CA1115342A - Internal battery fuse - Google Patents

Internal battery fuse

Info

Publication number
CA1115342A
CA1115342A CA324,812A CA324812A CA1115342A CA 1115342 A CA1115342 A CA 1115342A CA 324812 A CA324812 A CA 324812A CA 1115342 A CA1115342 A CA 1115342A
Authority
CA
Canada
Prior art keywords
current collector
cell
fuse
current
section
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Expired
Application number
CA324,812A
Other languages
French (fr)
Inventor
Per Bro
Hong Y. Kang
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
Duracell Inc USA
Original Assignee
PR Mallory and Co Inc
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by PR Mallory and Co Inc filed Critical PR Mallory and Co Inc
Application granted granted Critical
Publication of CA1115342A publication Critical patent/CA1115342A/en
Expired legal-status Critical Current

Links

Classifications

    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M50/00Constructional details or processes of manufacture of the non-active parts of electrochemical cells other than fuel cells, e.g. hybrid cells
    • H01M50/50Current conducting connections for cells or batteries
    • H01M50/572Means for preventing undesired use or discharge
    • H01M50/574Devices or arrangements for the interruption of current
    • H01M50/581Devices or arrangements for the interruption of current in response to temperature
    • HELECTRICITY
    • H01ELECTRIC ELEMENTS
    • H01MPROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M50/00Constructional details or processes of manufacture of the non-active parts of electrochemical cells other than fuel cells, e.g. hybrid cells
    • H01M50/50Current conducting connections for cells or batteries
    • H01M50/572Means for preventing undesired use or discharge
    • H01M50/574Devices or arrangements for the interruption of current
    • H01M50/583Devices or arrangements for the interruption of current in response to current, e.g. fuses
    • YGENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02EREDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E60/00Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
    • Y02E60/10Energy storage using batteries
    • YGENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02PCLIMATE CHANGE MITIGATION TECHNOLOGIES IN THE PRODUCTION OR PROCESSING OF GOODS
    • Y02P70/00Climate change mitigation technologies in the production process for final industrial or consumer products
    • Y02P70/50Manufacturing or production processes characterised by the final manufactured product

Landscapes

  • Chemical & Material Sciences (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Electrochemistry (AREA)
  • General Chemical & Material Sciences (AREA)
  • Connection Of Batteries Or Terminals (AREA)
  • Secondary Cells (AREA)
  • Primary Cells (AREA)
  • Cell Electrode Carriers And Collectors (AREA)

Abstract

INTERNAL BATTERY FUSE

ABSTRACT
An internal battery fuse comprising a portion of a current collector which is thermally shielded whereby excessive built-up heat resulting from a short circuit is concentrated in said portion and which heat fuses the shielded portion and interrupts the circuit prior to excessive internal pressure conditions.

