping in the S2 is 0.01-0.05 MPa, and the time is 5-15 min.
Compared with the prior art, the invention has the beneficial effects that:
according to the invention, a multilayer structure is used, and the anti-solidification release paper is added, so that the flame-retardant heat-insulating effect of the material is better than that of the existing material; not only has stable structure, but also reduces the volume by nearly 33%. The material can greatly reduce dust hazard, reduce environmental pollution of a construction site, improve working efficiency of the construction site, and achieve the effect of construction requirements by using lighter and less space.
Drawings
FIG. 1 is a schematic structural view of a flame retardant insulation aerogel composite.
In the figure: the fire-proof heat insulation paper comprises a 1-fire-proof material layer, a 2-first flame-retardant adhesive layer, a 3-aerogel heat insulation felt layer, a 4-second flame-retardant adhesive layer, a 5-flame-retardant material fiber layer, a 6-flame-retardant adhesive sticker layer and a 7-curing-proof release paper layer.
Detailed Description
The following describes the detailed implementation of the embodiments of the present invention with reference to the drawings. It should be understood that the detailed description and specific examples, while indicating and illustrating the invention, are not intended to limit the invention.
It should be noted that, without conflict, the embodiments of the present invention and features of the embodiments may be combined with each other.
The invention will be described in detail below with reference to the drawings in connection with exemplary embodiments.
Example 1
Referring to fig. 1, the multifunctional flame-retardant and heat-insulating aerogel composite material of the present invention has a multi-layer structure, and comprises a fireproof material layer 1, a first flame-retardant adhesive layer 2, an aerogel heat-insulating felt layer 3, a second flame-retardant adhesive layer 4, a flame-retardant material fiber layer 5, a flame-retardant adhesive layer 6 and a curing-preventing release paper layer 7 which are sequentially stacked from top to bottom.
Further, the fireproof material layer 1 is one or a combination of more than one of marine flame-retardant white cloth, glass fiber cloth, aluminum silicate cloth, high silica fiber cloth, aluminum foil fiber cloth or basalt fiber cloth.
Further, the first flame retardant adhesive 2 and the second flame retardant adhesive layer 4 are formed by mixing 5% of artificial seawater, 10 # machine oil, 6% of hydrochloric acid and 5% of sodium hydroxide.
Further, the aerogel heat insulation felt layer 3 is made of aerogel composite materials.
Further, the flame retardant material fiber layer 5 is one of glass fiber cloth or basalt fiber cloth.
Further, the flame retardant adhesive layer 6 is formed by mixing 30% of acrylic resin, 20% of ammonium polyphosphate and 50% of base paper.
The invention also provides a preparation method of the multifunctional flame-retardant heat-insulating aerogel composite material, which comprises the following steps:
s1, coating a first flame-retardant adhesive on one side of a fireproof material layer 1 (formed by sequentially laminating and hot-pressing marine flame-retardant white cloth, glass fiber cloth, aluminum silicate cloth, high-silica fiber cloth, aluminum foil fiber cloth and basalt fiber cloth from top to bottom) to form a first flame-retardant adhesive layer 2, coating a second flame-retardant adhesive on one side of an aerogel heat-insulating felt layer to form a second flame-retardant adhesive layer 4, coating the first flame-retardant adhesive layer with the fireproof material layer 1 on the surface of the aerogel heat-insulating felt layer 3 far away from the second flame-retardant adhesive layer, coating a flame-retardant material fiber layer 5 on the surface of the second flame-retardant adhesive layer, and carrying out composite shaping through a high-temperature rolling method to preliminarily prepare the multifunctional flame-retardant heat-insulating aerogel composite board;
s2, covering the surface of a flame-retardant material fiber layer 5 of the preliminarily formed composite board with flame-retardant self-adhesive layer 6, coating anti-curing release paper 7 on the surface of the flame-retardant self-adhesive layer, and carrying out rolling composite shaping at normal temperature to finally form a multifunctional flame-retardant heat-insulation aerogel composite material finished product;
s3, cutting the composite board formed in the step S2 into different sizes according to actual needs.
Further, the hot pressing temperature in the step S1 is 675 ℃, the pressure is 5.76MPa, and the time is 20min.
Further, the first flame-retardant adhesive and the second flame-retardant adhesive in the step S1 are formed by mixing 3% of artificial seawater, 10 # engine oil, 3% of hydrochloric acid and 7% of sodium hydroxide.
Further, the pressure of the normal-temperature rolling composite shaping in the step S2 is 0.02MPa, and the time is 10min.
Example 2
The difference from example 1 is that: the first flame-retardant adhesive and the second flame-retardant adhesive are formed by mixing 8% of artificial seawater, 10 # engine oil, 8% of hydrochloric acid and 9% of sodium hydroxide.
The hot pressing temperature in the step S1 is 700 ℃, the pressure is 5.76MPa, and the time is 20min.
Example 3
The difference from example 1 is that: the first flame-retardant adhesive and the second flame-retardant adhesive are formed by mixing 5% of artificial seawater, 10 # engine oil, 10% of hydrochloric acid and 9% of sodium hydroxide.
The hot pressing temperature in the step S1 is 710 ℃, the pressure is 5.76MPa, and the time is 30min.
Test case
Example 1, example 2 and example 3 were tested for fire resistance according to the temperature rise profile of GB/T9978.1-2008 and a commercial fire protection panel was selected for comparison with the following results:
duration of fire resistance (min)
Example 1 20
Example 2 25
Example 3 30
Comparison group 10
Therefore, the material provided by the invention has obviously improved flame retardant property compared with the traditional material.
It will be evident to those skilled in the art that the invention is not limited to the details of the foregoing illustrative embodiments, and that the present invention may be embodied in other specific forms without departing from the spirit or essential characteristics thereof. The present embodiments are, therefore, to be considered in all respects as illustrative and not restrictive, the scope of the invention being indicated by the appended claims rather than by the foregoing description, and all changes which come within the meaning and range of equivalency of the claims are therefore intended to be embraced therein. Any reference sign in a claim should not be construed as limiting the claim concerned.
Furthermore, it should be understood that although the present disclosure describes embodiments, not every embodiment is provided with a separate embodiment, and that this description is provided for clarity only, and that the disclosure is not limited to the embodiments described in detail below, and that the embodiments described in the examples may be combined as appropriate to form other embodiments that will be apparent to those skilled in the art.

Claims (10)

1. The multifunctional flame-retardant heat-insulating aerogel composite material is of a multilayer structure and is characterized by comprising a fireproof material layer, a first flame-retardant adhesive layer, an aerogel heat-insulating felt layer, a second flame-retardant adhesive layer, a flame-retardant material fiber layer, a flame-retardant adhesive layer and a curing-preventing release paper layer which are sequentially stacked from top to bottom.
2. The multifunctional flame-retardant and heat-insulating aerogel composite material according to claim 1, wherein the fireproof material layer is one or a combination of a plurality of marine flame-retardant white cloth, glass fiber cloth, aluminum silicate cloth, high silica fiber cloth, aluminum foil fiber cloth or basalt fiber cloth.
3. The multifunctional flame-retardant and heat-insulating aerogel composite material according to claim 1, wherein the first flame-retardant adhesive and the second flame-retardant adhesive layer are formed by mixing 3% -5% of artificial seawater, 10 # engine oil, 3% -10% of hydrochloric acid and 7% -9% of sodium hydroxide.
4. The multifunctional flame retardant and thermal insulation aerogel composite of claim 1, wherein the aerogel insulation blanket is comprised of an aerogel composite.
5. The multifunctional flame retardant and thermal insulation aerogel composite of claim 1, wherein the flame retardant material fiber layer is one of fiberglass cloth or basalt fiber cloth.
6. The multifunctional flame-retardant and heat-insulating aerogel composite material according to claim 1, wherein the flame-retardant adhesive layer is formed by mixing 30% of acrylic resin, 20% of ammonium polyphosphate and 50% of base paper.
7. The preparation method of the multifunctional flame-retardant heat-insulating aerogel composite material is characterized by comprising the following steps of:
s1, coating a first flame-retardant adhesive on one side of a fireproof material layer to form a first flame-retardant adhesive layer, coating a second flame-retardant adhesive on one side of an aerogel heat insulation felt layer to form a second flame-retardant adhesive layer, coating the first flame-retardant adhesive layer with the fireproof material layer on the surface of the aerogel heat insulation felt layer far away from the second flame-retardant adhesive layer, coating a flame-retardant material fiber layer on the surface of the second flame-retardant adhesive layer, and carrying out composite shaping through a high-temperature rolling method to initially prepare the multifunctional flame-retardant heat insulation aerogel composite board;
s2, covering the surface of a flame-retardant material fiber layer of the preliminarily formed composite board with flame-retardant self-adhesive layer to form a flame-retardant self-adhesive layer, coating anti-curing release paper on the surface of the flame-retardant self-adhesive layer, and carrying out rolling composite shaping at normal temperature to finally form a multifunctional flame-retardant heat-insulation aerogel composite material finished product;
s3, cutting the composite board formed in the step S2 into different sizes according to actual needs.
8. The method for preparing the multifunctional flame-retardant and heat-insulating aerogel composite material according to claim 7, wherein the hot pressing temperature in the step S1 is 675-700 ℃, the pressure is 5.76-10 MPa, and the time is 20-30 min.
9. The method for preparing the flame-retardant and heat-insulating aerogel composite material according to claim 7, wherein the first flame-retardant adhesive and the second flame-retardant adhesive in the step S1 are formed by mixing 5% -10% of artificial seawater, 10 # engine oil, 6% -15% of hydrochloric acid and 5% -10% of sodium hydroxide.
10. The method for preparing the flame-retardant and heat-insulating aerogel composite material according to claim 7, wherein the pressure of the normal-temperature rolling composite sizing in the step S2 is 0.01-0.05 MPa, and the time is 5-15 min.
CN202311158743.7A 2023-09-08 2023-09-08 Multifunctional flame-retardant heat-insulation aerogel composite material and preparation method thereof Pending CN117264554A (en)

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Cited By (1)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
CN118306068A (en) * 2024-04-25 2024-07-09 保利长大工程有限公司 Inorganic fiber composite aerogel plate and application thereof

Cited By (1)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
CN118306068A (en) * 2024-04-25 2024-07-09 保利长大工程有限公司 Inorganic fiber composite aerogel plate and application thereof

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