Description

.5~

This invention relates to electrochemical cells æub;ect to internal temperature rise and excessive internal pres~ure bulld-up upon short circuiting and more particularly to lithium/sulfur dioxide cells having ~uch characteristics.
One of the dangers Df cells having high discharge rate capabilities is that a short circuit can result in a rapid rise in temperature within the cell caused by ohmic energy dissipation with concomitant increase in pressure. With such increase in pressure, cells may e~ther explode violen-tly or at the very least open and expel their corrosive contents.
Various expedients have been utilized in preventing the above-mentioned consequences in cells when short circuited. Included in such expedients are thermally responsive elements whereby mechanical or electrical means are used to break the circuit and prevent further untoward consequences. Among such thermal control elements are external fuses, tiodes, electrically res-ponsive cut off switches, low temperature melting solder connections and the like. However, the aorementioned control devices have the disadvantage in that they require elements which are normally not included with or within the cells thereby reducing useful available volumetric space and additionally are for the most part costly in implementation.
It is therefore an object of the present invention to provide a means whereby an integral element within a cell can function as a temperature responsive fuse for preventing untoward consequences resulting from short circuit conditions.
This and other objects, features and advantages will be more clearly seen from the following discussion as well as from the drawing in which the single figure is a partially sectioned elevation view of an electrochemical cell containing the temperature responsive means of the present invention.
Generally stated the present invention involves the use of a portion of a normally disposed metal current collector, whether attached to the anode or the cathDde in an electrochemical cell, as a fuse in preventing excessive temperature and pressu~e rise resulting from short circuit conditions.
Normally, a current collector will not fuse under short circuit conditions lllS3~12 in sufficient time if at all for excessive pressure build-up to be prevented. Fusion of the current collector does not occur because heat built up therein is dissipated through the cell usually by convection currents in the liquid electrolyte caused by the heating of the current collector. In accordance with the present invention a section of the current collector of a suitable size able to retain enough heat to fuse the current collector is enclosed by a thermal shield. Heat lS thereby contained therein and quickly fuses the current collector and interrupts the circuit before excessive pressure conditions occur. The thermal shield functions in a manner whereby heat conduction from the current collector is substantially diminished by preventing the electrolyte from conducting heat (directly or indirectly) from the current collector at the fusing site. With respect to the fusing site it is important that such site be situated between the point or points at ~hich the current collector is attached for external terminal connection and the point6 or points at which the current collector is electrically connected to the electrode so that the circuit is interrupt-able.
The thermal shield may either be a separate thermally insulative material such as plastic including polyolefins such as polyethylene or polypropylene heat sealed around the fusing site or the cell separator itself if made of a ~imilarly thermally insulative material and sufficiently tightly contacted with .. ..... .. .. ...... .
the fusing site to prevent thermal contact between the fusing site and the cell electrolyte. Heat sealable films of polyethylene and polypropylene are commer-cially available in various thicknesses ranging from 0.001 to 0.01 inch. Thick-nesses of 0.001 and 0.002 inch polyethylene are satisfactory and will adequately ~hield the fusing site. Heat sealing of polyethylene or polypropylene film to the metal current collector is preferably done by light, localized pressure by heated platens.
In order for a section of the current collector to properly function as a fuse it should be dimensioned such that the desired fusing current provides sufficient resistance heat to fuse the current collector in air. It is desir-able to thin the section of the current collector, which is to function as a fuse, to such dimensions. ~ current collector having uniform thinned qimensions . .
, 1115.~

throughout ~s less desirable because of the loss of structural integrity engendered thereby. Factors to be consldered ln determining the dimensions of the section to be fused include the resistance, density and meltin~ polnt of the metal used. Table I indicates 60me width dimensions for fusing ~trips of various metals commonly used as current collectors:

TABL~ I ~

~ Heat Generated Compared to Fusing Heat of Fusing Strips (0.5" long - 0.002" thick) Metal Width Cross Section Weight Resist. Heat req. Heat ~ener-inch cm cm~ gms ohms to fuse ated by lOA.
joulessec ~oules Al.010 .0254 .00013 3.51xlO 4 2.05xlO 20.304 2.05 .015 .0381 .00019 5.13xlO 4 1.40xlO 20.444 1.40 .020 .0508 .00026 7.02xlO 4 1.03xlO 20.608 1.03 .025 .0635 .00032 8.64xlO 4 0.83xlO 20.748 0.83 Cu.010 .0254 .00013 1.16xlO 3 1.32xlO 20.683 1.32 .015 .0381 .00019 1.60xlO 3 O.90xlO 21.00 o.go .020 .0508 .00026 2.32xlO 3 0.66x10-2 1.37 0.66 .025 .0635 .00032 2.86xlO 3 0.54xlO 21.68 0.54 Ni.010 .0254 .00013 1.16xlO 5.57xlO1.09 5.57 .015 .0381 .00019 1.69xlO 3 3.81xlO 21.58 3.81 .020 .0508 .00026 2.31xlO 3 2.78xlO 22.16 2.78 .~25 .0635 .00032 2.85xlO 3 2.26xlO 22.68 2.26 Ti.010 .0254 .00013 5.85xlO 0.262 0.887 26.2 , .015 .0381 .00019 8.35xlO 0.179 1.30 17.9 .020 .0508 .00026 1.17xlO 3 0.131 1.77 13.1 .025 .0635 .obo32 1.44x10-3 0.106 2.18 10.6 Note from Table I that copper requires the smallest widths for fusing making it more difficult to handle as a current collector and therefore is least desirable as a fuse metal. Titanium can ha~e the greatest width and ~till fuse and would therefore be the most preferred except for its high cost. As between nickel and aluminum, nickel is preferred as a fuse metal .

.

i~l S.~

.

because of lts greater mechanical strength when in thin strip form. In all instances compatibillty between the electrode and the metal of the current collector associated therewlth is however the determining factor in selec-ting a suitable metal for the current collector. Note that if desired, the fuse slte metal may be different from that of the rest of the current col-: lector and may be welded to the current collector between secttons ~hereof.
In determining currents at which aluminum and nickel fuse, in cellshaving heat conductive electrolytes, when Ruch cells are short circuited wires of aluminum and nickel of varying cross sections are immersed in elec-trolyte solutions of sulfur dioxide used as a cathode depolarizer in acetoni-~ trile and subjected to various current loads. Table II indicates the results of such tests with a comparison between shielded and unshielded metals in solutions as compared to unshielded metals in air:

TABLE II
(0.5 inch lengths) Current Cross Environ- Thermal Current at Time to Collector Section mentShield Which fused Fuse All~36 AWG 1 Strand (1.27xlO ~m ) Air No 5 amp l sec " l Strand " Sol'n No 20 amp 2 sec " " 1 Strand" Sol'n Yes 5 amp 2 sec " " 2 Strand(2.54xlO cm ) Air No 10 amp 2 sec " " 2 Strand" Sol'n No 25 amp 2 sec " " 2 Strand" Sol'n Yes 10 amp 2 sec ll " 4 Strand(5.08xlO cm ) Air No 15 amp 2 sec " " 4 Strand" Sol'n No 25 amp No fusing " " 4 Strand" Sol'n Yes 20 amp 2 sec Ni#40 AWG 4 Strand ~2.0xlO cm ) Air No 5 amp 2 sec " " 4 Strand " Sol'n No 20 amp 2 sec " 4 Strand " Sol'n Yes 5 amp 2 sec " " ô Strand ( -4 2) i No 10 amp 2 sec " " 8 Strand " Sol'n No 25 amp 3 sec " " 8 Strand " Sol'n Yes lO amp 4 sec 5~

Current Cross Environ-Thermal Current atTime to Collector Section mentShield Which Fused Fuse ~i#4~ AWG 12 Strand (6.0xlO cm ) A~r No 15 amp 2 sec 12 Strand " Sol'n No 25 amp No fusing " " 12 Strand " Sol'nYes 15 amp 2 sec By shielding the metal in solution, results comparable to metals in air with respect to fusing capability are obtained. It should be further noted that though the compari60ns were conducted with sulfur dioxide in acetonitrile solutions similar result6 are expected regardless of the elec-trolyte solution composit$on.
The placement and configuration of the internal fuse of the present invention can be more clearly seen with reference to the drawing $n which electrochemical cell 10 $s shown as hav$ng a spirally wound electrode/separa-tor configuration. (The electrode configuration is however, generally immaterial to the operation of the present invention unless the separator is to be used as the thermal shield.) Section lla of nickel current collector 11 extends beneath polypropylene separator 13 and electrically engages lithium anode 12 and i8 the only point of electrical connection between current collector 11 and anode 12 with separator 13 electrically insulating the rest of current collector 11 from anode 12. Thinned strip section 16 with thermally non-conduc-tive shield 17 functions as the thermally responsive fuse. Shield 17 is made of a material such as polyethylene and iB heat sealed around section 16 in order to retain heat in said section during short circuit heat build-up condi-tions. If the current collector 11 with fusing site 16 is tightly pressed ngainst separator 13 and insulative member 14 whereby the sulfur dioxide cathode depolarizer in acetonitrile electrolyte $s excluded from thermal contact with 6ection lo, shield member 17 may be dispensed with, with the separator 13 and insulative member 14 functioning as the thermal shield.

Current collector 11 makes external terminal connection with the cell con-tainer 1 above insulative member 14 at area 18 of the cell container 1. Below area 18 and particularly between section 16 and the contact area of current collector 11 and anode 12, insulative members 14 and 15 prevent external elec-trical connection between current collector 11 and cell container 1. Such ll~S34~:

Shoult a short circuit condition occur, heat is concentrated in ~ection 16 of the current collector 11, particularly s$nce the thinned section provides a greater electrical re6istance. The heat contained fuses section 16 with the short circuit electrical connection being interrupted thereby, prior to excessive internal cell heat build-up and concomitant excesRive pressure.
Section 16 is preferably dimensioned to fuse at a 5 amp current load.
In a ~imilar manner aluminum cathode current collector 21 for carbona-ceous cathode 20 can function as the internal cell fuse by wrapping a portion thereof with a thermal shield and suitably dimensioning the fusing site.
It is understood that changes and variations in cell construction, current collector configuration, fusing ~ite and thermal shielding and the like can be made without departing from the scope of the present invention as defined in the following claims.

Claims (7)

The embodiments of the invention in which an exclusive property or privilege is claimed are defined as follows:
1. An electrochemical cell comprising a container containing a first electrode, a second electrode, a liquid electrolyte and one or more current collectors electrically connected to at least one of said electrodes with said current collector electrically engaged with a section of said con-tainer characterized in that a portion of said current collector between said electrical connection and electrical engagement is enclosed by thermal shielding means whereby excessive heat generated by ohmic dissipation with-in said current collector caused by a short circuit of said cell is retained within said portion to fuse said portion and interrupt the circuit.
2. The cell of claim 1 wherein said portion of said current collector is of a smaller cross section than the remainder of said current collector.
3. The cell of claim 2 wherein said thermal shielding means comprises a heat sealed film comprised of a polyolefin selected from the group consisting of polyethylene and polypropylene.
4. The cell of claim 1 wherein said first electrode is com-prised of lithium.
5. The cell of claim 4 wherein said electrolyte includes sulfur dioxide dissolved therein as a cathode depolarizer.
6. The cell of claim 1 wherein said portion is dimensioned such that it fuses when subjected to a current of S amperes.
7. The cell of claim 1 wherein said current collector comprises a metal selected from the group consisting of nickel and aluminum.
CA324,812A 1978-05-01 1979-04-03 Internal battery fuse Expired CA1115342A (en)

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
US901,404 1978-05-01
US05/901,404 US4188460A (en) 1978-05-01 1978-05-01 Internal battery fuse

Publications (1)

Publication Number Publication Date
CA1115342A true CA1115342A (en) 1981-12-29

Family

ID=25414102

Family Applications (1)

Application Number Title Priority Date Filing Date
CA324,812A Expired CA1115342A (en) 1978-05-01 1979-04-03 Internal battery fuse

Country Status (13)

Country Link
US (1) US4188460A (en)
JP (1) JPS5514691A (en)
BE (1) BE875951A (en)
CA (1) CA1115342A (en)
DE (1) DE2917328A1 (en)
DK (1) DK177379A (en)
FR (1) FR2425157A1 (en)
GB (1) GB2020089B (en)
IL (1) IL57047A (en)
IT (1) IT1112835B (en)
NL (1) NL7903289A (en)
NO (1) NO149013C (en)
SE (1) SE7903745L (en)

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US4879187A (en) * 1987-10-22 1989-11-07 Eveready Battery Company Battery terminal fuse
GB8815800D0 (en) * 1988-07-02 1988-08-10 Dowty Electronic Components Improvements relating to batteries
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FR2655479A1 (en) * 1989-12-04 1991-06-07 Accumulateurs Fixes High-power lithium cell
US5204194A (en) * 1992-05-21 1993-04-20 Magnavox Electronic Systems Company Multicell battery having a tab-fuse for overcurrent interruption
US5358798A (en) * 1993-12-06 1994-10-25 Motorola, Inc. Battery assembly having a thermal fuse
DE19529849C2 (en) * 1995-08-12 2003-12-24 Nbt Gmbh Electrochemical cells with protective device and accumulator with non-aqueous electrolytes
US5750277A (en) * 1996-04-10 1998-05-12 Texas Instruments Incorporated Current interrupter for electrochemical cells
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US6069551A (en) * 1997-05-02 2000-05-30 Therm-O-Disc, Incorporated Thermal switch assembly
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US5844464A (en) * 1997-11-24 1998-12-01 Therm-O-Disc, Incorporated Thermal switch
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US6239686B1 (en) 1999-08-06 2001-05-29 Therm-O-Disc, Incorporated Temperature responsive switch with shape memory actuator
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US6617953B2 (en) * 2001-03-26 2003-09-09 Wilson Greatbatch Ltd. Link fuse
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US20070048595A1 (en) * 2005-08-24 2007-03-01 Paul Graham Batteries
US9028986B2 (en) * 2009-01-07 2015-05-12 A123 Systems Llc Fuse for battery cells
US9413031B2 (en) * 2009-03-24 2016-08-09 Lenovo (Singapore) Pte. Ltd. Apparatus and system for an internal fuse in a battery cell
KR101254903B1 (en) 2011-06-07 2013-04-18 삼성에스디아이 주식회사 Battery pack with fuse part
KR101264579B1 (en) 2011-06-30 2013-05-14 로베르트 보쉬 게엠베하 Secondary battery Having Current Collector With Fuse Portion
JP5727090B2 (en) * 2012-03-15 2015-06-03 株式会社東芝 Lithium ion secondary battery
DE102013017228B3 (en) 2013-10-17 2015-04-23 Airbus Defence and Space GmbH Switching device for an electrochemical energy storage, electrochemical energy storage and energy storage system
JP6288057B2 (en) * 2015-12-02 2018-03-07 トヨタ自動車株式会社 Stacked all-solid battery
JP6766736B2 (en) 2017-04-05 2020-10-14 トヨタ自動車株式会社 All solid state battery
KR102569103B1 (en) * 2020-11-18 2023-08-23 주식회사 유앤에스에너지 Current collector for electrodes
CN115521267B (en) * 2022-08-26 2023-07-04 贵州大学 Benzenesulfonamide compound containing N-5-chloroisoxazole malonate structure, preparation method and application
CN115521271B (en) * 2022-08-26 2023-07-04 贵州大学 A chiral malonate compound containing N-isothiazolebenzenesulfonamide group, preparation method and use
CN115521270B (en) * 2022-08-26 2023-08-29 贵州工业职业技术学院 A kind of malonate compound containing N-oxazobenzenesulfonamide group, preparation method and application

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Also Published As

Publication number Publication date
SE7903745L (en) 1979-11-02
FR2425157B1 (en) 1985-02-08
DE2917328C2 (en) 1988-04-14
IL57047A (en) 1982-04-30
IL57047A0 (en) 1979-07-25
NO149013B (en) 1983-10-17
GB2020089A (en) 1979-11-07
NL7903289A (en) 1979-11-05
GB2020089B (en) 1982-08-04
BE875951A (en) 1979-10-30
JPS6333264B2 (en) 1988-07-05
JPS5514691A (en) 1980-02-01
US4188460A (en) 1980-02-12
IT7922249A0 (en) 1979-04-30
IT1112835B (en) 1986-01-20
DK177379A (en) 1979-11-02
FR2425157A1 (en) 1979-11-30
NO791378L (en) 1979-11-02
DE2917328A1 (en) 1979-11-15
NO149013C (en) 1984-01-25

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